With the remarkable advances in vertical-cavity surface-emitting lasers (VCSELs) in recent decades, VCSELs have been considered promising light sources in the field of optical wireless communications. However, off-the-shelf VCSELs still have a limited modulation bandwidth to meet the multi-Gb/s data rate requirements imposed on the next-generation wireless communication system. Recently, employing machine learning (ML) techniques as a method to tackle such issues has been intriguing for researchers in wireless communication. In this work, through a systematic analysis, it is shown that the ML technique is also very effective in VCSEL-based visible light communication. Using a commercial VCSEL and bidirectional long short-term memory (Bi-LSTM)-based ML scheme, a high-speed visible light communication (VLC) link with a data rate of 13.5 Gbps is demonstrated, which is the fastest single channel result from a cost-effective, off-the-shelf VCSEL device, to the best of the authors’ knowledge.