Chiral Spin Liquid State Research Articles

Possible chiral spin liquid state in the S = 1/2 kagome Heisenberg model

The nature of the ground state for the S = 1/2 Kagome Heisenberg antiferromagnet (KHAF) has been elusive. We revisit this challenging problem and provide numerical evidence that its ground state is a chiral spin liquid. Combining the density matrix renormalization group method with analytical analyses, we demonstrate that the previously observed chiral spin liquid phase in the KHAF with longer-range couplings is stable in a broader region of the phase diagram. We characterize the nature of the ground state by computing energy derivatives, revealing the ground-state degeneracy arising from the spontaneous breaking of the time-reversal symmetry, and targeting the semion sector. We further investigate the phase diagram in the vicinity of the KHAF and observe a 3×3\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\sqrt{3}\ imes \\sqrt{3}$$\\end{document} magnetically ordered phase and two valence-bond crystal phases.

Isolated flat bands in 2D lattices based on a novel path-exchange symmetry

The increased ability to engineer two-dimensional (2D) systems, either using materials, photonic lattices, or cold atoms, has led to the search for 2D structures with interesting properties. One such property is the presence of flat bands. Typically, the presence of these requires long-ranged hoppings, fine-tuning of nearest neighbor hoppings, or breaking time-reversal symmetry by using a staggered flux distribution in the unit cell. We provide a prescription based on carrying out projections from a parent system to generate different flat band systems. We identify the conditions for maintaining the flatness and identify a path-exchange symmetry in such systems that cause the flat band to be degenerate with the other dispersive ones. Breaking this symmetry leads to lifting the degeneracy while still preserving the flatness of the band. This technique does not require changing the topology nor breaking time-reversal symmetry as was suggested earlier in the literature. The prescription also eliminates the need for any fine-tuning. Moreover, it is shown that the subsequent projected systems inherit the precise fine-tuning conditions that were discussed in the literature for similar systems, in order to have and isolate a flat band. As examples, we demonstrate the use of our prescription to arrive at the flat band conditions for popular systems like the Kagomé, the Lieb, and the Dice lattices. Finally, we are also able to show that a flat band exists in a recently proposed chiral spin-liquid state of the Kagomé lattice only if it is associated with a gauge field that produces a flux modulation of the Chern-Simons type.

Chiral spin liquid state of strongly interacting bosons with a moat dispersion: A Monte Carlo simulation

We consider a system of strongly interacting bosons in two dimensions with moat band dispersion which supports an infinitely degenerate energy minimum along a closed contour in the Brillouin zone. The system has been theoretically predicted to stabilize a chiral spin liquid (CSL) ground state. In the thermodynamic limit and vanishing densities, n→0, chemical potential, μ, of the uniform CSL state was shown to scale with n as μ∼n2log2n. Here we perform a Monte Carlo simulation to find the parametric window for particle density, n≲k0282π, where k0 is the linear size of the moat (the radius for a circular moat), for which the scaling ∼n2log2n in the equation of state of the homogeneous CSL is preserved. We variationally show that the uniform CSL state is favorable in an interval beyond the obtained scale and present a schematic phase diagram for the system. Our results offer some density estimates for observing the low-density behavior of CSL in time-of-flight experiments with a recently Floquet-engineered moat band system of ultracold atoms in Bracamontes et al. (2022), and for the recent experiments on emergent excitonic topological order in imbalanced electron–hole bilayers.

Gate-tunable heavy fermion quantum criticality in a moiré Kondo lattice

The authors propose a transition metal dichalcogenide moir\'e heterostructure that realizes a Kondo lattice and is capable of tuning across a quantum phase transition corresponding to the breakdown of Kondo screening. For a dual-gated setup, they theoretically identify the requisite gating conditions and find a quantum critical scenario where the local moments in a chiral spin-liquid state dissolve in the conduction electron Fermi sea to form an anomalous Hall heavy-fermion liquid. They discuss how the proposed gate-tunable Kondo lattice simulator can experimentally distinguish between various competing scenarios for the quantum phase transition, and thereby enable progress in the understanding of heavy-fermion quantum criticality.

Generalized Gibbs ensemble description of real-space entanglement spectra of (2+1) -dimensional chiral topological systems with SU(2) symmetry

We provide a quantitative analysis of the splittings in low-lying numerical entanglement spectra (ES), at given momentum, of a number of quantum states that can be identified, based on "Li-Haldane state-counting", as ground states of (2+1)-dimensional chiral topological phases with global SU(2) symmetry. The ability to account for numerical ES splittings solely within the context of conformal field theory (CFT) is an additional diagnostic of the underlying topological theory, of finer sensitivity than "state-counting". We use the conformal boundary state description of the ES, which can be viewed as a quantum quench. In this language, the ES splittings arise from local conservation laws in the chiral CFT besides the energy, which we view as a Generalized Gibbs Ensemble (GGE). Global SU(2) symmetry imposes strong constraints on the number of such conservation laws, so that only a small number of parameters can be responsible for the splittings. We work out these conservation laws for chiral SU(2) Wess-Zumino-Witten CFTs at levels one and two, and for the latter we notably find that some of the conservation laws take the form of local integrals of operators of fractional dimension, as proposed by Cardy for quantum quenches. We analyze numerical ES from systems with SU(2) symmetry including chiral spin-liquid ground states of local 2D Hamiltonians and two chiral Projected Entangled Pair States (PEPS) tensor networks, which exhibit the "state-counting" of the SU(2)-level-one and -level-two theories. We find that the low-lying ES splittings can be well understood by the lowest of our conservation laws, and we demonstrate the importance of accounting for the fractional conservation laws at level two. Thus the states we consider, including the PEPS, appear chiral also under our more sensitive diagnostic.

Bosonic resonating valence bond theory of the possible chiral spin-liquid state in the triangular-lattice Hubbard model

Recent numerical simulations find a possible chiral spin-liquid state in the intermediate coupling regime of the triangular lattice Hubbard model. Here we provide a simple picture for its origin in terms of a bosonic resonating valence bond (RVB) description. More specifically, we show that such a chiral spin-liquid state can be understood as a quantum disordered tetrahedral spin state stabilized by the four spin ring exchange coupling, which suppresses the order-by-disorder effect toward a stripy spin state. Such a chiral spin-liquid state features a spin Berry phase of $\frac{\ensuremath{\pi}}{2}$ per triangle. However, we show that the topological property of such a state is totally missed in the Schwinger boson mean-field description as a result of the lack of boson rigidity caused by the no double occupancy constraint.

Critical dielectric susceptibility at a magnetic BEC quantum critical point

Magnetic-field-induced phase transitions are investigated in the frustrated gapped quantum paramagnet Rb$_{2}$Cu$_{2}$Mo$_3$O$_{12}$ through dielectric and calorimetric measurements on single-crystal samples. It is clarified that the previously reported dielectric anomaly at 8~K in powder samples is not due to a chiral spin liquid state as has been suggested, but rather to a tiny amount of a ferroelectric impurity phase. Two field-induced quantum phase transitions between paraelectric and paramagnetic and ferroelectric and magnetically ordered states are clearly observed. It is shown that the electric polarization is a secondary order parameter at the lower-field (gap closure) quantum critical point but a primary one at the saturation transition. Having clearly identified the magnetic Bose-Einstein condensation (BEC) nature of the latter, we use the dielectric channel to directly measure the critical divergence of BEC susceptibility. The observed power-law behavior is in very good agreement with theoretical expectations for three-dimensional BEC. Finally, dielectric data reveal magnetic presaturation phases in this compound that may feature exotic order with unconventional broken symmetries.

Topological chiral spin liquids and competing states in triangular lattice SU(N) Mott insulators

SU($N$) Mott insulators have been proposed and/or realized in solid-state materials and with ultracold atoms on optical lattices. We study the two-dimensional SU($N$) antiferromagnets on the triangular lattice. Starting from an SU($N$) Heisenberg model with the fundamental representation on each site in the large-$N$ limit, we perform a self-consistent calculation and find a variety of ground states including the valence cluster states, stripe ordered states with a doubled unit-cell and topological chiral spin liquids. The system favors a cluster or ordered ground state when the number of flavors $N$ is less than 6. It is shown that, increasing the number of flavors enhances quantum fluctuations and eventually transfer the clusterized ground states into a topological chiral spin liquids. This chiral spin liquid ground state has an equivalent for the square lattice SU($N$) magnets. We further identify the corresponding lowest competing states that represent another distinct type of chiral spin liquid states. We conclude with a discussion about the relevant systems and the experimental probes.

Doping the chiral spin liquid: Topological superconductor or chiral metal

We point out that there are two different chiral spin liquid states on the triangular lattice and discuss the conducting states that are expected on doping them. These states labeled CS1 and CS2 are associated with two distinct topological orders with different edge states, although they both spontaneously break time reversal symmetry and exhibit the same quantized spin Hall conductance. While CSL1 is related to the Kalmeyer-Laughlin state, CSL2 is the $\nu =4$ member of Kitaev's 16 fold way classification. Both states are described within the Abrikosov fermion representation of spins, and the effect of doping can be accessed by introducing charged holons. On doping CSL2, condensation of charged holons leads to a topological d+id superconductor. However on doping CSL1 , in sharp contrast , two different scenarios can arise: first, if holons condense, a chiral metal with doubled unit cell and finite Hall conductivity is obtained. However, in a second novel scenario, the internal magnetic flux adjusts with doping and holons form a bosonic integer quantum Hall (BIQH) state. Remarkably, the latter phase is identical to a $d+id$ superconductor. In this case the Mott insulator to superconductor transition is associated with a bosonic variant of the integer quantum Hall plateau transition for the holon. We connect the above two scenarios to two recent numerical studies of doped chiral spin liquids on triangular lattice. Our work clarifies the complex relation between topological superconductors, chiral spin liquids and quantum criticality .

Topological Superconductivity in the Doped Chiral Spin Liquid on the Triangular Lattice.

It has long been proposed that doping a chiral spin liquid (CSL) or fractional quantum Hall state can give rise to topological superconductivity. Despite intensive effort, definitive evidences still remain lacking. We address this problem by studying the t-J model supplemented by time-reversal symmetry breaking chiral interaction J_{χ} on the triangular lattice using density-matrix renormalization group with a finite concentration δ of doped holes. It has been established that the undoped, i.e., δ=0, system has a CSL ground state in the parameter region 0.32≤J_{χ}/J≤0.56. Upon light doping, we find that the ground state of the system is consistent with a Luther-Emery liquid with power-law superconducting and charge-density-wave correlations but short-range spin-spin correlations. In particular, the superconducting correlations, whose pairing symmetry is consistent with d±id wave, are dominant at all hole doping concentrations. Our results provide direct evidences that doping the CSL on the triangular lattice can naturally give rise to topological superconductivity.

Chiral spin liquid with spinon Fermi surfaces in the spin- 12 triangular Heisenberg model

We study the interplay of competing interactions in spin-$1/2$ triangular Heisenberg model through tuning the first- ($J_1$), second- ($J_2$), and third-neighbor ($J_3$) couplings. Based on large-scale density matrix renormalization group calculation, we identify a quantum phase diagram of the system and discover a new {\it gapless} chiral spin liquid (CSL) phase in the intermediate $J_2$ and $J_3$ regime. This CSL state spontaneously breaks time-reversal symmetry with finite scalar chiral order, and it has gapless excitations implied by a vanishing spin triplet gap and a finite central charge on the cylinder. Moreover, the central charge grows rapidly with the cylinder circumference, indicating emergent spinon Fermi surfaces. To understand the numerical results we propose a parton mean-field spin liquid state, the $U(1)$ staggered flux state, which breaks time-reversal symmetry with chiral edge modes by adding a Chern insulator mass to Dirac spinons in the $U(1)$ Dirac spin liquid. This state also breaks lattice rotational symmetries and possesses two spinon Fermi surfaces driven by nonzero $J_2$ and $J_3$, which naturally explains the numerical results. To our knowledge, this is the first example of a gapless CSL state with coexisting spinon Fermi surfaces and chiral edge states, demonstrating the rich family of novel phases emergent from competing interactions in triangular-lattice magnets.

Indirect chiral magnetic exchange through Dzyaloshinskii\u2013Moriya-enhanced RKKY interactions in manganese oxide chains on Ir(100)

Localized electron spins can couple magnetically via the Ruderman–Kittel–Kasuya–Yosida interaction even if their wave functions lack direct overlap. Theory predicts that spin–orbit scattering leads to a Dzyaloshinskii–Moriya type enhancement of this indirect exchange interaction, giving rise to chiral exchange terms. Here we present a combined spin-polarized scanning tunneling microscopy, angle-resolved photoemission, and density functional theory study of MnO2 chains on Ir(100). Whereas we find antiferromagnetic Mn–Mn coupling along the chain, the inter-chain coupling across the non-magnetic Ir substrate turns out to be chiral with a 120° rotation between adjacent MnO2 chains. Calculations reveal that the Dzyaloshinskii–Moriya interaction results in spin spirals with a periodicity in agreement with experiment. Our findings confirm the existence of indirect chiral magnetic exchange, potentially giving rise to exotic phenomena, such as chiral spin-liquid states in spin ice systems or the emergence of new quasiparticles.

Impact of off-diagonal exchange interactions on the Kitaev spin-liquid state of α−RuCl3

Motivated by the recent experimental observation of the half-quantized thermal Hall conductivity for the candidate material of the Kitaev spin liquid, $\alpha$-RuCl$_3$[ Y. Kasahara et al., Nature 559, 227 (2018)], we investigate effects of non-Kitaev exchange interactions, which exist in the real material, on the gapped chiral spin liquid state realized in the case with an applied magnetic field. It is found that off-diagonal exchange interactions enhance significantly the mass gap of Majorana fermions. This result provides a possible explanation for robust quantization of the thermal Hall conductivity observed in the above-mentioned experiment. Furthermore, we demonstrate that if the Kitaev spin liquid state and the zigzag antiferromagnetic order coexist around the border of these two phases, off-diagonal exchange interactions can induce Fermi surfaces of Majorana fermions, leading to a state similar to the U(1) spin liquid.

Fermionization of bosons in a flat band

Strongly interacting bosons that live in a lattice with degeneracy in its lowest energy band experience frustration that can prevent the formation of a Bose-Einstein condensate. Such systems form an ideal playground to investigate spin-liquid behavior. We use the variational principle and the Chern-Simons technique of fermionization of hard-core bosons on Kagome lattice to find that below lattice filling fraction $\nu=1/3$ the system favors a topologically ordered chiral spin-liquid state that is gapped in bulk, spontaneously breaks Time-Reversal Symmetry, and supports massless chiral bosonic edge mode. We construct the many-body variational wave function of the state and show that the corresponding energy coincides with the energy of the flat band. This result proves that the ground state of the system cannot stabilize a Bose condensate below $\nu=1/3$. The fermionization and variational scheme we outline apply to any non-Bravais lattice. We distinguish between the roles played by the Chern-Simons gauge field in lattices with a flat band and those exhibiting a moat-like dispersion (which is degenerate along a closed contour in the reciprocal space). We also suggest experimental probes to differentiate the proposed ground state from a condensate.

Effective field theory of chiral spin liquid between ordered phases in a kagome antiferromagnet

We propose in this work an effective field theory description of the chiral spin liquid state in a Heisenberg spin system on a kagome lattice. To this end, we derive the low-energy effective theory of a kagome (isotropic) Heisenberg antiferromagnet around its ordered ground states found numerically and show that quantum fluctuations induced by further neighbor spin exchanges are equally strong as those from the first neighbor. We use a chiral order parameter theory to argue for the occurrence of finite temperature chiral symmetry breaking transition into a chiral ordered state in a kagome antiferromagnet with further neighbor spin exchange interactions. We compute the chiral symmetry breaking term in the effective ground state energy and show that chiral spin liquid necessarily occurs in the ground state of a kagome antiferromagnet with the first three nearest-neighbor spin exchange interactions. Finally, we consider the quantum criticality of the kagome antiferromagnet and show that a Chern–Simons term emerges naturally at the transition between the two ordered states that satisfy an appropriate ‘matching condition’ that we derive, providing an explanation for why chiral spin liquid could occur at the transition between appropriate ordered states. This emergent Chern–Simons term is the low energy effective theory of the chiral spin liquid state, where the chirality is the immediate consequence of the breaking of discrete symmetries by this topological field theory.

Emergent Chiral Spin State in the Mott Phase of a Bosonic Kane-Mele-Hubbard Model.

Recently, the frustrated XY model for spins 1/2 on the honeycomb lattice has attracted a lot of attention in relation with the possibility to realize a chiral spin liquid state. This model is relevant to the physics of some quantum magnets. Using the flexibility of ultracold atom setups, we propose an alternative way to realize this model through the Mott regime of the bosonic Kane-Mele-Hubbard model. The phase diagram of this model is derived using bosonic dynamical mean-field theory. Focusing on the Mott phase, we investigate its magnetic properties as a function of frustration. We do find an emergent chiral spin state in the intermediate frustration regime. Using exact diagonalization we study more closely the physics of the effective frustrated XY model and the properties of the chiral spin state. This gapped phase displays a chiral order, breaking time-reversal and parity symmetry, but is not topologically ordered (the Chern number is zero).

Weyl magnons in noncoplanar stacked kagome antiferromagnets

Weyl nodes have been experimentally realized in photonic, electronic, and phononic crystals. However, magnonic Weyl nodes are yet to be seen experimentally. In this paper, we propose Weyl magnon nodes in noncoplanar stacked frustrated kagome antiferromagnets, naturally available in various real materials. Most crucially, the Weyl nodes in the current system occur at the lowest excitation and possess a topological (anomalous) thermal Hall effect, therefore they are experimentally accessible at low temperatures due to the population effect of bosonic quasiparticles. In stark contrast to other magnetic systems, the current Weyl nodes do not rely on time-reversal symmetry breaking by the magnetic order. Rather, they result from explicit macroscopically broken time reversal symmetry by the scalar spin chirality of noncoplanar spin textures, and can be generalized to chiral spin liquid states. Moreover, the scalar spin chirality gives a real space Berry curvature which is not available in previously studied magnetic Weyl systems. We show the existence of magnon arc surface states connecting projected Weyl magnon nodes on the surface Brillouin zone. We also uncover the first realization of triply-degenerate nodal magnon point in the non-collinear regime with zero scalar spin chirality.

Chiral quantum spin liquid on the repulsive Haldane–Hubbard model in square lattices

In this paper, we present a study on the repulsive Haldane–Hubbard model with spin-rotation symmetry in square lattices by deriving non-linear σ model for magnetic states. It is found that a chiral spin liquid state as the ground state of the correlated system exists in the topological spin-density wave proposed by Wu et al (2016 J. Phys.: Condens. Matter 28 115602), of which the low energy physics can be determined by the Chern–Simons–Hopf gauge field theory.

Possible SU(3) chiral spin liquid on the kagome lattice

We propose an SU(3) symmetric Hamiltonian with short-range interactions on the Kagome lattice and show that it hosts an Abelian chiral spin liquid (CSL) state. We provide numerical evidence based on exact diagonalization to show that this CSL state is stabilized in an extended region of the parameter space and can be viewed as a lattice version of the Halperin 221 fractional quantum Hall (FQH) state of two-component bosons. We also construct a parton wave function for this CSL state and demonstrate that its variational energies are in good agreement with exact diagonalization results. The parton description further supports that the CSL is characterized by a chiral edge conformal field theory (CFT) of the SU(3)_1 Wess-Zumino-Witten type.

Spin structure factors of chiral quantum spin liquids on the kagome lattice

We calculate dynamical spin structure factors for gapped chiral spin liquid states in the spin-1/2 Heisenberg antiferromagnet on the kagome lattice using Schwinger-boson mean-field theory. In contrast to static (equal-time) structure factors, the dynamical structure factor shows clear signatures of time-reversal symmetry breaking for chiral spin liquid states. In particular, momentum inversion $\bm{k} \to -\bm{k}$ symmetry as well as the six-fold rotation symmetry around the $\Gamma$-point are lost. We highlight other interesting features, such as a relatively flat onset of the two-spinon continuum for the \emph{cuboc1} state. Our work is based on the projective symmetry group classification of time-reversal symmetry breaking Schwinger-boson mean-field states by Messio, Lhuillier, and Misguich.