Concentrations Of 40K Research Articles

Radiological hazards assessment associated with granitoid rocks in Egypt

The present study aimed to assess the radioactive hazards associated with the application of granitoid rocks in building materials. An HPGe spectrometer was used to detect the levels of the radioactive elements uranium-238, thorium-232, and potassium-40 in the granitoid rocks. The results showed that the levels of these elements were lower (38.32 < 33 Bq kg−1), comparable (47.19–45 Bq kg-1) and higher (992.26 ≫> 412 Bq kg−1) than the worldwide limits for 238U, 232Th, and 40K concentration, respectively. The exposure to gamma radiation of granitoid rocks was studied by various radiological hazard variables like the absorbed dose rate (Dair), the outdoor and indoor annual effective dose (AEDout and AEDin), and excess lifetime cancer risk (ELCR). A variety of statistical methods, including Pearson correlation, principal component analysis (PCA), and hierarchical cluster analysis (HCA) was used, to study the relationship between the radioactive elements and the radiological hazards. According to statistical analysis, the main radioactive risk of granitoid rocks is contributed to by the elements uranium-238, thorium-232, and potassium-40. Granitoid rocks can be applied in building materials, but under control to prevent risk to the public.

Symkanych О.І., Коkhan О.P., Glukh О.S., Krch K.L., Lytvyn О.V., Svatiuk N.І., Butsyak І.V. MONITORING OF RADIONUCLIDE MIGRATION IN THE BOTTOM SEDIMENTS OF THE TISA BILA RIVER' SOURCE

The regularities of distribution, migration, and accumulation of natural gamma-active nuclides 40K, uranium 238U (214Pb, 214Bi), and thorium 232Th (212Pb, 212Bi, 228Ac, 208Tl) series, as well as man-made 137Cs in the sediments of the tributary of the Tysa River (Bila Tysa), have been established. It is shown that the total content of the studied radionuclides in the bottom sediments along the entire length of the Tysa River differs slightly and is proportional to the level of its siltation. And this largely depends on many factors, in particular - the intensity of radionuclide exchange processes between soil and water, the water content in the soil, organic substances, and the morphological features of the river. Fluctuations of the total specific activity of natural gamma-active radionuclides (excluding 40K) in sediments within the range of 195.5-293.9 Bq/kg were established. The highest content of these isotopes was determined at the confluence of the White and Black Tisza. Mapping of the studied territories according to the content of 40K and 137Cs has show that the area of accumulation of gamma-active nuclides is concentrated in the lower part of the river (the point of confluence of the White and Black Tisza), and the probable causes of this phenomenon were substantiated. The analysis of the degree of connection between the content of radionuclides (238U and 232Th, 40K and 137Cs series) and the territorial factor showed that for the majority of GAN there is a zonal distribution - in the bottom sediments of the river source.&#x0D; Keywords: radionuclides; gamma-active nuclides; radioecological monitoring; bottom deposits; migration; accumulation; Cs/K content; Tysa river.

Activity concentration and transfer of 226Ra, 232Th, and 40K from soil-to-crops in Irele Local Government Area of Ondo State, Southwestern Nigeria

The activity concentration of radionuclides in soil and crop samples obtained from Irele local government area in Ondo State, Southwestern Nigeria, was evaluated using a 760 mm x 760 mm NaI(Tl) gamma-ray detector system of model 8075, and resolution of 8 % at 0.662 MeV line of 137Cs. In addition, the radionuclide transfer from soil to crops was determined as a result. In soil samples, the mean activity concentrations of 226Ra, 232Th, and 40K were (21.81 ± 3.32, 12.10 ± 4.13, 381.02 ± 11.87Bqkg−1); (31.26 ± 3.98, 15.20 ± 3.82, 357.46 ± 14.62Bqkg−1); (29.81 ± 2.43, 18.86 ± 2.34, 504.25 ± 20.42Bqkg−1) and (27.44 ± 3.07, 21.54 ± 3.61, 449.48 ± 16.14Bqkg−1) corresponding to plantain, maize, yam and cassava, respectively. The mean activity concentration of 226Ra, 232Th, and 40K for plantain, maize, yam and cassava samples are (13.27 ± 4.58, 6.48 ± 3.94, 265.81 ± 13.19Bqkg−1); (27.03 ± 3.70, 10.72 ± 3.07, 345.70 ± 14.63Bqkg−1); (24.03 ± 4.65, 13.79 ± 4.25, 523.53 ± 16.43Bqkg−1) and (21.47 ± 3.57, 14.44 ± 2.20, 432.99 ± 18.56Bqkg−1), respectively. The mean transfer factor values of 226Ra, 232Th and 40K are (0.611, 0.536, 0.700); (0.867, 0.708, 0.967); (0.807, 0.736, 1.040) and (0.785, 0.668, 0.974) for soil-to-plantain, soil-to-maize, soil-to-yam, and soil-to-cassava, respectively. The results revealed that the transfer factor of the crop samples is in the following order: yam>cassava>maize>plantain. The activity concentrations of 226Ra, 232Th, and 40K in the soil and crop samples and corresponding soil-to-crop transfer values did not cause radiation damage to human health as reported levels were below recommended limits. The results of this study may serve as the basis and future criteria for the radionuclide concentrations in soil and their migration factors for the various crops in the study area.

Assessment of radioactivity in sand samples from eastern Nepal in perspective of radiological hazards.

This study was conducted to investigate the activity concentrations of 226Ra, 232Th and 40K in the sand samples and the health hazards associated with them utilizing a NaI (Tl) gamma spectrometer. The average activity concentrations of 226Ra, 232Th and 40K were found to be 24.8±10.1, 39.8±16.4 and 531.3±52.8Bq kg-1, respectively. The calculated radiological hazard parameters, including radium equivalent activity, absorbed gamma dose and effective dose rate, were found to be 122.7±34.0Bq kg-1, 57.7±14.9 nGy h-1 and 0.3±0.1mSv y-1, respectively. Notably, these results were observed to be below the recommended thresholds. Other measured hazard indices were also lower than the prescribed values. From a radiological perspective, the present study concludes that the sand samples do not pose any threat to human health when utilized as a building material.

A preliminary study on determination of radioactivity levels and estimation of the annual effective dose in dried fruits consumed in Albania.

This work aimed to support Albania's food safety monitoring regime. In this context, the natural and artificial radioactivity was measured in 20 samples of dried fruits collected randomly in different markets of Tirana. The activity concentration of 40K, 226Ra, 232Th and 137Cs was determined by using the high-purity germanium detector. The maximum values of activity concentration in dried fruits were calculated as 517±22Bqkg-1 for 40K, 11.10±0.93Bqkg-1 for 226Ra, 4.38±0.26Bqkg-1 for 232Th and 0.83±0.14Bqkg-1 for 137Cs. The average values of activity concentration of 40K and 226Ra were 269and 6.05Bqkg-1 and the average effective dose to individuals from the intake of the dried fruits was 44μSv y-1. All average values in this study were lower than recommended values by reports United Nations Scientific Committee on the Effect of Atomic Radiation, World Health Organization and International Commission on Radiological Protection for all age groups. Therefore, all dried fruit samples in this study are safe for consumption with acceptable radiological risk and none of them pose any significant radiological impact. The obtained data in this paper and information for levels of radioactivity and ingestion absorbed dose from dried fruits can be used to be the basic data for future comparative analysis of the other studies.

Assessment of gamma absorbed doses and radiological risk indexes from soil radioactivity around the phosphate area in south Tunisia.

Human beings are constantly exposed to the radiations coming from the environment. This work assesses the radiological hazards of natural radioactivity in soil samples taken at four locations around the phosphate area in south Tunisia. Concentrations of primordial radionuclides were measured by gamma spectrometer using an HPGe detector. The overall mean values of 40K, 226Ra and 232Th concentrations were 264, 27 and 13Bqkg-1, respectively. From the radioactivity measurements, radiation hazard indices specified by the United Nation Scientific Committee on the Effect of Atomic Radiation such as radium equivalent activity (Raeq), absorbed dose rates ($ {\dot{\text D}} $) and annual effective dose (AED) to the population for outdoor environment were determined. The mean values for the abovementioned parameters were 64Bqkg-1, 33 nGy h-1 and 40μSv y-1, respectively.

Environmental Radioactivity, Ecotoxicology (238U, 232Th and 40K) and Potentially Toxic Elements in Water and Sediments from North Africa Dams

The natural radioactivity of 238U, 232Th and 40K was measured in water and sediment samples collected from Sidi Salem dam (Tunisia) and Aïn Dalia dam (Algeria) in the Tuniso-Algerian transboundary basin. The samples were measured using a TERRA detector of gamma, beta, and alpha rays, and atomic absorption and gamma-ray spectrometry were used to analyze the levels of radionuclides and toxic elements, respectively. Potentially toxic elements (Fe, Pb, Zn, Ni, Cr, Cu and Cd) and associated health risks in surface water and sediment of dams were investigated in this present study. The concentrations of Fe, Pb, Zn, Ni, Cr, Cu and Cd in surface water ranged from 5.430 to 9.700 mg·L−1, 0.022 to 0.168, 0.018 to 0.142, 0.065 to 0.366, BDL to 0.0351, BDL to 0.071 and BDL to 0.048 mg·L−1, respectively. In the sediments, the concentrations of Fe, Pb, Zn, Cu, Ni, Cd and Cr were of the order of 136.7, 3.41, 3.22, 0.213, 0.182, 0.15 mg·L−1 and BDL, respectively. The mean radioactivity rates in the water samples were 1.72, 0.068 and 94.6 Bq·L−1 for 238U, 232Th and 40K, respectively (Tunisia dam), and were 1.9, 0.09 and 131.43 Bq·L−1 for 238U, 232Th and 40K, respectively (Algeria dam). The mean 238U, 232Th and 40K radioactivity concentrations measured in the sediment samples were 2.67, 0.18 and 197.87 Bq·kg−1, respectively (Tunisian dam), and were 4.34, 0.27 and 287.61 Bq·kg−1, respectively (Algeria dam). The activity concentration of 40K was higher than that of 238U and 232Th for the water and sediment samples. The activity concentrations follow the order 40K &gt; 238U &gt; 232Th. The cumulative impact of these radio-geochemical elements can cause immediate serious problems in the ecosystem due to their high potential toxicity to the environment and human health in this study area and can be transposable to any other similar region. A good knowledge of monitoring quality and quantity for transboundary water resources and international collaborations are essential to safeguard human health (women’s breast cancer, thyroid cancer, neurological impact) and avoid conflicts, especially during climatic upheavals of drought.

Fractionation of environmental radioactivity in road dust from a megacity: external and internal health risks.

Naturally occurring radioactive materials (NORMs: 232Th, 226Ra, 40K) can reach our respiratory system by breathing of road dust which can cause severe health risks. Targeting the pioneering consideration of health risks from the NORMs in road dust, this work reveals the radioactivity abundances of NORMs in road dust from a megacity (Dhaka) of a developing country (Bangladesh). Bulk chemical compositions of U, Th, and K obtained from neutron activation analysis were converted to the equivalent radioactivities. Radioactivity concentrations of 226Ra, 232Th, and 40K in road dust ranged from 60-106, 110-159, and 488-709Bqkg-1 with an average of 84.4 ± 13.1, 126 ± 11, and 549 ± 48Bqkg-1, respectively. Estimated 226Ra, 232Th, and 40K radioactivities were, respectively, 1.7-3.0-, 3.7-5.3-, and 1.2-1.8-folds greater than the affiliated world average values. Mechanistic pathway of NORMs' enrichment and fractionation relative to the major origin (pedosphere) were evaluated concerning the water logging, relative solubility-controlled leaching and translocation, climatic conditions, and aerodynamic fractionations (dry and wet atmospheric depositions). Computation of customary radiological risk indices invokes health risks. Noticing the ingress of NOMR-holding dust into the human respiratory system along with the associated ionizing radiations, the computed radiological indices represent only the least probable health hazards. Nevertheless, in real situations, α-particles from the radioactive decay products of 232Th and 238U can create acute radiation damages of respiratory system. Policymakers should emphasize on limiting the dust particle evolution, and public awareness is required to alleviate the health risks.

Age-dependent annual effective dose and radiological health risk from salt and soil collected from Padag, Chaghi, Balochistan, Pakistan

ABSTRACT This study aimed to investigate the annual effective dose for different age groups and health hazards associated with natural radioactivity in salt and soil collected from Padag, Chaghi, Balochistan. All samples were analysed by using high-purity germanium (HPGe) and sodium iodide (NaI) detectors. The average values of concentration of 226Ra, 232Th and 40K in salt samples were found to be 10.49, 9.6 and 169.65 Bq.kg−1, respectively, using HPGe detector, while in case of NaI detector, these values were found to be 10.48, 9.89 and 161.73 Bq.kg−1, respectively. Similarly, the average values of concentration of 226Ra, 232Th and 40K in soil were found to be 24.59, 24.89 and 391.72 Bq.kg−1, respectively, using HPGe detector, while in case of NaI detector, these values were found to be 24.46, 24.71 and 358.31 Bq.kg−1, respectively. Significant correlations were found between the results obtained from HPGe and NaI detectors. The values of total annual effective dose due to ingestion of salt were found to be 2.46 × 10−5, 2.45 × 10−5, 3.55 × 10−5 and 1.13 × 10−5 μSv.y−1 using HPGe detector and 2.43 × 10−5, 2.44 × 10−5, 3.55 × 10−5 and 1.13 × 10−5 μSv.y−1 using NaI detector for the age groups (2–7 years), (7–12 years), (12–17 years) and (≥17 years), respectively. The highest value of annual effective dose was found in the age group 12–17 years and minimum was found in the age group ≥ 17 years. However, all values were found to be below the recommended value of 0.29 mSv. Total average radiological risk due to ingestion of salt for all age groups was found to be lower than the reported value.

Evaluation of Natural Radioactivity Level in Surface Soil from Bambasi District in Benishangul Gumuz Region, Ethiopia.

The study assessed the concentration of natural radionuclides in soil samples from the Bambasi district in Ethiopia's Benishangul Gumuz region using a gamma-ray spectrometer equipped with a high-purity germanium (HPGe) detector. The measured activity concentrations of 238U, 232Th, and 40K in soil samples varied from 46.2 ± 2.25 to 88.49 ± 5.73 Bq/kg, 73.4 ± 4.12 to 119.65 ± 8.45 Bq/kg, and 176.78 ± 8.63 to 396.71 ± 25.39 Bq/kg, respectively. The average concentration of 238U and 232Th exceeded the recommended worldwide population weighted average values of 32.0 and 45.0 Bq/kg, respectively, while the average concentration of 40K was below the recommended value of 420.0 Bq/kg. The mean absorbed dose rate was calculated to be 91.6 ± 5.1 nGy/h, which is above the recommended safe value of 59 nGy/h. The average annual effective dose equivalents for indoor and outdoor exposure were determined to be 2.65 ± 0.14 mSv/y and 0.66 ± 0.1 mSv/y, respectively. The calculated mean values of the internal hazard index, external hazard index, and gamma index across all soil samples were 0.72 ± 0.05, 0.55 ± 0.02, and 0.72 ± 0.02, respectively, all below the recommended safe threshold of one. These findings suggest that the activity concentrations observed in the soil samples exceed safe levels, indicating the necessity for further investigation into radioactivity levels and epidemiological studies regarding potential hazards from high background radiation.

Evaluation of Radioactivity Contents and Excess Lifetime Cancer Risk Due to Ingestion from Natural Radionuclides in Maize Samples from Some Selected Maize Farms in Ekiti State, Nigeria

The study was carried out to evaluate the radioactivity concentrations of 40K, 232Th and 238U in five maize samples collected from maize farms within Ekiti State, Nigeria. The activity concentration measurements were determined using n – type co-axial HPGe detectors for the state. The activity concentrations were found to vary from 994.67 – 2457.01 Bq Kg-1 for 40K, 32.84 – 91.88 Bq kg-1 for 232Th and 43.21 – 97.77 Bq kg-1 for 238U respectively. The annual effective dose to individuals from the consumption of the Maize was estimated on the basis of the measured radionuclides content in the food crop which ranged between 0.41 and 1.51 m Svy-1 respectively. The value1.04 m Svy-1 were obtained for the state as the mean total annual effective dose. The mean excess life time cancer risk was also calculated to be 2.06x10-9 . The value was compared with the internationally acceptable limits and found to be far less to the maximum permissible dose of 1.0 x10-3 recommended for the public by the United Nations Scientific Committee on the Effects of Atomic Radiation. Hence, the maize was found to be safe for human consumption.

Assessment of natural radioactivity in soil and olive mill pomace utilizing nal (TI) gamma-ray spectrometry and low background alpha/beta counting system

The study conducted in the northwest region of Jordan aimed to assess the levels of natural radioactivity in soil and olive mill pomace (OMP) samples. The researchers used Nal (TI) gamma-ray spectrometry to measure the activity concentrations of 226Ra, 232Th, 40K, and 137Cs in the samples. The average activity concentrations of 226Ra, 232Th, 40K, and 137Cs in the soil samples were found to be 18.624 ± 5.82, 12.276 ± 5.728, 518.33 ± 212.57, and 0.140 ± 0.09 (Bq,kg−1), respectively. In the OMP samples, the average activity concentrations of 226Ra, 232Th, and 40K were 7.272 ± 4.386, 3.454 ± 1.503, and 169.997 ± 81.873 (Bqkg−1), respectively, and no 137Cs was detected.The study also investigated fundamental parameters associated with radon, specifically the radon emanation coefficient (RnEC) and radon mass exhalation rate (Ex). The RnEC values ranged from 0.621 to 0.78 (Bqkg−1), with an average value of 0.71 ± 0.06 (Bqkg−1). The estimated Ex from the soil samples ranged from 65.83 to 124.86 (mBqkg−1h−1), with an average value of 99.74 ± 21.73 (mBqkg−1h−1).Regarding radiological hazards, the study examined various parameters, including radium equivalent activity, external and internal hazard indices, gamma and alpha indices, absorbed gamma dose rate, and excess lifetime cancer risk. All of these assessed values were found to be below the worldwide recommended limits for radiological safety.Additionally, the study analyzed the concentrations of gross alpha and gross beta radioactivities in soil and OMP samples. The soil samples had an average gross alpha activity of 4.642 ± 1.04 (Bqkg−1) and an average gross beta activity of 48.13 ± 14.50 (Bqkg−1). The OMP samples showed an average gross alpha activity of 0.32 ± 0.27 (Bqkg−1) and an average gross beta activity of 59.19 ± 12.94 (Bqkg−1).Overall, the obtained results are crucial for evaluating the radiological risks associated with natural radioactivity in the northwest region of Jordan. The findings establish baseline data for comparison and reference for radioactivity levels in the environment.

MEASUREMENT OF NATURAL RADIOACTIVITY IN TAP WATER SAMPLES FOR SELECTED REGIONS IN ADEN GOVERNORATE, YEMEN

In the present work, we have measured specific activity concentrations of in eleven tap water samples for selected regions in Aden governorate by using high purity germanium detector (HPGe). The (HPGe) detector (CANBERA-model 7229N, USA) with an efficiency of 35% and energy resolution (2.6keV) at energy (1332.6keV) for 60Co, the high purity N-type semiconductor detector with physical characteristics of (geometry closed-end coaxial, (3×3 inch). The results have shown that, The highest value of specific activity concentration of 226Ra was found in in T7 Daar-Saad region which was equal to (0.525±0.29)Bq/L, while the lowest value of specific activity concentration of 226Ra was found in T11 Aden Assughra region which was equal to (0.017±0.006)Bq/L with an average value of (0.228±0.13)Bq/L. The highest value of specific activity concentration of 232Th was found in in T5 Khor-makser region which was equal to (0.319±0.18)Bq/L, while the lowest value of specific activity concentration of 232Th was found in T11 Aden Assughra region which was equal to (0.009±0.001)Bq/L with an average values of (0.129±0.089)Bq/L. The highest value of specific activity concentration of (40K) was found in in T2 (Al-Ma,allah) region which was equal to (0.4±0.26)Bq/L, while the lowest value of specific activity concentration of (40K) was found in T11 Aden Assughra region which was equal to (0.027±0.004)Bq/L with an average values of (0.141±0.021)Bq/L respectively. The annual ingestion effective dose (AED) ranged from (3.05 to 98.77μSv/y), (5.67 to 178.16μSv/y), and (3.41 to 119.08μSv/y), with average values of 42.65μSv/y, 78.62μSv/y and 48.62μSv/y, for infants, children and adults respectively. The excess lifetime cancer risk (ELCR) have been calculated, its values were lower than the world’s average value of (0.29×10−3) as reported by EPA. The overall annual effective dose and cancer risks corresponding to radionuclide intake in tap water were below the recommended maximum values. It was inferred from the findings of this study that the water used as the sample does not have any significant radiological impacts to human body and is safe to be used as drinking water.

Estimation of Radiation Dose in Building Materials Used In Federal University Gusau Using Gamma-Ray Spectroscopy Analysis

This study estimated the radiation dose in building materials (sand, cement, and granite) in Federal University Gusau, Zamfara State, Nigeria, through gamma-ray spectrometry system using a Sodium Iodide Thallium activated "NaITl" detector in a low background configuration. The range of the average activity concentration of 226Ra was found to be 56.65±0.75Bqkg-1 to 159.45±2.68Bqkg-1, which was higher than that of the world mean value for soil 35Bqkg-1,for 232Th the range was 46.65±0.45Bqkg-1 to 79.32±1.68Bqkg-1, all the samples, were found to be higher than that of the world mean for soil 30Bqkg-1. While the activity concentrations of 232Th levels of blocks, granite, and sand samples are all above the world range, except the cement which was within the worldwide range 194.84±1.31Bqkg-1 to 656.84±0.76Bqkg-1. The average activity concentration of 40K for cement, sand, and blocks was within the worldwide range, with granite samples slightly higher than the world mean value for soil 400Bqkg-1. The results have been compared with the world mean values of 35, 30, and 400Bqkg-1 specified by the UNSCEAR (2016). Concerning radiological risk to human health, the absorbed gamma dose rate (D) was estimated to be above the world average range of 55nGyh-1; the outdoor annual effective dose equivalent (AEDE) were, estimated to be below the permissible limit of 0.07mSvy-1. The values of Raeq, Hex, and Hin for all the samples in the present work are lower than the accepted safety limit value of 370Bqkg-1 and below the limit of unity, respectively.

Assessment of the radiological health risk from radionuclide presence and transfer factor from soil to corn in some selected non-oil producing riverine areas of Akwa Ibom state

The main objective of this study was to estimate the activity concentration (AC) of 238U, 232Th and 40K, assess the health risk information from radionuclides presence in the soil and corn and the transfer influence from soil to corn. The key device used for the analysis was a Sodium Iodide Thallium detector. 238U AC in soil ranges from 14.09±0.27 Bqkg-1 to 18.70±0.31 Bqkg-1 with mean value of 15.69±0.28 Bqkg-1; 238U AC in corn varies from 9.36±0.22 Bqkg-1 to 14.78±0.27 Bqkg-1 with mean value of 11.53±0.24 Bqkg-1. 232Th AC in soil is from 12.32±0.46 Bqkg-1 to 48.76±0.91 Bqkg-1 with mean value of 35.97±0.76 Bqkg-1. 232Th AC in corn ranges from 8.26±0.37 Bqkg-1 to 35.19±0.77 Bqkg-1 with average value of 17.86±0.53 Bqkg-1. 40K values from the soil samples varies from 313.61±6.81 Bqkg-1 to 472.63±8.36 Bqkg-1 with mean value of 384.672±7.52 Bqkg-1. 40K varies from 374.85±7.45 Bqkg-1 to 478.55±8.41 Bqkg-1 with average value of 425.51±7.93 Bqkg-1from corn samples. The mean transfer factor for 238U, 232Th and 40K was obtained as 0.73, 0.62 and 1.13 respectively. The mean values for the Radium equivalent, absorbed dose, annual effective dose, and excess lifetime cancer risk from soil are 96.75 Bqkg-1, 47.05 nGyh-1, 0.06 mSvy-1, 0.20×10-3 correspondingly [values from corn are 69.83 Bqkg-1, 35.04 nGyh-1, 0.04 mSvy-1, 0.15×10-3 respectively]. These values clearly showed, the radiation doses exposed to Akwa Ibomites through the consumption of corn cultivated in these areas and inhalation of soil poses no effect to their health. Therefore, there is no radiological risk of ingestion.

Radioactivity levels, soil-to-grass and grass-to-milk transfer factor of natural radionuclides from grazing area in Erbil governorate, Iraq

The levels of naturally occurring radionuclides in soil, grass, and milk were measured in this study in order to calculate the transfer factor of radionuclides from soil to grass and grass to milk obtained from Erbil governorate in Iraq. High efficiency gamma spectrometry used for the measurement. It has been determined that the mean activity concentrations of 232Th, 226Ra, and 40K are 3.08, 8.37, and 253 BqKg−1 in soil, 0.5, 0.39, and 203.05 BqKg−1, in grass, and 0.29, 0.084, and 29.69 BqL−1, in milk, respectively. For soil to grass, the transfer factor values for 232Th, 226Ra, and 40K were found to be 0.18, 0.052, and 0.84, respectively, for soil to grass. For grass to milk, the transfer factor values for 232Th, 226Ra, and 40K were found to be 0.45, 0.166, and 0.11 dayL−1, respectively. The average transfer factor for 232Th, 226Ra, and 40K in all samples were lower than the world average value.

Determine the hazards of radioactive elements and radon gas manufacturing processes in an Egyptian fertilizer factory

This study investigated the levels of radioactivity in soil surrounding a phosphate fertilizer factory in Egypt, aiming to assess potential risks to the population exposed to radiation. Concentrations of 238U, 226Ra, 232Th, and 40K were measured in soil samples collected from two subsites: one near the factory (subsite 1) and another further away (subsite 2). Two different systems were used for measuring radioactivity, a high-purity gamma ray spectroscopy system with an HPGe detector for gamma-emitting isotopes and a CR-39 solid nuclear track detector for alpha-emitting radon gas. Subsite 1, located close to the factory, displayed significantly elevated levels of 226Ra compared to global background levels (514 and 456 Bq/kg vs. 35 Bq/kg). Additionally, the concentrations of 238U (241.06 Bq/kg vs. global average 35 Bq/kg), 232Th (16.15 Bq/kg vs. global average 30 Bq/kg), and 40K (146.36 Bq/kg vs. global average 400 Bq/kg) were all above global averages. Furthermore, a high concentration of radon gas (337.06 μSv/y) was measured at subsite 1. The strong positive correlation observed between 226Ra and 238U (0.96256) provides further evidence of potentially elevated radioactivity levels near the factory. In contrast, subsite 2, situated farther from the factory, exhibited natural radioactive background levels within international limits. Quantitative analysis revealed that gamma ray absorbed doses for 226Ra and 232Th exceeded global averages in some samples. Specifically, 226Ra doses ranged from 7.8 to 46.26 ppm (exceeding the 20 ppm global average in some cases), and 232Th doses ranged from 1.98 to 9.14 ppm (exceeding the 10 ppm global average in some cases). The concentration of 40K, however, remained within the global range (0.07%–0.69 %). The observed imbalances in the ratios of Th/U (0.17–0.24 Bq/kg and 0.73–0.24 ppm) and U/Ra (0.81–0.73 Bq/kg and 0.73–0.17 ppm), both of which are significantly lower than their respective global averages of 4 and 2.4, point towards the presence of fertilizer-derived contamination. This conclusion is further supported by the high phosphate concentrations detected in the samples. Overall, this study suggests that radioactive contamination near the phosphate fertilizer factory significantly exceeds global background levels and international limits in some cases. This raises concerns about potential risks posed to surrounding agricultural land and crops.

Assessment of natural radioactivity levels and potential radiological risks of commonly used building materials in Uttara Kannada District, Karnataka, India.

The main goal of this study is to evaluate the natural radioactivity and potential radiological risks of frequently used building materials in Uttara Kannada district. Using an High purity Germanium Detector (HPGe) detector-based gamma-ray spectrometer, the activity concentration of 226Ra, 232Th and 40K was determined. The activity concentration of 226Ra, 232Th and 40K in the construction materials vary from 13.78±0.90 to 151.9±1.85, 14.21±0.80 to 207.72±2.9 and 55.26±1.20 to 1298.24±25Bqkg-1 with an average value of 40.57±1.37,60.13±1.70 and 425.38±4.75Bqkg-1 having a geometric mean of 33.07, 46.49 and 290.20Bqkg-1, respectively. The mean annual effective dose equivalent was found to be 0.68mSv y-1 and is less than the International Commission on Radiological Protection proposed acceptable limit of 1mSv y-1. The estimated radiological hazard parameters show that these building materials are safe to use in the construction of homes and do not offer a substantial source of radiation hazard.

Uranium Isotope Characterization in Volcanic Deposits in a High Natural Background Radiation Area, Mamuju, Indonesia

Mamuju is an area of high natural radiation in Indonesia with high natural radiation levels (average 613 nSv h−1). Mamuju is anomalous due to its high average 238U and 232Th concentrations of 22,882 and 33,549 Bq kg−1, respectively, in laterite and rock. High natural radionuclide concentrations of 238U, 232Th, and 40K have also been reported in soil samples from several locations in Mamuju, including Botteng, Northern Botteng, Takandeang, Ahu, and Taan. High radiation levels are related to radioactive mineral occurrences in the Adang volcanic complex, comprised of phonolitoid and foiditoid lithologies. According to the International Atomic Energy Agency (IAEA), uranium deposits can be classified into several types, among them a volcanic-related deposits, which include three sub-types: stratabound, structure-bound, and volcano-sedimentary deposits. This study aims to characterize volcanic rock deposit sub-types in the Mamuju area based on uranium radioisotope measurements. The uranium isotopes were measured using a tandem quadrupole inductively coupled plasma mass spectrometer combined with chemical separation by extraction chromatography using UTEVA resin. The analytical results for the 234U/238U ratios are used to determine the formation characteristics of minerals in each deposit sub-type based on mineral formation age, post-formation processes, and disturbances that affected the formation processes. Based on geochronological calculations using 234U/238U mineralization age, the deposits in the Mamuju area are 0.914–1.11 million years old and are classified as recent mineralization. These data have important implications for tracing uranium source rocks in the Mamuju area and may explain the anomalously high radiation levels in the Mamuju area.

Radioactivity of 226Ra, 232Th and 40K in soil in Northwest part of Turkey: assessment of radiological impacts

Abstract The surface soil samples were collected from Northwest Turkey. The activity concentrations of 226Ra, 232Th, and 40K were measured using an HPGe gamma-spectroscopy system. The activity concentrations of 226Ra, 232Th, and 40K in the soils were found to be in the range of 11.78 ± 1.12–43.89 ± 14.94, 3.19 ± 2.01–88.22 ± 0.92, 362.81 ± 5.94–829.27 ± 12.38 Bq kg−1 d.w., respectively. The Surfer program was used to obtain 3-dimensional maps of the specific activities. Radium Equivalent Activity (Raeq), Absorbed Gamma Dose Rate (D), Annual Effective Dose Equivalent (AEDE), The Excess Life Time Cancer Risk (ELCR), External (H ex) and Internal (H in) Hazard Indexes, Annual Gonadal Dose Equivalent (AGDE), and Activity Utilization Index (AUI) were calculated and compared with the recommended values. Pearson’s correlation analysis (PCA) and factor analysis (FA) were utilized to analyze the data and indicate between the radiological parameters. The analysis showed that the total radiation was mainly caused by 226Ra and 232Th.