Coherent Transfer Research Articles

Major depressive disorder diagnosis based on effective connectivity in EEG signals: a convolutional neural network and long short-term memory approach.

Deep learning techniques have recently made considerable advances in the field of artificial intelligence. These methodologies can assist psychologists in early diagnosis of mental disorders and preventing severe trauma. Major Depression Disorder (MDD) is a common and serious medical condition whose exact manifestations are not fully understood. So, early discovery of MDD patients helps to cure or limit the adverse effects. Electroencephalogram (EEG) is prominently used to study brain diseases such as MDD due to having high temporal resolution information, and being a noninvasive, inexpensive and portable method. This paper has proposed an EEG-based deep learning framework that automatically discriminates MDD patients from healthy controls. First, the relationships among EEG channels in the form of effective brain connectivity analysis are extracted by Generalized Partial Directed Coherence (GPDC) and Direct directed transfer function (dDTF) methods. A novel combination of sixteen connectivity methods (GPDC and dDTF in eight frequency bands) was used to construct an image for each individual. Finally, the constructed images of EEG signals are applied to the five different deep learning architectures. The first and second algorithms were based on one and two-dimensional convolutional neural network (1DCNN-2DCNN). The third method is based on long short-term memory (LSTM) model, while the fourth and fifth algorithms utilized a combination of CNN with LSTM model namely, 1DCNN-LSTM and 2DCNN-LSTM. The proposed deep learning architectures automatically learn patterns in the constructed image of the EEG signals. The efficiency of the proposed algorithms is evaluated on resting state EEG data obtained from 30 healthy subjects and 34 MDD patients. The experiments show that the 1DCNN-LSTM applied on constructed image of effective connectivity achieves best results with accuracy of 99.24% due to specific architecture which captures the presence of spatial and temporal relations in the brain connectivity. The proposed method as a diagnostic tool is able to help clinicians for diagnosing the MDD patients for early diagnosis and treatment.

Long-distance coherence of Majorana wires

Theoretically, a pair of Majorana bound states in a topological superconductor forms a single fermionic level even at large separations, implying that the parity information is stored nonlocally. The nonlocality leads to a long-distance coherence for electrons tunneling through a Coulomb blockaded Majorana wire [Fu, Phys. Rev. Lett. 104, 056402 (2010)], an effect that can be observed, e.g., in an interferometer. Here, we examine theoretically the coherent electron transfer, taking into account that tunneling implies the long-distance transfer of charge, which is carried by one-dimensional plasmons. We show that the charge dynamics does not affect the coherence of the electron tunneling process in a topological superconductor consisting of a semiconductor wire proximitized by a single bulk superconductor. The coherence may be strongly suppressed, however, if the topological superconductivity derives from a semiconductor wire proximitized by a granular superconductor.

Optomechanical discrete-variable quantum teleportation scheme

We propose an experimental protocol to realize discrete variable quantum teleportation using optomechanical devices. The photonic polarization superposition state of a single photon is teleported to a phononic superposition of two micromechanical oscillators by means of photon/phonon entanglement generation and optical Bell state measurement using two-photon interference. Verification of the protocol is performed by coherent state transfer between the mechanical devices and light. Simulations show the feasibility of the proposed scheme at millikelvin temperatures using state-of-the-art gigahertz optomechanical devices.

Noncontact Spin Pumping by Microwave Evanescent Fields.

The angular momentum of evanescent light fields has been studied in nano-optics and plasmonics but not in the microwave regime. Here we predict noncontact pumping of electron spin currents in conductors by the evanescent stray fields of excited magnetic nanostructures. The coherent transfer of the photon to the electron spin is proportional to the g factor, which is large in narrow gap semiconductors and surface states of topological insulators. The spin pumping current is chiral when the spin susceptibility displays singularities that indicate collective states. However, 1D systems with linear dispersion at the Fermi energy, such as metallic carbon nanotubes, are an exception since spin pumping is chiral even without interactions.

Light‐Harvesting Supramolecular Polymers: Energy Transfer to Various Polyaromatic Acceptors

A supramolecular light‐harvesting antenna consisting of 3,6‐disubstituted phosphodiester‐linked phenanthrene trimers (donors) was doped with different charged and uncharged polyaromatic and heteroaromatic acceptor chromophores. Excitation of the phenanthrene moieties is followed by energy transfer to the acceptor molecules and radiative relaxation. The self‐assembled fiber structure of the phenanthrene trimers is not altered by the dopant, as verified by atomic force microscopy (AFM). Among several neutral and cationic acceptor chromophores, benzo(a)pyrene emerged as one of the highest fluorescence quantum yields, reaching 31 % at a chromophore/phenanthrene ratio of 12 mol‐%. The energy transfer is probably a combination of Förster resonance energy transfer (FRET) and a coherent energy transfer mechanism.

Coherent Transfer of Spin Angular Momentum by Evanescent Spin Waves within Antiferromagnetic NiO.

Insulating antiferromagnets have recently emerged as efficient and robust conductors of spin current. Element-specific and phase-resolved x-ray ferromagnetic resonance has been used to probe the injection and transmission of ac spin current through thin epitaxial NiO(001) layers. The spin current is found to be mediated by coherent evanescent spin waves of GHz frequency, rather than propagating magnons of THz frequency, paving the way towards coherent control of the phase and amplitude of spin currents within an antiferromagnetic insulator at room temperature.

Perfect coherent transfer in an on-chip reconfigurable nanoelectromechanical network

Realizing a controllable network with multiple degrees of interaction is a challenge to physics and engineering. Here, we experimentally report an on-chip reconfigurable network based on nanoelectromechanical resonators with nearest-neighbor (NN) and next-nearest-neighbor (NNN) strong couplings. By applying different parametric voltages on the same on-chip device, we carry out perfect coherent transfer in NN and NNN coupled array networks. Moreover, the low-loss resonators ensure the desired evolution to achieve perfect transfer and the demonstration of the parity-dependent phase relation at transmission cycles. The realization of NNN couplings demonstrates the capability of engineering coherent coupling beyond a simple model of a NN coupled array of doubly clamped resonators. Our reconfigurable nanoelectromechanical network provides a highly tunable physical platform and offers the possibilities of investigating various interesting phenomena, such as topological transport, synchronization of networks, as well as metamaterials.

Manifestation of the Transfer of Coherence in Spectroscopy: A New Paradigm of Spin Exchange and Its Manifestations in EPR Spectra

The transfer of spin coherence leads to surprising effects in electron paramagnetic resonance (EPR) spectroscopy. This is demonstrated by the example of quantum coherence transfer caused by exchange interaction in bimolecular collisions of paramagnetic particles in dilute solutions. Detailed analysis of the role of quantum coherence transfer has altered the paradigm of spin exchange and its manifestation in the EPR spectra of solutions of paramagnetic particles.

Vibronic Quantum Beating between Electronic Excited States in a Heterodimer.

Energy transfer in multichromophoric molecules can be affected by coherences that are induced by the electronic and vibrational couplings between chromophore units. Coherent electron-vibrational dynamics can persist at the subpicosecond time scale even at room temperature. Furthermore, wave-like localized-delocalized motions of the electronic wave function can be modulated by vibrations that actively participate in the intermolecular energy transfer process. Herein, nonadiabatic excited state molecular dynamics simulations have been performed on a rigid synthetic heterodimer that has been proposed as a simplified model for investigating the role and mechanism of coherent energy transfer in multichromophoric systems. Both surface hopping (SH) and Ehrenfest approaches (EHR) have been considered. After photoexcitation of the system at room temperature, EHR simulations reveal an ultrafast beating of electronic populations between the two lowest electronic states. These oscillations are not observed at low temperature and have vibrational origins. Furthermore, they cannot be reproduced using SH approach. This periodic behavior of electronic populations induces oscillations in the spatial localization of the electronic transition density between monomers. Vibrations whose frequencies are near-resonant with energy difference between the two lowest electronic excited states are in the range of the electronic population beating, and they are the ones that contribute the most to the coherent dynamics of these electronic transitions.

European compact against tax fraud—VAT solidarity and new dimension of effective and coherent tax data transfer

The aim of this article is to present a new concept and scope of exchange of VAT information/data and tax technologies between EU Member States, better designed to combat VAT fraud. In the authors’ view, bilateral agreements on strengthened cooperation are a more effective solution—at least in the short and medium term—than EU legislation. Bilateral agreements in the field of VAT already exist between some EU Member States and work effectively for the better and more structured exchange of tax data. Effective cooperation based on bilateral agreements/intergovernmental agreements could positively influence EU legislation and serve as an effective sandbox for the introduction of new common solutions for the EU legislator.

Generation and Manipulation of Superoscillatory Hotspots Using Virtual Fourier Filtering and CTF Shaping

Superoscillation is a technique that is used to produce a spot of light (known as ‘hotspot’) which is smaller than the conventional diffraction limit of a lens and even smaller than the optical wavelength. Over the past few years, several techniques have been realized for the generation of the superoscillatory hotspot. In this article, for the first time to the best of our knowledge, we propose a novel and a more efficient technique for producing superoscillation in microscopic imaging by shaping the Coherent Transfer Function (CTF) of a lens via virtual Fourier filtering followed by a phase retrieval algorithm. We design and realize a phase mask which when placed at the pupil plane of a diffraction-limited lens produces a superoscillatory hotspot with sidelobes properly matched to the field of view (FOV) required in microscopic imaging applications, i.e. hotspot always coexists with huge intense rings known as ‘sidebands’ close to it and hence limiting the FOV. Our technique is also capable of extending the FOV with minimal loss in resolution of the hotspot generated and considerable ratio between the intensity of the hotspot to that of the side lobes while optimizing the obtainable FOV to the requirement of microscopy.

Light-induced magnetism in plasmonic gold nanoparticles

Strategies for ultrafast optical control of magnetism have been a topic of intense research for several decades because of the potential impact in technologies such as magnetic memory, spintronics, and quantum computation, as well as the opportunities for non-linear optical control and modulation in applications such as optical isolation and non-reciprocity. Here we report the first experimental quantification of optically induced magnetization in plasmonic Au nanoparticles due to the inverse Faraday effect (IFE). The induced magnetic moment in nanoparticles is found to be ~1,000x larger than that observed in bulk Au, and ~20x larger than the magnetic moment from optimized magnetic nanoparticle colloids such as magnetite. Furthermore, the magnetization and demagnetization kinetics are instantaneous within the sub-picosecond time resolution of our study, supporting a mechanism of coherent transfer of angular momentum from the circularly polarized excitation to the orbital angular momentum of the electron gas.

Cascaded optical frequency transfer over 500-km fiber link using regenerative amplifier**Project supported by the National Key Research and Development Program of China (Grant No. 2016YFF0200200), the National Natural Science Foundation of China (Grant Nos. 91636101, 91836301, and 11803041), the West Light Foundation of the Chinese Academy of Sciences (Grant No. XAB2016B47), and the Strategic Priority Research Program of the Chinese

We demonstrate a 300-km+200-km cascaded coherent phase transfer via fiber link. The transfer is divided into a 300-km span and a 200-km span with independent phase locking loops, aiming to extend the phase control bandwidth of the whole link. The phase noise and transfer instability of the cascaded transmission are investigated and compared with those in the case of a single-span 500-km transfer. We achieve the transfer instabilities of 1.8 × 10−14 at 1 s, 8.9 × 10−20 at 104 s for the 300-km + 200-km cascaded transmission, and 2.7 × 10−14 at 1 s for the 500-km single-span transfer.

Linear and nonlinear coherence transfer of resonant nuclear-spin-dressed effect via metastability-exchange collisions

We present a systematic analysis to explain the observed magnetic resonance spectrum with three or five peaks spaced at Rabi frequency when the metastable 3He atoms are probed with a transverse circularly or linearly polarized 1083 nm laser beam, respectively. The resonance signals are generated in the ground state of 3He atoms, dressed by a resonant magnetic field, and transferred to the metastable state by collisions. The triplet spectrum is thought to be the result of the linear coupling between the metastable state and the ground state, while the quintuplet is thought to be that of the nonlinear coupling, and indicates that higher-order atomic polarization is created during the atomic collisions. More features of the magnetic resonance signals are investigated.

Another transfer channel for shock energy flowing into intra-molecular: the coherent transfer channel

In this paper, we have proposed that there is another transfer channel for shock energy flowing into to intra-molecular vibration mode. During this energy transfer process, these higher frequency vibrations would gradually possess a coherence at the direction of shock wave. Namely, these optical phonons could be coherent after shock wave compressed. Based on the probe light can be scattered by the coherent optical phonons, a series of light scattering experiments at varying detection angles were performed to explore the existing evidence of coherent optical phonon in shocked materials. No matter the incident angle is 6.2° or 15.7°, the Signal intensity ratio γs and the line width Γ of compressed vibration were both showed peak value around the corresponding phase matching angle which was attributed to the contribution of coherent optical phonons. Taken together, these experimental results demonstrated the existence of new proposed shock energy transfer channel, that coherent transfer channel, and open new perspectives in the molecular dissociation channel research in shocked materials.

Two-dimensional 19F-13C correlation NMR for 19F resonance assignment of fluorinated proteins.

19F solid-state NMR is an excellent approach for measuring long-range distances for structure determination and for studying molecular motion. For multi-fluorinated proteins, assignment of 19F chemical shifts has been traditionally carried out using mutagenesis. Here we show 2D 19F-13C correlation experiments that allow efficient assignment of the 19F chemical shifts. We have compared several rotational-echo double-resonance-based pulse sequences and 19F-13C cross polarization (CP) for 2D 19F-13C correlation. We found that direct transferred-echo double-resonance (TEDOR) transfer from 19F to 13C and vice versa outperforms out-and-back coherence transfer schemes. 19F detection gives twofold higher sensitivity over 13C detection for the 2D correlation experiment. At MAS frequencies of 25-35kHz, double-quantum 19F-13C CP has higher coherence transfer efficiencies than zero-quantum CP. The most efficient TEDOR transfer experiment has higher sensitivity than the most efficient double-quantum CP experiment. We demonstrate these 2D 19F-13C correlation experiments on the model compounds t-Boc-4F-phenylalanine and GB1. Application of the 2D 19F-13C TEDOR correlation experiment to the tetrameric influenza BM2 transmembrane peptide shows intermolecular 13C-19F cross peaks that indicate that the BM2 tetramers cluster in the lipid bilayer in an antiparallel fashion. This clustering may be relevant for the virus budding function of this protein.

Coherent long-range transfer of angular momentum between magnon Kittel modes by phonons

We report ferromagnetic resonance in the normal configuration of an electrically insulating magnetic bilayer consisting of two yttrium iron garnet (YIG) films epitaxially grown on both sides of a 0.5-mm-thick nonmagnetic gadolinium gallium garnet (GGG) slab. An interference pattern is observed and it is explained as the strong coupling of the magnetization dynamics of the two YIG layers either in phase or out of phase by the standing transverse sound waves, which are excited through a magnetoelastic interaction. This coherent mediation of angular momentum by circularly polarized phonons through a nonmagnetic material over macroscopic distances can be useful for future information technologies.

Thermalization and Sub-Poissonian Density Fluctuations in a Degenerate Molecular Fermi Gas.

We observe thermalization in the production of a degenerate Fermi gas of polar ^{40}K^{87}Rb molecules. By measuring the atom-dimer elastic scattering cross section near the Feshbach resonance, we show that Feshbach molecules rapidly reach thermal equilibrium with both parent atomic species. Equilibrium is essentially maintained through coherent transfer to the ground state. Sub-Poissonian density fluctuations in Feshbach and ground-state molecules are measured, giving an independent characterization of degeneracy and directly probing the molecular Fermi-Dirac distribution.

Lasing‐Encoded Microsensor Driven by Interfacial Cavity Resonance Energy Transfer

AbstractMicrolasers are emerging tools for biomedical applications. In particular, whispering‐gallery‐mode (WGM) microlasers are promising candidates for sensing at the biointerface owing to their high quality‐factor and potential in molecular assays, and intracellular and extracellular detection. However, lasing particles with sensing functionality remain challenging since the overlap between the WGM optical mode and external gain medium is much lower compared to internal gain inside the cavity. To overcome this problem, the concept of Förster resonant energy transfer (FRET) is exploited on WGM droplet microlaser by separating donor and acceptor molecules at the cavity–surface interface. It is first discovered that the interfacial FRET laser not only originates from conventional FRET but utilizes coherent radiative energy transfer (CRET) to excite acceptor molecules by inducing light‐harvesting effect near the cavity interface. Simulations and experiments have revealed that the absorption spectrum of individual analyte plays a crucial role in interfacial FRET laser. Distinct lasing spectra can therefore distinguish molecules of different absorption properties upon binding. Finally, detection of small fluorescent molecules and photosynthetic protein is performed. The results presented here not only demonstrate the wide‐ranging potential of microlaser external cavity implementation in molecular sensing applications, but also provide comprehensive insights into cavity energy transfer in laser physics.

Ultrafast optically induced spin transfer in ferromagnetic alloys.

The vision of using light to manipulate electronic and spin excitations in materials on their fundamental time and length scales requires new approaches in experiment and theory to observe and understand these excitations. The ultimate speed limit for all-optical manipulation requires control schemes for which the electronic or magnetic subsystems of the materials are coherently manipulated on the time scale of the laser excitation pulse. In our work, we provide experimental evidence of such a direct, ultrafast, and coherent spin transfer between two magnetic subsystems of an alloy of Fe and Ni. Our experimental findings are fully supported by time-dependent density functional theory simulations and, hence, suggest the possibility of coherently controlling spin dynamics on subfemtosecond time scales, i.e., the birth of the research area of attomagnetism.