Cloud Lifetime Research Articles

Momentum feedback from marginally resolved H ii regions in isolated disc galaxies

ABSTRACT We present a novel, physically motivated sub-grid model for H ii region feedback within the moving mesh code arepo, accounting for both the radiation pressure-driven and thermal expansion of the ionized gas surrounding young stellar clusters. We apply this framework to isolated disc galaxy simulations with mass resolutions between 103 and 105 M⊙ per gas cell. Each simulation accounts for the self-gravity of the gas, the momentum and thermal energy from supernovae, the injection of mass by stellar winds, and the non-equilibrium chemistry of hydrogen, carbon, and oxygen. We reduce the resolution dependence of our model by grouping those H ii regions with overlapping ionization front radii. The Strömgren radii of the grouped H ii regions are at best marginally resolved, so that the injection of purely thermal energy within these radii has no effect on the interstellar medium. By contrast, the injection of momentum increases the fraction of cold and molecular gas by more than 50 per cent at mass resolutions of 103 M⊙, and decreases its turbulent velocity dispersion by ∼10 km s−1. The mass-loading of galactic outflows is decreased by an order of magnitude. The characteristic lifetime of the least-massive molecular clouds ($M/{\rm M}_\odot \lesssim 5.6 \times 10^4$) is reduced from ∼18 to $\lesssim 10$ Myr, indicating that H ii region feedback is effective in destroying these clouds. Conversely, the lifetimes of intermediate-mass clouds ($5.6 \times 10^4 \lesssim M/{\rm M}_\odot \lesssim 5 \times 10^5$) are elongated by ∼7 Myr, likely due to a reduction in supernova clustering. The derived cloud lifetimes span the range from 10 to 40 Myr, in agreement with observations. All results are independent of whether the momentum is injected from a ‘spherical’ or a ‘blister-type’ H ii region.

A scaling relation for the molecular cloud lifetime in Milky Way-like galaxies.

We study the time evolution of molecular clouds across three Milky Way-like isolated disc galaxy simulations at a temporal resolution of 1Myr and at a range of spatial resolutions spanning two orders of magnitude in spatial scale from ∼10pc up to ∼1kpc. The cloud evolution networks generated at the highest spatial resolution contain a cumulative total of ∼80 000 separate molecular clouds in different galactic-dynamical environments. We find that clouds undergo mergers at a rate proportional to the crossing time between their centroids, but that their physical properties are largely insensitive to these interactions. Below the gas-disc scale height, the cloud lifetime τlife obeys a scaling relation of the form τlife∝ℓ-0.3 with the cloud size ℓ, consistent with over-densities that collapse, form stars, and are dispersed by stellar feedback. Above the disc scale height, these self-gravitating regions are no longer resolved, so the scaling relation flattens to a constant value of ∼13Myr, consistent with the turbulent crossing time of the gas disc, as observed in nearby disc galaxies.

Observational Quantification of Aerosol Invigoration for Deep Convective Cloud Lifecycle Properties Based on Geostationary Satellite

AbstractAerosols affect cloud microstructure, dynamics, and precipitation by acting as cloud condensation nuclei (CCN) and ice nuclei with a large uncertainty for deep convective clouds (DCCs). Here, we quantify the relationships between aerosols and DCC properties after isolating aerosol impacts from meteorology based on the METEOSAT geostationary satellite and Modern‐Era Retrospective Analysis for Research and Application Version 2 (MERRA‐2) reanalysis data. Results show that fine aerosols (radius <1 µm), which serve as the best proxy for CCN from MERRA‐2, exhibit the strongest aerosol invigoration for DCC compared with aerosol optical depth and coarse aerosols. Overall, added fine aerosols result in colder cloud top temperatures (CTTs), longer lifetime, and more rainfall amounts, especially over land. As CTT decreases monotonically with added aerosols, cloud lifetime and rainfall amount reach a maximum at aerosol loading of 5 and 1.5 µg/m3 over land and ocean, respectively. Added precipitable water (PW) vapor and convective available potential energy (CAPE) are conducive to the development of more vigorous DCC. For fixed PW and CAPE, CTT decreases by up to −12.2°C ± 0.5°C with fine aerosol concentration over land and up to −4.4°C ± 1.0°C over ocean. The DCC lifetime is lengthened by a factor of 1.3 ± 0.1 from clean condition to optimal aerosol loading over land. A respective enhancement in rainfall amounts over land is indicated by a factor of 2.6 ± 0.4. The decreases in lifetime and rainfall beyond the optimal aerosol concentration are likely due to less aerosol wet scavenging from smaller and less rainy DCCs. The increases in the lifetime and rainfall amounts over ocean are much weaker.

Simulation study on the indirect effect of sulfate on the summer climate over the eastern China monsoon region

In this study, we designed a sensitivity test using the half number concentration of sulfate in the nucleation calculation process to study the aerosol-cloud interaction (ACI) of sulfate on clouds, precipitation, and monsoon intensity in the summer over the eastern China monsoon region (ECMR) with the National Center for Atmospheric Research Community Atmosphere Model version 5. Numerical experiments show that the ACI of sulfate led to an approximately 30% and 34% increase in the cloud condensation nuclei and cloud droplet number concentrations, respectively. Cloud droplet effective radius below 850 hPa decreased by approximately 4% in the southern ECMR, while the total liquid water path increased by 11%. The change in the indirect radiative forcing due to sulfate at the top of the atmosphere in the ECMR during summer was − 3.74 W·m−2. The decreased radiative forcing caused a surface cooling of 0.32 K and atmospheric cooling of approximately 0.3 K, as well as a 0.17 hPa increase in sea level pressure. These changes decreased the thermal difference between the land and sea and the gradient of the sea-land pressure, leading to a weakening in the East Asian summer monsoon (EASM) and a decrease in the total precipitation rate in the southern ECMR. The cloud lifetime effect has a relatively weaker contribution to summer precipitation, which is dominated by convection. The results show that the ACI of sulfate was one possible reason for the weakening of the EASM in the late 1970s.

On the duration of the embedded phase of star formation

ABSTRACT Feedback from massive stars plays a key role in molecular cloud evolution. After the onset of star formation, the young stellar population is exposed by photoionization, winds, supernovae, and radiation pressure from massive stars. Recent observations of nearby galaxies have provided the evolutionary timeline between molecular clouds and exposed young stars, but the duration of the embedded phase of massive star formation is still ill-constrained. We measure how long massive stellar populations remain embedded within their natal cloud, by applying a statistical method to six nearby galaxies at $20{-}100~\mbox{${\rm ~pc}$}$ resolution, using CO, Spitzer 24$\rm \, \mu m$, and H α emission as tracers of molecular clouds, embedded star formation, and exposed star formation, respectively. We find that the embedded phase (with CO and 24$\rm \, \mu m$ emission) lasts for 2−7 Myr and constitutes $17{-}47{{\ \rm per\ cent}}$ of the cloud lifetime. During approximately the first half of this phase, the region is invisible in H α, making it heavily obscured. For the second half of this phase, the region also emits in H α and is partially exposed. Once the cloud has been dispersed by feedback, 24$\rm \, \mu m$ emission no longer traces ongoing star formation, but remains detectable for another 2−9 Myr through the emission from ambient CO-dark gas, tracing star formation that recently ended. The short duration of massive star formation suggests that pre-supernova feedback (photoionization and winds) is important in disrupting molecular clouds. The measured time-scales do not show significant correlations with environmental properties (e.g. metallicity). Future JWST observations will enable these measurements routinely across the nearby galaxy population.

A Lagrangian Perspective on Tropical Anvil Cloud Lifecycle in Present and Future Climate

AbstractThe evolution of tropical anvil clouds from their origin in deep convective cores to their slow decay determines the climatic effects of clouds in tropical convective regions. Despite the relevance of anvil clouds for climate and responses of clouds to global warming, processes dominating their evolution are not well understood. Currently available observational data reveal instantaneous snapshots of anvil cloud properties, but cannot provide a process‐based perspective on anvil evolution. We therefore conduct simulations with the high resolution version of the exascale earth system model in which we track mesoscale convective systems over the tropical Western Pacific and compute trajectories that follow air parcels detrained from peaks of convective activity. With this approach we gain new insight into the anvil cloud evolution both in present day and future climate.Comparison with geostationary satellite data shows that the model is able to simulate maritime mesoscale convective systems reasonably well. Trajectory results indicate that anvil cloud lifetime is about 15 h with no significant change in a warmer climate. The anvil ice mixing ratio is larger in a warmer climate due to a larger source of ice by detrainment and larger depositional growth leading to a more negative net cloud radiative effect along detrained trajectories. However, the increases in sources are counteracted by increases in sinks of ice, particularly snow formation and sedimentation. Furthermore, we find that the mean anvil cloud feedback along trajectories is positive and consistent with results from more traditional cloud feedback calculation methods.

Exploiting Photoionization Reflectron Time-of-Flight Mass Spectrometry to Explore Molecular Mass Growth Processes to Complex Organic Molecules in Interstellar and Solar System Ice Analogs.

ConspectusThis Account presents recent advances in our understanding on the formation pathways of complex organic molecules (COMs) within interstellar analog ices on ice-coated interstellar nanoparticles upon interaction with ionizing radiation exploiting reflectron time-of-flight mass spectrometry (ReTOF-MS) coupled with tunable vacuum ultraviolet (VUV) single photon ionization (PI) and resonance enhanced multiphoton ionization (REMPI) of the subliming molecules during the temperature-programmed desorption (TPD) phase. Laboratory simulation experiments provided compelling evidence that key classes of complex organics (aromatic hydrocarbons, alcohols, ethers, aldehydes, enols, ketones, and carboxylic acids) can be synthesized upon exposure of astrophysically relevant model ices to ionizing radiation within and throughout the ices at temperatures as low as 5 K.Molecular mass growth processes can be initiated by suprathermal or electronically excited reactants along with barrierless radical-radical recombination if both radicals hold a proper recombination geometry. Methyl (CH3), amino (NH2), hydroxyl (OH), ethyl (C2H5), vinyl (C2H3), ethynyl (C2H), formyl (HCO), hydroxycarbonyl (HOCO), hydroxymethyl (CH2OH), methoxy (CH3O), and acetyl (CH3CO) represent readily available reactants for radical-radical recombination within the ices. Reactive singlet species were found to insert without barrier into carbon-hydrogen and carbon-carbon single bonds (carbene) leading to an extension of the carbon chain and may add to carbon-carbon double bonds (carbene, atomic oxygen) forming cyclic reaction products. These galactic cosmic ray-triggered nonequilibrium pathways overcome previous obstacles of hypothesized thermal grain-surface processes and operate throughout the ice at 5 K. Our investigations discriminate between multiple structural isomers such as alcohols/ethers, aldehydes/enols, and cyclic/acyclic carbonyls. These data provide quantitative, isomer selective input parameters for a cosmic ray-dictated formation of complex organics in interstellar ices and are fully able to replicate the astronomical observations of complex organics over typical lifetimes of molecular clouds of a few 106 to 107 years. Overall, PI-ReTOF-MS revealed that the processing of astrophysically relevant ices can lead to multifaceted mixtures of organics reaching molecular weights of up to 200 amu. Further advances in laboratory techniques beyond the FTIR-QMS limit are clearly desired not only to confidently assign detection in laboratory ice analog experiments of increasingly more complex molecules of interest but also from the viewpoint of future astronomical searches in the age of the Atacama Large Millimeter/submillimeter Array (ALMA).

Pressure Drag for Shallow Cumulus Clouds: From Thermals to the Cloud Ensemble

AbstractThis study takes the first step to bridge the gap between the pressure drag of a shallow cloud ensemble and that of an individual cloud composed of rising thermals. It is found that the pressure drag for a cloud ensemble is primarily controlled by the dynamical component. The dominance of dynamical pressure drag and its increased magnitude with height are independent of cloud lifetime and are common features of individual clouds except that the total drag of a single cloud over life cycle presents vertical oscillations. These oscillations are associated with successive rising thermals but are further complicated by the evaporation‐driven downdrafts outside the cloud. The horizontal vorticity associated with the vortical structure is amplified as the thermals rise to higher altitudes due to continuous baroclinic vorticity generation. This leads to the increased magnitude of local minima of dynamical pressure perturbation with height and consequently to increased dynamical pressure drag.

Enhancement of Network Lifetime of Cloud Assisted Internet of Things: New Contribution of Deer Hunting and Particle Swarm Optimization

In general, WSN maintains the chief support of cloud-assisted internet of things (CIoT). This paper intends to implement a WSN-assisted CIoT model which involves two processes: one is optimal cluster head selection, and the other is optimal shortest path selection. The main intent of this optimal cluster head selection is to select a cluster head using a hybrid optimisation algorithm with the objective of minimising the distance between each IoT sensor node and cluster head and consumed energy. Moreover, the same hybrid algorithm is used in the optimal shortest path selection process. The beneficial concepts of two well-performing meta-heuristic algorithms like deer hunting optimisation algorithm (DHOA), and particle swarm optimisation (PSO) are merged to frame a hybrid algorithm termed as particle swarm-based deer hunting optimisation algorithm (PS-DHOA) to be suited for both cluster head selection and route selection. Developed model has been validated through effective performance analysis.

Impact of biomass burning aerosols on radiation, clouds, and precipitation over the Amazon: relative importance of aerosol–cloud and aerosol–radiation interactions

Abstract. Biomass burning (BB) aerosols can influence regional and global climate through interactions with radiation, clouds, and precipitation. Here, we investigate the impact of BB aerosols on the energy balance and hydrological cycle over the Amazon Basin during the dry season. We performed simulations with a fully coupled meteorology–chemistry model, the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem), for a range of different BB emission scenarios to explore and characterize nonlinear effects and individual contributions from aerosol–radiation interactions (ARIs) and aerosol–cloud interactions (ACIs). The ARIs of BB aerosols tend to suppress low-level liquid clouds by local warming and increased evaporation and to facilitate the formation of high-level ice clouds by enhancing updrafts and condensation at high altitudes. In contrast, the ACIs of BB aerosol particles tend to enhance the formation and lifetime of low-level liquid clouds by providing more cloud condensation nuclei (CCN) and to suppress the formation of high-level ice clouds by reducing updrafts and condensable water vapor at high altitudes (>8 km). For scenarios representing the lower and upper limits of BB emission estimates for recent years (2002–2016), we obtained total regional BB aerosol radiative forcings of −0.2 and 1.5 W m−2, respectively, showing that the influence of BB aerosols on the regional energy balance can range from modest cooling to strong warming. We find that ACIs dominate at low BB emission rates and low aerosol optical depth (AOD), leading to an increased cloud liquid water path (LWP) and negative radiative forcing, whereas ARIs dominate at high BB emission rates and high AOD, leading to a reduction of LWP and positive radiative forcing. In all scenarios, BB aerosols led to a decrease in the frequency of occurrence and rate of precipitation, caused primarily by ACI effects at low aerosol loading and by ARI effects at high aerosol loading. The dependence of precipitation reduction on BB aerosol loading is greater in a strong convective regime than under weakly convective conditions. Overall, our results show that ACIs tend to saturate at high aerosol loading, whereas the strength of ARIs continues to increase and plays a more important role in highly polluted episodes and regions. This should hold not only for BB aerosols over the Amazon, but also for other light-absorbing aerosols such as fossil fuel combustion aerosols in industrialized and densely populated areas. The importance of ARIs at high aerosol loading highlights the need for accurately characterizing aerosol optical properties in the investigation of aerosol effects on clouds, precipitation, and climate.

Enhancing the Aggressive Intensity of a Cavitating Jet by Introducing Water Flow Holes and a Long Guide Pipe

Abstract It is known that the geometry of the nozzle has a great effect on the aggressive intensity of a cavitating jet. In previous reports, various nozzle geometries were proposed, and improvements made to the aggressive intensity were reported. However, no detailed description of the reasons why the aggressive intensity is improved by these various geometries was given. In this study, we conducted erosion tests on pure aluminum Japanese Industrial Standards JIS A1050P using 11 different nozzles with different geometries downstream from the throat outlet in order to understand the effects of the nozzle geometry on the aggressive intensity. In addition, in order to investigate the characteristics of the cavitating jet produced by each nozzle, measurements of the erosion areas, images of the cavitating jet using a high-speed video camera, and measurements of the impingement pressure of the cavitating jet were taken, and correlations between the parameters were obtained. It was found that the nozzle with the largest mass loss was a nozzle with water flow holes near to the throat outlet and a long guide pipe (LGP). The mass loss was 2.5 times that of the previously reported optimum geometry nozzle. Very high correlations were obtained between the mass loss, the inner diameter of the annular erosion area, the impingement pressure measured at the same standoff distance and the cavitation cloud lifetime. Based on these results and the images of the cavitating jets taken with the high-speed video camera, a new cavitating jet progression process is proposed.

Studying Scale Dependency of Aerosol Cloud Interactions using Multi-Scale Cloud Formulations.

The WRF-ACI model configuration is used to investigate the scale dependency of aerosol-cloud interactions (ACI) across the "grey zone" scales for grid and subgrid-scale clouds. The impacts of ACI on weather are examined across regions in the eastern and western U. S. at 36, 12, 4, and 1 km grid spacing for short-term periods during the summer of 2006. ACI impacts are determined by comparing simulations with current climatological aerosol levels to simulations with aerosol levels reduced by 90%. The aerosol-cloud lifetime effect is found to be the dominant process leading to suppressed precipitation in regions of the eastern U.S., while regions in the western U. S. experience offsetting impacts on precipitation from the cloud lifetime effect and other effects that enhance precipitation. Generally, the cloud lifetime effect weakens with decreasing grid spacing due to a decrease in relative importance of autoconversion compared to accretion. Subgrid-scale ACI are dominant at 36 km, while grid-scale ACI are dominant at 4 and 1 km. At 12 km grid spacing, grid-scale and subgrid-scale ACI processes are comparable in magnitude and spatial coverage, but random perturbations in grid-scale-ACI impacts make the overall grid-scale-ACI impact appear muted. This competing behavior of grid and subgrid-scale clouds complicate the understanding of ACI at 12 km within the current WRF modeling framework. The work implies including subgrid-scale-cloud microphysics and ice/mixed phase cloud ACI processes may be necessary in weather and climate models to study ACI effectively.

Dynamical environments of MU69 and similar objects

We explore properties of the long-term dynamics of particles (moonlets, fragments, debris etc.) around KBO 2014 MU69 (Arrokoth), as well as around similar contact-binary objects potentially present in the Kuiper belt. The chaotic diffusion of particles inside the Hill sphere of MU69 (or, generally, a similar object) is studied by means of construction of appropriate stability diagrams and by application of analytical approaches generally based on the Kepler map theory. The formation and evolution of the particle clouds, due to the chaotic diffusion inside the Hill sphere, are studied and the cloud lifetimes are estimated.

Exploring the Chemistry Induced by Energetic Processing of the H2-bearing, CO-rich Apolar Ice Layer

Abstract Interstellar ice mantles on the surfaces of dust grains are thought to have a bilayered structure, with a H2O-rich polar layer, covered by a CO-rich apolar layer that probably harbors H2 and other volatiles such as N2. In this work, we explore the chemistry induced by 2 keV electrons and Lyα photons in H2:CO:15N2 ice analogs of the CO-rich layer when exposed to similar fluences to those expected from the cosmic-ray-induced secondary electrons and UV photons during the typical lifetime of dense clouds. Six products were identified upon 2 keV electron irradiation: CO2, C2O (and other carbon chain oxides), CH4, H2CO, H2C2O, and H15NCO. The total product abundances corresponded to 5%−10% of the initial CO molecules exposed to electron irradiation. Lyα photon irradiation delivered one to two orders of magnitude lower yields with a similar product branching ratio, which may be due to the low UV-photon absorption cross section of the ice sample at this wavelength. Formation of additional N-bearing species, namely C2 15N2 and 15NH3, was only observed in the absence of H2 and CO molecules, respectively, suggesting that reactants derived from H2 and CO molecules preferentially react with each other instead of with 15N2 and its dissociation products. In summary, ice chemistry induced by energetic processing of the CO-rich apolar ice layer provides alternative formation pathways for several species detected in the interstellar medium, including some related to the complex organic molecule chemistry. Further quantification of these pathways will help astrochemical models constrain their relative contribution to the interstellar budget of, especially, the organic species H2CO and HNCO.

A biogenic secondary organic aerosol source of cirrus ice nucleating particles

Atmospheric ice nucleating particles (INPs) influence global climate by altering cloud formation, lifetime, and precipitation efficiency. The role of secondary organic aerosol (SOA) material as a source of INPs in the ambient atmosphere has not been well defined. Here, we demonstrate the potential for biogenic SOA to activate as depositional INPs in the upper troposphere by combining field measurements with laboratory experiments. Ambient INPs were measured in a remote mountaintop location at –46 °C and an ice supersaturation of 30% with concentrations ranging from 0.1 to 70 L–1. Concentrations of depositional INPs were positively correlated with the mass fractions and loadings of isoprene-derived secondary organic aerosols. Compositional analysis of ice residuals showed that ambient particles with isoprene-derived SOA material can act as depositional ice nuclei. Laboratory experiments further demonstrated the ability of isoprene-derived SOA to nucleate ice under a range of atmospheric conditions. We further show that ambient concentrations of isoprene-derived SOA can be competitive with other INP sources. This demonstrates that isoprene and potentially other biogenically-derived SOA materials could influence cirrus formation and properties.

The ice-nucleating activity of Arctic sea surface microlayer samples and marine algal cultures

Abstract. In recent years, sea spray as well as the biological material it contains has received increased attention as a source of ice-nucleating particles (INPs). Such INPs may play a role in remote marine regions, where other sources of INPs are scarce or absent. In the Arctic, these INPs can influence water–ice partitioning in low-level clouds and thereby the cloud lifetime, with consequences for the surface energy budget, sea ice formation and melt, and climate. Marine aerosol is of a diverse nature, so identifying sources of INPs is challenging. One fraction of marine bioaerosol (phytoplankton and their exudates) has been a particular focus of marine INP research. In our study we attempt to address three main questions. Firstly, we compare the ice-nucleating ability of two common phytoplankton species with Arctic seawater microlayer samples using the same instrumentation to see if these phytoplankton species produce ice-nucleating material with sufficient activity to account for the ice nucleation observed in Arctic microlayer samples. We present the first measurements of the ice-nucleating ability of two predominant phytoplankton species: Melosira arctica, a common Arctic diatom species, and Skeletonema marinoi, a ubiquitous diatom species across oceans worldwide. To determine the potential effect of nutrient conditions and characteristics of the algal culture, such as the amount of organic carbon associated with algal cells, on the ice nucleation activity, Skeletonema marinoi was grown under different nutrient regimes. From comparison of the ice nucleation data of the algal cultures to those obtained from a range of sea surface microlayer (SML) samples obtained during three different field expeditions to the Arctic (ACCACIA, NETCARE, and ASCOS), we found that they were not as ice active as the investigated microlayer samples, although these diatoms do produce ice-nucleating material. Secondly, to improve our understanding of local Arctic marine sources as atmospheric INPs we applied two aerosolization techniques to analyse the ice-nucleating ability of aerosolized microlayer and algal samples. The aerosols were generated either by direct nebulization of the undiluted bulk solutions or by the addition of the samples to a sea spray simulation chamber filled with artificial seawater. The latter method generates aerosol particles using a plunging jet to mimic the process of oceanic wave breaking. We observed that the aerosols produced using this approach can be ice active, indicating that the ice-nucleating material in seawater can indeed transfer to the aerosol phase. Thirdly, we attempted to measure ice nucleation activity across the entire temperature range relevant for mixed-phase clouds using a suite of ice nucleation measurement techniques – an expansion cloud chamber, a continuous-flow diffusion chamber, and a cold stage. In order to compare the measurements made using the different instruments, we have normalized the data in relation to the mass of salt present in the nascent sea spray aerosol. At temperatures above 248 K some of the SML samples were very effective at nucleating ice, but there was substantial variability between the different samples. In contrast, there was much less variability between samples below 248 K. We discuss our results in the context of aerosol–cloud interactions in the Arctic with a focus on furthering our understanding of which INP types may be important in the Arctic atmosphere.

Influence of Arctic Microlayers and Algal Cultures on Sea Spray Hygroscopicity and the Possible Implications for Mixed‐Phase Clouds

AbstractAs Arctic sea ice cover diminishes, sea spray aerosols (SSA) have a larger potential to be emitted into the Arctic atmosphere. Emitted SSA can contain organic material, but how it affects the ability of particles to act as cloud condensation nuclei (CCN) is still not well understood. Here we measure the CCN‐derived hygroscopicity of three different types of aerosol particles: (1) Sea salt aerosols made from artificial seawater, (2) aerosol generated from artificial seawater spiked with diatom species cultured in the laboratory, and (3) aerosols made from samples of sea surface microlayer (SML) collected during field campaigns in the North Atlantic and Arctic Ocean. Samples are aerosolized using a sea spray simulation tank (plunging jet) or an atomizer. We show that SSA containing diatom and microlayer exhibit similar CCN activity to inorganic sea salt with a κ value of ∼1.0. Large‐eddy simulation (LES) is then used to evaluate the general role of aerosol hygroscopicity in governing mixed‐phase low‐level cloud properties in the high Arctic. For accumulation mode aerosol, the simulated mixed‐phase cloud properties do not depend strongly on κ, unless the values are lower than 0.4. For Aitken mode aerosol, the hygroscopicity is more important; the particles can sustain the cloud if the hygroscopicity is equal to or higher than 0.4, but not otherwise. The experimental and model results combined suggest that the internal mixing of biogenic organic components in SSA does not have a substantial impact on the cloud droplet activation process and the cloud lifetime in Arctic mixed‐phase clouds.

Observational Evidence that Radiative Heating Modifies the Life Cycle of Tropical Anvil Clouds

AbstractA variety of satellite and ground-based observations are used to study how diurnal variations of cloud radiative heating affect the life cycle of anvil clouds over the tropical western Pacific Ocean. High clouds thicker than 2 km experience longwave heating at cloud base, longwave cooling at cloud top, and shortwave heating at cloud top. The shortwave and longwave effects have similar magnitudes during midday, but only the longwave effect is present at night, so high clouds experience a substantial diurnal cycle of radiative heating. Furthermore, anvil clouds are more persistent or laterally expansive during daytime. This cannot be explained by variations of convective intensity or geographic patterns of convection, suggesting that shortwave heating causes anvil clouds to persist longer or spread over a larger area. It is then investigated if shortwave heating modifies anvil development by altering turbulence in the cloud. According to one theory, radiative heating drives turbulent overturning within anvil clouds that can be sufficiently vigorous to cause ice nucleation in the updrafts, thereby extending the cloud lifetime. High-frequency air motion and ice-crystal number concentration are shown to be inversely related near cloud top, however. This suggests that turbulence depletes or disperses ice crystals at a faster rate than it nucleates them, so another mechanism must cause the diurnal variation of anvil clouds. It is hypothesized that radiative heating affects anvil development primarily by inducing a mesoscale circulation that offsets gravitational settling of cloud particles.

Compaction of Porous H2O Ice via Energetic Electrons

Abstract Here we have investigated the degree to which energetic electrons cause structural changes in microporous H2O ice using infrared and ultraviolet–visible spectroscopy as analytical tools. In these studies, we found that energetic electrons destroy both the dangling bond (DB) absorption bands, indicative of internal surface area, and the internal porosity of our samples. In addition, we find it takes about a factor of 3 higher fluence to decrease the internal pore volume by 63.2% than it does the internal surface area, which is likely because the surface area decreases by both destruction of the internal pores and also by smaller pores coalescing into large ones. Extrapolating our results to the interstellar medium (ISM), we estimate that the time needed for these processes to occur is significantly shorter than the expected lifetime of a molecular cloud, leading us to speculate that future detections of the DB absorption bands or other indicators of porosity in the ISM will be relatively rare.

Influence of tilting effect on charge structure and lightning flash density in two different convective environments

AbstractThe influence of the tilting effect on charge density and lightning flash density was investigated using idealized Weather Research and Forecasting explicit charging/discharge module (WRF‐ELEC) simulations for two thunderclouds. No shear (NS) and with shear (WS) simulations were conducted based on different values of wind velocity components in input sounding. Results from the NS and WS simulations show that the tilting effect extended the lifetime of the simulated convective clouds in both case studies, while leading to higher maximum vertical velocity only for the environment with intense convection. The ice and graupel in the cloud cell appear almost simultaneously in both the NS and WS simulations for the two case studies, but larger values are obtained for the WS simulations. It is noted that the increase of convection intensity postpones the larger values to the mature stage. The tilting effect results in an increase of total non‐inductive charging, especially in a severe thundercloud. Moreover, the tilting effect does not lead to the same results for the polarity and intensity of charge density in the two studied cases. In the real case study, a dipolar charge structure was seen for both NS and WS simulations, but the intensity of charge density decreased with regard to the tilting effect. In contrast, the intensity of the charge increased with the tilting effect and resulted in tripolarity in the idealized case with a high value of convective available potential energy. Finally, considering the tilting effect leads to an increase of the number of lightning occurrences in the two case studies.