Coherent Pump Research Articles

Experimental observation of nonreciprocal magnonic frequency combs

We demonstrate the nonreciprocal transmission of magnonic frequency combs (MFCs) in a dissipative cavity-magnonic system. We utilize the recently emerged pump-induced magnon (PIM) mode in YIG spheres to generate an MFC, as the PIM mode exhibits excellent nonlinearity under coherent pumping. Meanwhile, the dissipative cavity magnonic device is prepared to critical bound states in the continuum (BIC), providing clear nonreciprocity. Based on the different absorption efficiencies of the device in two opposite directions, we have demonstrated a clear difference in the number of frequency comb teeth for forward and reverse transmission, showcasing the ability to generate unidirectional combs. The nonreciprocal MFCs can be systematically tuned by modulating the detuning of the pump and BIC, the magnon and cavity modes, as well as the pump and perturbation tone. This research promotes the combination of MFCs and functional non-Hermitian cavity-magnon electronic devices, realizing new applications for nonreciprocal magnonic devices.

Frequency conversion in a hydrogen-filled hollow-core fiber using continuous-wave fields.

In large-area quantum networks based on optical fibers, photons are the fundamental carriers of information as so-called flying qubits. They may also serve as the interconnect between different components of a hybrid architecture, which might comprise atomic and solid-state platforms operating at visible or near-infrared wavelengths, as well as optical links in the telecom band. Quantum frequency conversion is the pathway to change the color of a single photon while preserving its quantum state. Currently, nonlinear crystals are utilized for this process. However, their performance is limited by their acceptance bandwidth, tunability, polarization sensitivity, and undesired background emission. A promising alternative is based on stimulated Raman scattering (SRS) in gases. Here, we demonstrate polarization-preserving frequency conversion in a hydrogen-filled antiresonant hollow-core fiber. This approach holds promises for seamless integration into optical fiber networks and interfaces to single emitters. Disparate from related experiments that employ a pulsed pump field, we here take advantage of two coherent continuous-wave pump fields.

Role of the inverse Čerenkov effect in the formation of ultrashort Raman solitons in silica microspheres.

We theoretically demonstrate a new regime, to the best of our knowledge, of the formation of ultrashort optical solitons in spherical silica microresonators with whispering gallery modes. The solitons are driven by a coherent CW pump at the frequency in the range of normal dispersion, and the energy is transferred from this pump to the solitons via two channels: the Raman amplification and inverse Čerenkov effect. We discuss three different regimes of soliton propagation and we also show that these Raman solitons can be controlled by weak coherent CW signals.

Thermal and Coherent Spin Pumping by Noncollinear Antiferromagnets.

Antiferromagnets attract much interest because of their potential for spintronic applications and open fundamental physics questions, but especially noncollinear antiferromagnets remain relatively unexplored. Here, we formulate the thermal and coherent pumping of spins in noncollinear antiferromagnets|normal metal bilayers. We find that the spin current polarization is a vector with components along both the Néel vector and net magnetic moment. The spin mixing conductance for the coherent spin pumping is a tensor with elements depending on the degree of noncollinearity and interface spin configuration. We explain the controversial sign problem of the antiferromagnetic spin Seebeck effect by interface effects and suggest that interface engineering may enhance the spin pumping efficiency.

Ultra-high spin emission from antiferromagnetic FeRh

An antiferromagnet emits spin currents when time-reversal symmetry is broken. This is typically achieved by applying an external magnetic field below and above the spin-flop transition or by optical pumping. In this work we apply optical pump-THz emission spectroscopy to study picosecond spin pumping from metallic FeRh as a function of temperature. Intriguingly we find that in the low-temperature antiferromagnetic phase the laser pulse induces a large and coherent spin pumping, while not crossing into the ferromagnetic phase. With temperature and magnetic field dependent measurements combined with atomistic spin dynamics simulations we show that the antiferromagnetic spin-lattice is destabilised by the combined action of optical pumping and picosecond spin-biasing by the conduction electron population, which results in spin accumulation. We propose that the amplitude of the effect is inherent to the nature of FeRh, particularly the Rh atoms and their high spin susceptibility. We believe that the principles shown here could be used to produce more effective spin current emitters. Our results also corroborate the work of others showing that the magnetic phase transition begins on a very fast picosecond timescale, but this timescale is often hidden by measurements which are confounded by the slower domain dynamics.

Feasibility of a localized mode analysis method in an SOI platform based on carrier grating

In order to measure the intensity of modes that are transmitted inside the devices on the silicon-on-insulator (SOI) platform, researchers usually use pre-processed couplers to make the optical modes diffract out of the chip. However, the output couplers have an influence (e.g., attenuation and wavelength selectivity) on the modes of concern. Besides, as the quantity and variety of devices integrated into the SOI platform continue to escalate, the traditional method also shows limits on detecting devices far from the chip edge. So, is it feasible to directly and locally measure one specific mode’s intensity on some waveguide-based devices like the directional coupler, polarization beam splitter, and so on. Interference of two coherent pump beams has the capability to induce a periodic carrier distribution in the material, thus modulating the refractive index, effectively creating a temporary and erasable diffraction grating. In this study, an off-chip, non-destructive, and localized detection method based on carrier grating is proposed. A theoretical model is developed to calculate carrier dynamics under various pump configurations. Leveraging the finite-difference time-domain (FDTD) method and accounting for free carrier index (FCI) and free carrier absorption (FCA) effects, analysis of the quantitative impact of pump intensity and radius on the diffraction efficiency of the carrier grating in the silicon-on-insulator (SOI) platform and its far-field divergence characteristics is provided. Ultimately, this research contributes to a discussion on several commonly used application scenarios and the feasibility of experimental approaches. A spatial resolution of less than 10 µm and a diffraction efficiency of −15dB while simultaneously maintaining a far-field divergence of 7.8° for the SOI platform are proposed at the end of this article.

Bose-Einstein condensation of magnons under coherent pumping by light

Bose-Einstein condensation of magnons under coherent pumping by light

Deterministic Shaping of Quantum Light Statistics

We propose a theoretical method for the deterministic shaping of quantum light via photon number state selective interactions. Nonclassical states of light are an essential resource for high-precision optical techniques that rely on photon correlations and noise reshaping. Notable techniques include quantum enhanced interferometry, ghost imaging, and generating fault-tolerant codes for continuous variable optical quantum computing. We show that a class of nonlinear-optical resonators can transform many-photon wavefunctions to produce structured states of light with nonclassical noise statistics. The devices, based on parametric down conversion, utilize the Kerr effect to tune photon-number-dependent frequency matching, inducing photon-number-selective interactions. With a high-amplitude coherent pump, the number-selective interaction shapes the noise of a two-mode squeezed cavity state with minimal dephasing, illustrated with simulations. We specify the requisite material properties to build the device and highlight the remaining material degrees of freedom which offer flexible material design.

Reconfigurable spin current transmission and magnon–magnon coupling in hybrid ferrimagnetic insulators

Coherent spin waves possess immense potential in wave-based information computation, storage, and transmission with high fidelity and ultra-low energy consumption. However, despite their seminal importance for magnonic devices, there is a paucity of both structural prototypes and theoretical frameworks that regulate the spin current transmission and magnon hybridization mediated by coherent spin waves. Here, we demonstrate reconfigurable coherent spin current transmission, as well as magnon–magnon coupling, in a hybrid ferrimagnetic heterostructure comprising epitaxial Gd3Fe5O12 and Y3Fe5O12 insulators. By adjusting the compensated moment in Gd3Fe5O12, magnon–magnon coupling was achieved and engineered with pronounced anticrossings between two Kittel modes, accompanied by divergent dissipative coupling approaching the magnetic compensation temperature of Gd3Fe5O12 (TM,GdIG), which were modeled by coherent spin pumping. Remarkably, we further identified, both experimentally and theoretically, a drastic variation in the coherent spin wave-mediated spin current across TM,GdIG, which manifested as a strong dependence on the relative alignment of magnetic moments. Our findings provide significant fundamental insight into the reconfiguration of coherent spin waves and offer a new route towards constructing artificial magnonic architectures.

Linear and phase controllable terahertz frequency conversion via ultrafast breaking the bond of a meta-molecule

The metasurface platform with time-varying characteristics has emerged as a promising avenue for exploring exotic physics associated with Floquet materials and for designing photonic devices like linear frequency converters. However, the limited availability of materials with ultrafast responses hinders their applications in the terahertz range. Here we present a time-varying metasurface comprising an array of superconductor-metal hybrid meta-molecules. Each meta-molecule consists of two meta-atoms that are “bonded” together by double superconducting microbridges. Through experimental investigations, we demonstrate high-efficiency linear terahertz frequency conversion by rapidly breaking the bond using a coherent ultrashort terahertz pump pulse. The frequency and relative phase of the converted wave exhibit strong dependence on the pump-probe delay, indicating phase controllable wave conversion. The dynamics of the meta-molecules during the frequency conversion process are comprehensively understood using a time-varying coupled mode model. This research not only opens up new possibilities for developing innovative terahertz sources but also provides opportunities for exploring topological dynamics and Floquet physics within metasurfaces.

Coherent and incoherent pumping of a three-level laser

This article investigates the quantum and semi-classical aspects of a three-level atom-cavity system within the context of cavity quantum electrodynamics. The study examines the behavior of the system through a quantum perspective and a semi-classical approximation. The steady-state master equation is solved in the atom-cavity basis, resulting in a closed set of equations describing the atom’s level occupancies and the cavity’s photon number. The accuracy of the semi-classical approximation is assessed by comparing it with quantum simulations. The research analyzes the system’s behavior near the laser threshold, highlighting the interplay between semi-classical and quantum behaviors. Additionally, the conversion of the three-level atom to a two-level atom is explored under specific conditions, enabling an investigation into the weak driving limit. Quantum simulation results are used to validate the proposed approximations. This work contributes to the understanding of atom-cavity interactions and provides insights into the transition from semi-classical to quantum behavior in such systems.

Phonon Mediated Collective Dynamics of Coherently Pumped Two-Level Emitters

"We investigate the collective quantum dynamics of an ensemble of two-level emitters, embedded in a crystal, and coherently pumped by a moderately intense, and externally applied coherent electromagnetic field. The ensemble is damped preponderantly via the surrounding phonon reservoir which mediates the inter-particle collective interactions. We have found that generally phonon transitions among the corresponding dressed states are taking place involving simultaneously many single emitters or pairs of two-level emitters, respectively. In both cases the phonon intensity can be proportional to the squared number of involved two-level emitters."

Incoherently pumped event horizons in optical fibers

Optical event horizons in fibers, driven by coherent pumps, have been a prominent subject of study within the field of nonlinear optics. Previously, optical event horizons involving a potent pump and a linear-wave were interpreted as phase-matching processes wherein new spectral components are derived from the linear-wave due to the influence of the strong pump. This nonlinear interaction, coupled with the wave mixing mechanism, has been elaborated upon in the spectral domain. It’s portrayed as a cascaded four-wave mixing process, achieving quasi-phase-matching through intermediate spectral components. Until now, research focused on event horizons or soliton linear-wave interactions has predominantly relied on coherent laser pump sources. However, there has been a recent resurgence in the exploration of incoherently pumped nonlinear optics. While the specific dynamics of incoherent light fields and their subsequent nonlinear processes might be elusive due to their inherent random field fluctuations, their incoherent nature unveils a multitude of statistical dynamics for nonlinear phenomena. In this work, we delve into optical event horizons encountered by linear-waves propelled by an incoherent light field within nonlinear optical fibers. Our numerical analysis scrutinizes the dynamics of linear-waves during optical event horizons under incoherent pumping. We further dissect the temporal statistics of the newly birthed idler-waves emerging from these event horizon processes.

Forward pumped distributed Raman amplification in C and L bands using incoherent first-order and coherent second-order pumps

Forward pumped distributed Raman amplification in C and L bands using incoherent first-order and coherent second-order pumps

A superradiant two-level laser with intrinsic light force generated gain

The implementation of a superradiant laser as an active frequency standard is predicted to provide better short-term stability and robustness to thermal and mechanical fluctuations when compared to standard passive optical clocks. However, despite significant recent progress, the experimental realization of continuous wave superradiant lasing still remains an open challenge as it requires continuous loading, cooling, and pumping of active atoms within an optical resonator. Here we propose a new scenario for creating continuous gain by using optical forces acting on the states of a two-level atom via bichromatic coherent pumping of a cold atomic gas trapped inside a single-mode cavity. Analogous to atomic maser setups, tailored state-dependent forces are used to gather and concentrate excited-state atoms in regions of strong atom-cavity coupling while ground-state atoms are repelled. To facilitate numerical simulations of a sufficiently large atomic ensemble, we rely on a second-order cumulant expansion and describe the atomic motion in a semi-classical point-particle approximation subject to position-dependent light shifts which induce optical gradient forces along the cavity axis. We study minimal conditions on pump laser intensities and detunings required for collective superradiant emission. Balancing Doppler cooling and gain-induced heating we identify a parameter regime of a continuous narrow-band laser operation close to the bare atomic frequency.

Dynamic Interplay Between Kerr Combs and Brillouin Lasing in Fiber Cavities

AbstractHighly coherent frequency combs are of crucial importance for optical synthesis and metrology, spectroscopy, laser ranging, and optical communications. Kerr combs, generated via cascaded nonlinear frequency conversion in a passive optical cavity, typically offer high repetition rates, which is essential for some of these applications. Recently, new ways of generating Kerr combs combining Kerr and Brillouin effects have emerged with the aim of improving some performances, especially in the fiber cavity platform. Direct coherent pumping is replaced by lasing on specific cavity modes, offering easily adjustable repetition rates, and enhanced coherence by Brillouin purification. In this study, such a scheme is implemented and investigated in a non‐reciprocal cavity. Highly coherent combs are demonstrated by finely controlling bi‐chromatic Brillouin lasing and the Kerr comb parameters. A suitable numerical model is introduced to account for the interplay between Brillouin scattering, Kerr effect, and cavity resonant feedback. Quantitative agreements with experiments reveal the importance of the pump lasers detuning in setting the comb's properties, through the mode pulling effect. This phenomenon, along with multi‐mode lasing that impedes the coherence, is not studied in previous fiber‐based demonstrations. These limitations are discussed, and several scaling laws are devised.

Ab-initio simulations of coherent phonon-induced pumping of carriers in zirconium pentatelluride

Laser-driven coherent phonons can act as modulated strain fields and modify the adiabatic ground state topology of quantum materials. Here we use time-dependent first-principles and effective model calculations to simulate the effect of the coherent phonon induced by strong terahertz electric field on electronic carriers in the topological insulator ZrTe5. We show that a coherent A1g Raman mode modulation can effectively pump carriers across the band gap, even though the phonon energy is about an order of magnitude smaller than the equilibrium band gap. We reveal the microscopic mechanism of this effect which occurs via Landau–Zener-Stückelberg tunneling of Bloch electrons in a narrow region in the Brillouin zone center where the transient energy gap closes when the system switches from strong to weak topological insulator. The quantum dynamics simulation results are in excellent agreement with recent pump-probe experiments in ZrTe5 at low temperature.

Natural exceptional points in the excitation spectrum of a light–matter system

In this work, we observe natural exceptional points in the excitation spectrum of an exciton–polariton system by optically tuning the light–matter interactions. The observed exceptional points do not require any spatial or polarization degrees of freedom and result solely from the transition from weak to strong light–matter coupling. It was demonstrated that they do not coincide with the threshold for photon lasing, confirming previous theoretical predictions [Phys. Rev. Lett. 122, 185301 (2019)PRLTAO0031-900710.1103/PhysRevLett.122.185301, Optica 7, 1015 (2020)OPTIC82334-253610.1364/OPTICA.397378]. Using a technique where a strong coherent laser pump induces up-converted excitations, we encircle the exceptional point in the parameter space of coupling strength and particle momentum. Our method of local optical control of light–matter coupling paves the way to the investigation of fundamental phenomena, including dissipative phase transitions and non-Hermitian topological states.

Phonon Laser in the Quantum Regime.

We demonstrate a trapped-ion system with two competing dissipation channels, implemented independently on two ion species cotrapped in a Paul trap. By controlling coherent spin-oscillator couplings and optical pumping rates we explore the phase diagram of this system, which exhibits a regime analogous to that of a (phonon) laser but operates close to the quantum ground state with an average phonon number of n[over ¯]<10. We demonstrate phase locking of the oscillator to an additional resonant drive, and also observe the phase diffusion of the resulting state under dissipation by reconstructing the quantum state from a measurement of the characteristic function.

Towards a photonic integrated all-optical phase regenerator.

All-optical phase regeneration aims at restoring the phase information of coherently encoded data signals directly in the optical domain so as to compensate for phase distortions caused by transceiver imperfections and nonlinear impairments along the transmission link. Although it was proposed two decades ago, all-optical phase regeneration has not been seen in realistic networks to date, mainly because this technique entails complex bulk modules and relies on high-precision phase sensitive nonlinear dynamics, both of which are adverse to field deployment. Here, we demonstrate a new, to the best of our knowledge, architecture to implement all-optical phase regeneration using integrated photonic devices. In particular, we realize quadrature phase quantization by exploring the phase-sensitive parametric wave mixing within on-chip silicon waveguides, while multiple coherent pump laser tones are provided by a chip-scale micro-cavity Kerr frequency comb. Multi-channel all-optical phase regeneration is experimentally demonstrated for 40 Gbps QPSK data, achieving the best SNR improvement of more than 6 dB. Our study showcases a promising avenue to enable the practical implementation of all-optical phase regeneration in realistic long-distance fiber transmission networks.