Agricultural industrial waste has demonstrated potential as a soil acidity corrector and fertilizer, in addition to reducing environmental impacts caused by inadequate waste disposal. Ornamental rock waste is a sustainable alternative as it contains essential elements for plant growth. (1) Background: this study aims to evaluate using marble waste in SENA and the Gallo Crudo Quarry in Colombia as an acidity mitigator in soils cultivated with maize (Zea mays) in a greenhouse. (2) Method: four treatments were applied: T0: without marble dust—MD; three doses of MD (T1: 1.1 Mg of MD ha−1; T2: 2.2 Mg of MD ha−1; and T3: 3.3 Mg of MD ha−1). After 70 days, soil fertility analyses were carried out. (3) Results: The results show that the chemical properties of the soil improved with all treatments, mainly with T2, influencing the calcium (Ca), carbon (C), sulfur (S), and magnesium (Mg) contents. MD’s pH and Al + H values were higher than conventional treatments. The T2 treatment reduced soil acidity from 0.2 cmol + kg−1 to 0.0 cmol + kg−1 and increased pH to 7.91 compared to the control (5.4). The maize plants in the T2 treatment developed better, indicating that the dose of 2.2 Mg of MD ha−1 can replace commercial limestone. (4) Conclusions: This agroecological technique is an innovative alternative in Colombia, replicable in areas with ornamental rock reserves, benefiting the agricultural economy and contributing to target the Sustainable Development Goals, which promote sustainability, responsible management of natural resources, and a reduction in environmental impacts.
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