In response to the government’s heightened focus on recycling and remanufacturing, as well as the growing awareness among consumers about environmental security, manufacturing companies are currently required to establish efficient closed-loop supply chain networks in order to improve their socialreputation and competitive advantage. This study investigates the optimization of a Closed-Loop Supply Chain (CLSC) network that involves multiple products, multiple periods, and uncertain returns, which also considers the influence of many factors, such as carbon cap-and-trade policy, raw part procurement discounts, and facility capacity constraints, on the supply chain. Simultaneously, customer demand is sensitive to both product pricing and product greenness, and product greenness can be improved by investing in emission reduction technologies. To address the uncertainty in the returns, we propose a two-stage distributionally robust chance-constrained optimization model, which is transformed into a mixed integer linear programming model. To efficiently address the complex problem, we designan improved Benders decomposition (IBD) algorithm. The experimental results confirm that the IBD algorithm has significant advantages when compared to the Benders decomposition algorithm. Additionally, this study conducted a sensitivity analysis on key parameters and proposed operation suggestions of practical importance.