Cylindrical surface grinding can create defined textural patterns on a component with high quantity. This paper presents an experimental investigation of the frictional behaviours of ground cylindrical microstructural surfaces under a well lubrication condition. It shows that the coefficient of friction (COF) of microstructural surface is influenced by different workload and rotation speed. The results reveal that conventional surface roughness parameters do not present the influence of surface microstructure on friction performance well. However, the paper presents an interesting discovery that the friction behaviour of microstructural surfaces created by grinding could be controlled by combining dressing and grinding conditions. Such a discovery provides a logic way to reduce surface friction for energy efficiency applications. A few functional relationships have been established to illustrate the influence of microstructural features on friction. It was found that the ground microstructural surface could improve friction performance up to 20% compared to the smoother surfaces without defined surface textural patterns.