Chiral Dynamics Research Articles

Real-time chiral dynamics at finite temperature from quantum simulation

In this study, we explore the real-time dynamics of the chiral magnetic effect (CME) at a finite temperature in the (1+1)-dimensional QED, the massive Schwinger model. By introducing a chiral chemical potential μ5 through a quench process, we drive the system out of equilibrium and analyze the induced vector currents and their evolution over time. The Hamiltonian is modified to include the time-dependent chiral chemical potential, thus allowing the investigation of the CME within a quantum computing framework. We employ the quantum imaginary time evolution (QITE) algorithm to study the thermal states, and utilize the Suzuki-Trotter decomposition for the real-time evolution. This study provides insights into the quantum simulation capabilities for modeling the CME and offers a pathway for studying chiral dynamics in low-dimensional quantum field theories.

Chiral edge states and direct edge-to-edge transport in a bosonic magnetic ladder

Abstract Three-legged magnetic ladder reproduces the main features of two-dimensional Hofstadter butterfly spectrum and the related Chern insulating phases with typical topological edge states, providing new opportunity to study novel quantum states and chiral physics. Here, we propose an efficient scheme to detect various edge states and realize edge-to-edge transport in a three-legged bosonic magnetic ladder. Under the mean field approximation, the eigenstates, chiral edge-state dynamics, and edge-to-edge transport in the system are studied. The energy spectrum and the eigenstates of the system are presented, and both bulk and edge states are obtained, depending on the energy spectrum of the system. The existence of rich edge states (including symmetric and unsymmetric edge states) provides the evidence for realizing the topological transport in the system. Furthermore, chiral edge-state dynamics is excited by applying a weak linear external force, reproducing the underlying eigenstates dynamically, offering a robust way to detect the edge states of the system. Particularly, direct edge-to-edge transport is observed which can be identified by the observables (spin polarization, spin tensor, and chiral currents). The reversal of chiral currents induces the edge-to-edge transport. The edge-to-edge transport time can be manipulated by adjusting the external force and magnetic field. We provide a robust and efficient atomic transport scheme with potential applications in manipulating topological quantum transport and storing quantum states in the ultracold atomic system.

Chiral dynamics of ultracold atoms under a tunable SU(2) synthetic gauge field

Chiral dynamics of ultracold atoms under a tunable SU(2) synthetic gauge field

Non-Abelian chiral dynamics in a lattice under synthetic SU(2) gauge fields

Non-Abelian chiral dynamics in a lattice under synthetic SU(2) gauge fields

Giant Piezoelectric Effects of Topological Structures in Stretched Ferroelectric Membranes.

Freestanding ferroelectric oxide membranes emerge as a promising platform for exploring the interplay between topological polar ordering and dipolar interactions that are continuously tunable by strain. Our investigations combining density functional theory (DFT) and deep-learning-assisted molecular dynamics simulations demonstrate that DFT-predicted strain-driven morphotropic phase boundary involving monoclinic phases manifest as diverse domain structures at room temperatures, featuring continuous distributions of dipole orientations and mobile domain walls. Detailed analysis of dynamic structures reveals that the enhanced piezoelectric response observed in stretched PbTiO_{3} membranes results from small-angle rotations of dipoles at domain walls, distinct from conventional polarization rotation mechanism and adaptive phase theory inferred from static structures. We identify a ferroelectric topological structure, termed "dipole spiral," which exhibits a giant intrinsic piezoelectric response (>320 pC/N). This helical structure, possessing a rotational zero-energy mode, unlocks new possibilities for exploring chiral phonon dynamics and dipolar Dzyaloshinskii-Moriya-like interactions.

Chiral dynamics in soft triaxial nuclei

The chirality in soft triaxial nuclei is investigated for the first time with the time-dependent and tilted axis cranking covariant density functional theories on a three-dimensional space lattice in a microscopic and self-consistent way. Taking the puzzling chiral nucleus 106Ag as an example, the experimental energies of the observed nearly degenerate bands are well reproduced without any free parameters beyond the well-defined density functional. A novel chiral mode in soft triaxial nuclei is newly revealed from the microscopic dynamics of the total angular momentum. This opens a new research area for the study of chirality, particularly in relation to soft nuclear shapes.

Chiral dynamics of three-mode non-Hermitian systems with a periodical driving

Chiral dynamics of three-mode non-Hermitian systems with a periodical driving

Transient Chiral Dynamics in the Fenna-Matthews-Olson Complex Revealed by Two-Dimensional Circular Dichroism Spectroscopy.

Chirality plays a pivotal role across scientific disciplines with profound implications spanning light-matter interactions, molecular recognition, and natural evolutionary processes. This study delves into the active influence of molecular chirality on exciton energy transfer within photosynthetic protein complexes, focusing on the Fenna-Matthews-Olson (FMO) complex. Employing two-dimensional circular dichroism (2DCD) spectroscopy, we investigate the transient chiral dynamics of excitons during energy transfer processes within the FMO complex. Our approach, incorporating pulse information into population dynamics based on the third-order response function, facilitates the calculation of 2DCD spectra and dynamics. This enables the extraction of chiral contributions to excitonic energy transfer and the examination of electronic wave functions. We demonstrate that 2DCD spectra offer excitation energies that are better resolved than those from conventional two-dimensional electronic spectroscopy. These findings deepen our understanding of exciton energy transfer mechanisms in natural photosynthesis, emphasizing the potential of 2DCD spectroscopy as a powerful tool for unraveling the chiral contribution to exciton dynamics.

Unified unquenched quark model for heavy-light mesons with chiral dynamics

In this work, an unquenched quark model is proposed for describing the heavy-light mesons by taking into account the coupled-channel effects induced by chiral dynamics. After including a relativistic correction term for the strong transition amplitudes, both the mass spectra and decay widths of the observed heavy-light mesons can be successfully described simultaneously in a unified framework, several long-standing puzzles related to the small masses and broad widths are overcome naturally. We also provide valuable guidance in searching new heavy-light mesons by the detailed predictions of their masses, widths, and branching ratios. The success of the unquenched quark model presented in this work indicates it may be an important step for understanding the hadron spectrum. Published by the American Physical Society 2024

Manipulating ultrafast even-order nonlinear chiral responses of L-tryptophan by polarization pulse shaping

Molecular chirality has long been monitored in the frequency domain in the ultraviolet, visible, and infrared regimes. Recently developed time-domain approaches can detect time-dependent chiral dynamics by enhancing intrinsically weak chiral signals. Even-order nonlinear signals in chiral molecules have gained attention thanks to their existence in the electric dipole approximation, without relying on the weaker higher-order multipole interactions. We illustrate the optimization of temporal polarization pulse-shaping in various frequency ranges (infrared/optical and optical/X ray) to enhance chiral nonlinear signals. These signals can be recast as an overlap integral of matter and field pseudoscalars which contain the relevant chiral information. Simulations are carried out for second- and fourth-order nonlinear spectroscopies in L-tryptophan.

Dynamical encircling of multiple exceptional points in anti-PT symmetry system

Exceptional points (EPs) in non-Hermitian systems have turned out to be at the origin of many intriguing effects with no counterparts in Hermitian cases. A typically interesting behavior is the chiral mode switching by dynamically winding the EP. Most encircling protocols focus on the two-state or parity-time (PT) symmetry systems. Here, we propose and investigate the dynamical encircling of multiple EPs in an anti-PT-symmetric system, which is constructed based on a one-dimensional lattice with staggered lossy modulation. We reveal that dynamically encircling the multiple EPs results in the chiral dynamics via multiple non-Hermiticity-induced nonadiabatic transitions, where the output state is always on the lowest-loss energy sheet. Compared with the PT-symmetric systems that require complicated variation of the gain/loss rate or on-site potentials, our system only requires modulations of the couplings which can be readily realized in various experimental platforms. Our scheme provides a route to study non-Hermitian physics by engineering the EPs and implement novel photonic devices with unconventional functions.

Rydberg Platform for Nonergodic Chiral Quantum Dynamics.

We propose a mechanism for engineering chiral interactions in Rydberg atoms via a directional antiblockade condition, where an atom can change its state only if an atom to its right (or left) is excited. The scalability of our scheme enables us to explore the many-body dynamics of kinetically constrained models with unidirectional character. We observe nonergodic behavior via either scars, confinement, or localization, upon simply tuning the strength of two driving fields acting on the atoms. We discuss how our mechanism persists in the presence of classical noise and how the degree of chirality in the interactions can be tuned, opening towards the frontier of directional, strongly correlated, quantum mechanics using neutral atoms arrays.

Capturing electron-driven chiral dynamics in UV-excited molecules

Chiral molecules, used in applications such as enantioselective photocatalysis1, circularly polarized light detection2 and emission3 and molecular switches4,5, exist in two geometrical configurations that are non-superimposable mirror images of each other. These so-called (R) and (S) enantiomers exhibit different physical and chemical properties when interacting with other chiral entities. Attosecond technology might enable influence over such interactions, given that it can probe and even direct electron motion within molecules on the intrinsic electronic timescale6 and thereby control reactivity7–9. Electron currents in photoexcited chiral molecules have indeed been predicted to enable enantiosensitive molecular orientation10, but electron-driven chiral dynamics in neutral molecules have not yet been demonstrated owing to the lack of ultrashort, non-ionizing and perturbative light pulses. Here we use time-resolved photoelectron circular dichroism (TR-PECD)11–15 with an unprecedented temporal resolution of 2.9 fs to map the coherent electronic motion initiated by ultraviolet (UV) excitation of neutral chiral molecules. We find that electronic beatings between Rydberg states lead to periodic modulations of the chiroptical response on the few-femtosecond timescale, showing a sign inversion in less than 10 fs. Calculations validate this and also confirm that the combination of the photoinduced chiral current with a circularly polarized probe pulse realizes an enantioselective filter of molecular orientations following photoionization. We anticipate that our approach will enable further investigations of ultrafast electron dynamics in chiral systems and reveal a route towards enantiosensitive charge-directed reactivity.

Magnetic-induced chiral dynamics in an extended two-leg bosonic ladder

The realization and detection of chiral physics with ultracold atomic gases provide a unique path for the exploration of topological phases. Here, we show that the interplay of magnetic field and interacting particles in an extended two-leg ladder leads to rich chiral Bloch dynamics. Considering both the on-site contact interaction and nearest-neighbor interactions, the ground state and Bloch dynamics of the system are studied analytically and numerically. When the system is in the ground state, the threshold and phase diagram for the transition between zero-momentum state and plane-wave state are analytically obtained, showing the nearest-neighbor interactions along the legs and rungs have opposite impact on the ground state transition, providing new opportunity to manipulate the ground state transition. When the ladder is perturbated under an external linear force, chiral dephasing of Bloch oscillations (BOs), i.e. symmetry breaking damped BOs (the damping rate of BOs on one leg is larger than the other), are observed. This chirality is absent for vanishing the magnetic field and atomic interaction. Particularly, the chirality of damped BOs is inversed when the magnetic field (chiral current) is inversed. In addition, the damping of BOs induced by different types of atomic interactions is different, and the strength and damping rate of BOs initialized in different ground states are distinct, offering dynamic ways to detect the different ground states. Furthermore, the persistent chiral Bloch oscillations observed in single particle case is predicted analytically, which is a crucial requirement for observation and application of chiral BOs in nonlinear regime. Our results provide an interesting path towards the exploration of topological atomic superfluids.

Chiral spin textures creation and dynamics in a rectangular nanostructure

Abstract Controlled creation of stable chiral spin textures is required to use them as an energy-efficient information carrier in spintronics. Here we have studied the stable creation of isolated chiral spin texture (skyrmion and antiskyrmion) and its pair through the magnetization reversal of a rectangular nanostructure using spin-polarized currents. An isolated spin texture is created through a negative current pulse. Dynamics of the stable spin texture are explored under external magnetic fields, and the resonant frequencies are calculated. A stable skyrmion pair is created using an asymmetric current pulse, and their interaction is studied using the Thiele equation. The stability of isolated or paired spin texture depends on the Dzyaloshinskii–Moriya interaction strength, spin-polarized current density, and pulse duration. In addition, the stability of the skyrmion pair depends on their initial separation, and a threshold for the separation between skyrmions of 78 nm is observed.

Hosting exceptional point in all-lossy dual-core optical fiber and its exotic chiral light dynamics

Exploration of exceptional points (EPs) and associated unique features in gain-loss assisted optical systems to develop future all optical devices have been a great interest in recent years. However, incorporation and adjustment of gain distribution in a system is quite challenging. Here, we design a fabrication feasible dual-core optical fiber where only the customized transverse loss profile controls the interaction between two coupled modes and results in hosting an EP. Parametric encirclement of the identified EP and corresponding chirality-driven asymmetric mode conversion phenomenon between the supported modes have been reported. The proposed structure features ease of fabrication using state-of-the-art techniques with possible applications in all-optical components for communication and all fiber photonic devices.

Chiral transmission by an open evolution trajectory in a non-Hermitian system

Exceptional points (EPs), at which two or more eigenvalues and eigenstates of a resonant system coalesce, are associated with non-Hermitian Hamiltonians with gain and/or loss elements. Dynamic encircling of EPs has received significant interest in recent years, as it has been shown to lead to highly nontrivial phenomena, such as chiral transmission in which the final state of the system depends on the encircling handedness. Previously, chiral transmission for a pair of eigenmodes has been realized by establishing a closed dynamical trajectory in parity-time- (PT-) or anti-PT-symmetric systems. Although chiral transmission of symmetry-broken modes, more accessible in practical photonic integrated circuits, has been realized by establishing a closed trajectory encircling EPs in anti-PT-symmetric systems, the demonstrated transmission efficiency is very low due to path-dependent losses. Here, we demonstrate chiral dynamics in a coupled waveguide system that does not require a closed trajectory. Specifically, we explore an open trajectory linking two infinite points having the same asymptotic eigenmodes (not modes in PT- and anti-PT-symmetric systems), demonstrating that this platform enables high-efficiency chiral transmission, with each eigenmode localized in a single waveguide. This concept is experimentally implemented in a coupled silicon waveguide system at telecommunication wavelengths. Our work provides a new evolution strategy for chiral dynamics with superior performance, laying the foundation for the development of practical chiral-transmission devices.

Laser-Induced Electron Diffraction in Chiral Molecules

Strong laser pulses enable probing molecules with their own electrons. The oscillating electric field tears electrons off a molecule, accelerates them, and drives them back toward their parent ion within a few femtoseconds. The electrons are then diffracted by the molecular potential, encoding its structure and dynamics with angstrom and attosecond resolutions. Using elliptically polarized laser pulses, we show that laser-induced electron diffraction is sensitive to the chirality of the target. The field selectively ionizes molecules of a given orientation and drives the electrons along different sets of trajectories, leading them to recollide from different directions. Depending on the handedness of the molecule, the electrons are preferentially diffracted forward or backward along the light propagation axis. This asymmetry, reaching several percent, can be reversed for electrons recolliding from two ends of the molecule. The chiral sensitivity of laser-induced electron diffraction opens a new path to resolve ultrafast chiral dynamics. Published by the American Physical Society 2024

Dynamical chirality production in one dimension

Dynamical chirality production in one dimension

Thermodynamics of quark matter with multiquark clusters in an effective Beth-Uhlenbeck type approach

We describe multiquark clusters in quark matter within a Beth-Uhlenbeck approach in a background gluon field coupled to the underlying chiral quark dynamics using the Polyakov gauge. An effective potential for the traced Polyakov loop is used to establish the center symmetry of the SU(3) color which suppresses colored states and its dynamical breaking as an aspect of the confinement/deconfinement transition. Quark confinement is modeled by a large quark mass in vacuum which is motivated by a confining density functional approach. A multiquark cluster containing n quarks and antiquarks is described as a binary composite of smaller subclusters n1\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$n_1$$\\end{document} and n2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$n_2$$\\end{document} (n1+n2=n\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$n_1+n_2=n$$\\end{document}). It has a spectrum consisting of a bound state and a scattering state continuum. For the corresponding cluster-cluster phase shifts we use simple ansätze that capture the Mott dissociation of clusters as a function of temperature and chemical potential. We go beyond the simple “step-up-step-down” model that ignores continuum correlations and introduce an improved model that includes them in a generic form. In order to explain the model, we restrict ourselves here to the cases where the cluster size is 1≤n≤6\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$1 \\le n \\le 6$$\\end{document}. A striking result is the suppression of the abundance of colored multiquark clusters at low temperatures by the coupling to the Polyakov loop and their importance for a quantitative description of lattice QCD thermodynamics at non-vanishing baryochemical potentials. An important ingredient are Polyakov-loop generalized distribution functions of n-quark clusters which are derived here for the first time. Within our approach we calculate thermodynamic properties such as baryon density and entropy. We demonstrate that the limits of a hadron resonance gas at low temperatures and O(g2)\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\mathcal {O}(g^2)$$\\end{document} perturbative QCD at high temperatures are correctly reproduced. A comparison with lattice calculations shows that our model is able to give a unified, systematic approach to describe properties of the quark-gluon-hadron system.