Cavity Photon Research Articles

Dissipation-induced nonreciprocal magnon blockade in a magnon-based hybrid system

We propose an experimentally realizable nonreciprocal magnonic device at the single-magnon level by exploiting magnon blockade in a magnon-based hybrid system. The coherent qubit-magnon coupling, mediated by virtual photons in a microwave cavity, leads to the energy-level anharmonicity of the composite modes. In contrast, the corresponding dissipative counterpart, induced by traveling microwaves in a waveguide, yields inhomogeneous broadenings of the energy levels. As a result, the cooperative effects of these two kinds of interactions give rise to the emergence of the direction-dependent magnon blockade. We show that this can be demonstrated by studying the equal-time second-order correlation function of the magnon mode. Our study opens an avenue to engineer nonreciprocal magnonic devices in the quantum regime involving only a small number of magnons.

Topological band structure via twisted photons in a degenerate cavity

Synthetic dimensions based on particles’ internal degrees of freedom, such as frequency, spatial modes and arrival time, have attracted significant attention. They offer ideal large-scale lattices to simulate nontrivial topological phenomena. Exploring more synthetic dimensions is one of the paths toward higher dimensional physics. In this work, we design and experimentally control the coupling among synthetic dimensions consisting of the intrinsic photonic orbital angular momentum and spin angular momentum degrees of freedom in a degenerate optical resonant cavity, which generates a periodically driven spin-orbital coupling system. We directly characterize the system’s properties, including the density of states, energy band structures and topological windings, through the transmission intensity measurements. Our work demonstrates a mechanism for exploring the spatial modes of twisted photons as the synthetic dimension, which paves the way to design rich topological physics in a highly compact platform.

Laser induced enhanced coupling between photons and squeezed magnons in antiferromagnets

In this paper we consider a honeycomb antiferromagnet subject to an external laser field. Obtaining a time-independent effective Hamiltonian, we find that the external laser renormalizes the exchange interaction between the in-plane components of the spin-operators, and induces a synthetic Dzyaloshinskii–Moria interaction (DMI) between second neighbors. The former allows the control of the magnon dispersion’s bandwidth and the latter breaks time-reversal symmetry inducing non-reciprocity in momentum space. The eigen-excitations of the system correspond to squeezed magnons whose squeezing parameters depend on the properties of the laser. When studying how these spin excitations couple with cavity photons, we obtain a coupling strength which can be enhanced by an order of magnitude via careful tuning of the laser’s intensity, when compared to the case where the laser is absent. The transmission plots through the cavity are presented, allowing the mapping of the magnons’ dispersion relation.

Rydberg exciton-polaritons in a Cu2O microcavity.

Giant Rydberg excitons with principal quantum numbers as high as n = 25 have been observed in cuprous oxide (Cu2O), a semiconductor in which the exciton diameter can become as large as ∼1 μm. The giant dimension of these excitons results in excitonic interaction enhancements of orders of magnitude. Rydberg exciton-polaritons, formed by the strong coupling of Rydberg excitons to cavity photons, are a promising route to exploit these interactions and achieve a scalable, strongly correlated solid-state platform. However, the strong coupling of these excitons to cavity photons has remained elusive. Here, by embedding a thin Cu2O crystal into a Fabry-Pérot microcavity, we achieve strong coupling of light to Cu2O Rydberg excitons up to n = 6 and demonstrate the formation of Cu2O Rydberg exciton-polaritons. These results pave the way towards realizing strongly interacting exciton-polaritons and exploring strongly correlated phases of matter using light on a chip.

Temperature dependence of the single photon source efficiency based on QD-cQED

We study a photonic circuit consisting of a quantum dot, QD, coupled to a photon cavity over a wide range of temperature up to room temperature. A key component of such a system is presented here in the form of a Purcell-enhanced single-photon source based on Cavity Quantum Electrodynamics, cQED. We use a real set of pure dephasing data extracted from experimental measurements of InGaAs QD to calculate the effective QD-cavity coupling strength, the Purcell factor, and the single photon efficiency emerged from the QD-cavity system in the cases without and with detuning. In the non-detuned system, the effective coupling strength between the QD and the resonator decreases with increasing temperature, results in a decrease in efficiency. However, when the temperature of the QD-cavity system increases under Purcell effect conditions, the detuned QD-cavity system induces spontaneous emission rate enhancement. As a result, we found that the increase in efficiency can be obtained under a certain condition, when the maximum effective coupling strength and the Purcell factor are related to the spontaneous emission and the pure dephasing rates. Additionally, the influences of the pumping mechanism on the efficiency of the QD-system were examined and showed that the pumping process can be used to further increase in efficiency. Our results can be advantageous for advanced quantum optics applications once temperature is taken into account.

Can a terahertz metamaterial sensor be improved by ultra-strong coupling with a high-Q photonic resonator?

When a metamaterial (MM) is embedded in a one-dimensional photonic crystal (PC) cavity, the ultra-strong coupling between the MM plasmons and the photons in the PC cavity gives rise to two new polariton modes with high quality factor. Here, we investigate by simulations whether such a strongly coupled system working in the terahertz (THz) frequency range has the potential to be a better sensor than a MM (or a PC cavity) alone. Somewhat surprisingly, one finds that the shift of the resonance frequency induced by an analyte applied to the MM is smaller in the case of the dual resonator (MM and cavity) than that obtained with the MM alone. However, the phase sensitivity of the dual resonator can be larger than that of the MM alone. With the dielectric perturbation theory - well established in the microwave community - one can show that the size of the mode volume plays a decisive role for the obtainable frequency shift. The larger frequency shift of the MM alone is explained by its smaller mode volume as compared with the MM-loaded cavity. Two main conclusions can be drawn from our investigations. First, that the dielectric perturbation theory can be used to guide and optimize the designs of MM-based sensors. And second, that the enhanced phase sensitivity of the dual resonator may open a new route for the realization of improved THz sensors.

The linear and nonlinear inverse Compton scattering between microwaves and electrons in a resonant cavity

The new scheme of the energy measurement of the extremely high energy electron beam with the inverse Compton scattering between electrons and microwave photons requires the precise calculation of the interaction cross section of electrons and microwave photons in a resonant cavity. In the local space of the cavity, the electromagnetic field is expressed by Bessel functions. Although Bessel functions can form a complete set of orthogonal basis, it is difficult to quantify them directly as fundamental wave functions. Fortunately, with the Fourier expansion of Bessel functions, the local electromagnetic field can be considered as the superposition of a series of plane waves. Therefore, with corresponding corrections of the cross section formula of the classical Compton scattering, the cross section of the linear or nonlinear microwave Compton scattering in the local space can be described accurately. As an important application of our results in astrophysics, corresponding ground verification devices can be designed to perform experimental verifications on the prediction of the Sunyaev–Zeldovich (SZ) effect of the cosmic microwave background radiation. Our results could also provide a new way to generate wave sources with strong practical value, such as the terahertz waves, the ultra-violet (EUV) waves, or the mid-infrared beams.

Excitation-polarization-dependent dynamics of polariton condensates in the ZnO microwire at room temperature

Based on ZnO microcavities with high quality factors, where the gain medium exhibits confinement of wave packets due to the intrinsically formed whispering gallery microcavity, strong coupling between excitons and cavity photons can be obtained at room temperature resulting in hybrid quasiparticles, e.g. exciton polaritons. In this work, polariton condensation is induced under the non-resonant excitation by linearly polarized femtosecond laser pulses with different polarization directions. The dynamical angle-resolved k-space spectra of the photoluminescence emission of polariton condensates are measured with sub-picosecond resolution by the self-developed femtosecond angle-resolved spectroscopic imaging technique. Our results show that the ultrafast dynamics of polariton condensation is sensitive to the polarization direction of the excitation pulses which can be explained qualitatively by the combined effect of selective excitation of distinct exciton modes in the sample and the effective coupling strength of the excitation pulses in the ZnO microcavity for various polarization directions. This work strengthened the understanding of the condensation process for cavity exciton polaritons at room temperature.

Slow-light dispersion of a cavity polariton in an organic crystal microcavity

Herein, we have measured the phase dispersion of a cavity polariton in a single-crystalline anthracene microcavity via interference spectroscopy. Results show slow-light dispersion at the cavity polariton's lower polariton resonance, which agrees well with the transfer matrix method calculation results. According to the theoretical calculations, the slow-light dispersion's group refractive index is 24. We found that the structural dispersion due to a phenomenological photon cavity and material dispersion caused by the exciton contributed to the large group refractive index. These efforts will aid in realizing optical buffer memories for organic microcavities.

Toward a Quantum Memory in a Fiber Cavity Controlled by Intracavity Frequency Translation.

We propose a quantum memory protocol based on trapping photons in a fiber-integrated cavity, comprised of a birefringent fiber with dichroic reflective end facets. Photons are switched into resonance with the fiber cavity by intracavity Bragg-scattering frequency translation, driven by ancillary control pulses. After the storage delay, photons are switched out of resonance with the cavity, again by intracavity frequency translation. We demonstrate storage of quantum-level THz-bandwidth coherent states for a lifetime up to 16 cavity round trips, or 200ns, and a maximum overall efficiency of 73%.

Olfactory Sensations During Proton and Photon Radiotherapy: A Multicenter Prospective Observational Study.

Purpose: Patients often report a sense of smell during radiation therapy (RT), but the details of these events are not well understood. The purpose of the study was to evaluate events of smell during photon RT and proton beam therapy (PBT).Methods and materials: The subjects were all adult patients (≥20 years old) treated with photon RT or PBT at two centers from January 2019 to August 2020, with the exclusion of those with communication difficulties or olfactory abnormality. The presence of smell, odor type, intensity (five levels), and time period was examined prospectively using a weekly checklist.Results: A total of 649 courses were examined in 620 patients who received photon RT (n=415) or PBT (n=205). A smell during the procedure was sensed by 51 patients (8.2%). In multivariate logistic regression analysis, nasal cavity dose (p=0.002), age (p<0.001), and photon RT (p=0.018) were identified as significant factors associated with a sense of smell. Smell occurred in only 23/515 patients (4.5%) in whom the nasal cavity was not irradiated, but in 4/19 (21.1%) and 24/86 (27.9%) with nasal cavity maximum isodose lines of 10%-50% and 60%-100%, respectively. Patients who received photon RT sensed a smell (43/415; 10.4%) more frequently than those treated with PBT (8/205; 3.9%). Of the 51 patients who sensed a smell, 32 (63%) reported a burnt smell, eight (16%) a chemical smell, two (4%) a sour smell, and nine another smell (copier machine, sweet, garbage, etc.).Conclusions: The sense of a smell appears to be common during RT and this sensation is significantly associated with the nasal cavity dose, younger age, and photon RT.

Dissipation and spontaneous emission in quantum electrodynamical density functional theory based on optimized effective potential: A proof of concept study

We generalize the optimized effective potential (OEP) formalism in the quantum electrodynamical density functional theory (QEDFT) to the case of continuous distribution of photon modes, and study its applicability to dissipative dynamics of electron systems interacting with photons of lossy cavities. Specifically, we test whether this technique is capable of capturing the quantum features of electron-photon interaction related to spontaneous emission and the corresponding energy transfer from the electrons to cavity photons. For this purpose, we analyze a discrete three-site system with one electron coupled to photons of the cavity, which, in fact, is a minimal model allowing to eliminate classical radiation and the corresponding energy loss, but still have nontrivial density dynamics. By considering two typical spectral densities of photon modes, modeling (i) lossy cavity with Lorentzian broadening of photon peaks, and (ii) the Ohmic bath, and several representative dynamical regimes, we find that OEP-QEDFT demonstrates a good qualitative and quantitative performance, especially in the case when the disspation is dominated by one-photon processes.

Localization of Laterally Confined Modes in a 2D Semiconductor Microcavity

Monolayer semiconductor embedded planar microcavities are becoming a promising light-matter interacting system to uncover a wealth of photonic, excitonic, and polaritonic physics at the two-dimensional (2D) limit. In these 2D semiconductor microcavities employing the longitudinal Fabry-Perot resonance, major attention has been paid to the coupling of excitons with vertically confined cavity photons; by contrast, the lateral confinement effect on exciton-photon interactions is still elusive. Here we observe the localized distribution of laterally confined modes with discrete energies in a 2D semiconductor embedded microcavity. Monolayer tungsten disulfides with equilateral triangular geometries but varied edge lengths are selected as the active media incorporated into a dielectric planar microcavity. With the shortening of the edge length, photoluminescence mappings of active regions present spatially localized emission patterns, which are attributed to the presence of in-plane triangular waveguiding resonance caused by total internal reflection at the one-dimensional closed boundary between the monolayer semiconductor and its surrounding cavity material. Unlike the conventional quantum confinement effect of native excitons appearing at the nanometer scale, the mode emission at the active-medium center exhibits apparent size-dependent features at the micrometer scale due to the optical confinement effect correlated with its photonic nature. By reducing the area of active media, single-mode dominant emission is achieved together with its nondispersive energy and improved directionality. Our work highlights the crucial role of lateral mode control in monolayer semiconductor embedded planar microcavities and encourages the investigation of the quantum billiard problem in 2D semiconductors.

Hybridized Exciton-Photon-Phonon States in a Transition Metal Dichalcogenide van der Waals Heterostructure Microcavity

Excitons in atomically thin transition-metal dichalcogenides (TMDs) have been established as an attractive platform to explore polaritonic physics, owing to their enormous binding energies and giant oscillator strength. Basic spectral features of exciton polaritons in TMD microcavities, thus far, were conventionally explained via two-coupled-oscillator models. This ignores, however, the impact of phonons on the polariton energy structure. Here we establish and quantify the threefold coupling between excitons, cavity photons, and phonons. For this purpose, we employ energy-momentum-resolved photoluminescence and spatially resolved coherent two-dimensional spectroscopy to investigate the spectral properties of a high-quality-factor microcavity with an embedded WSe_{2} van der Waals heterostructure at room temperature. Our approach reveals a rich multibranch structure which thus far has not been captured in previous experiments. Simulation of the data reveals hybridized exciton-photon-phonon states, providing new physical insight into the exciton polariton system based on layered TMDs.

Cavities with nonspherical mirrors for enhanced interaction between a quantum emitter and cavity photons

We propose a procedure for the significant enhancement of the strong-coupling rate between photons in an optical cavity and a single quantum emitter, such as an atom, quantum dot, or trapped ion. We show that specially designed, nonspherical mirrors can lead to cavity eigenmodes that exhibit a large field enhancement at the center of the cavity while inducing significantly less beam divergence and therefore smaller round trip losses and higher cooperativity than can be achieved by operating a spherical-mirror cavity in the near-concentric regime. We verify our designs using mode matching theory and discuss their robustness relative to different kinds of manufacturing deviations.

Open Quantum System Simulation of Faraday's Induction Law via Dynamical Instabilities.

We propose a novel type of a Bose-Hubbard ladder model based on an open quantum-gas-cavity-QED setup to study the physics of dynamical gauge potentials. Atomic tunneling along opposite directions in the two legs of the ladder is mediated by photon scattering from transverse pump lasers to two distinct cavity modes. The resulting interplay between cavity photon dissipation and the optomechanical atomic backaction then induces an average-density-dependent dynamical gauge field. The dissipation-stabilized steady-state atomic motion along the legs of the ladder leads either to a pure chiral current, screening the induced dynamical magnetic field as in the Meissner effect, or generates simultaneously chiral and particle currents. For a sufficiently strong pump the system enters into a dynamically unstable regime exhibiting limit-cycle and period-doubled oscillations. Intriguingly, an electromotive force is induced in this dynamical regime as expected from an interpretation based on Faraday's law of induction for the time-dependent synthetic magnetic flux.

Many-body localization regime for cavity-induced long-range interacting models

Many-body localization (MBL) features are studied here for a large spin chain model with long range interactions. The model corresponds to cold atoms placed inside a cavity and driven by an external laser field with long range interactions coming from rescattering of cavity photons. Earlier studies were limited to small sizes amenable to exact diagonalization. It is shown that nonergodic features and MBL may exist in this model for random disorder as well as in the presence of tilted potential on experimental time scales also for experimentally relevant system sizes using tensor networks algorithms.

Negative Gilbert damping

Modern ferromagnetism theory is based on the Landau-Lifshitz-Gilbert equation that governs the dynamics of magnetic moment in a ferromagnet. As a deep-rooted notion, the Gilbert damping parameter must be positive because it describes the (energy and angular momentum) dissipation. In this paper, we report a negative Gilbert damping via the magneto-optical interaction of three orthogonal circularly-polarized laser beams with a submicron magnet placed in an optical cavity. We show that the off-resonant coupling between the driving laser and cavity photon in the far-blue detuning can induce a magnetic torque exactly of the Gilbert type with negative damping coefficient. A hyperbolic-tangent function ansatz is found to well describe the time-resolved spin switching as the intrinsic dissipation is overcome. Feasible experiments and materials are discussed to test our theory.

Front Cover: Characterization of a Triple Quantum Dot via an On‐chip Microwave Resonator (Adv. Quantum Technol. 2/2022)

Circuit quantum electrodynamics architecture provides a controllable artificial system and enriches the physics with the participation of electron-photon interaction. The cover shows this hybrid architecture comprised of a superconducting microwave resonator and a triple quantum dot. In article number 2100104, Si-Si Gu and colleagues investigate quantum cellular automata and “photon-assisted” quadruple point phenomena in this system, which involve the Coulomb interaction among multiple dots and the simultaneously-tunneling processes assisted with cavity photons. These results suggest that this hybrid system has the potential for studying exotic many-body effects and electron-photon interaction.

Rabi-like splitting and refractive index sensing with hybrid Tamm plasmon-cavity modes

Rabi-like splitting and self-referenced refractive index sensing in hybrid plasmonic-1D photonic crystal structures have been theoretically demonstrated. The coupling between Tamm plasmon and cavity photon modes are tuned by incorporating a low refractive index spacer layer adjacent to the metallic layer to form their hybrid modes. Anticrossing of the modes observed at different values of spacer layer thickness validates the strong coupling between the two modes and causes Rabi-like splitting with different splitting energy. The modes coupling has been supported by coupled mode theory. Rabi-like splitting energy decreases with increasing number of periods (N) and refractive index contrast (η) of two dielectric materials used to make the 1D photonic crystals, and the observed variation is explained by an analytical model. Angular and polarization dependency of the hybrid modes shows that the polarization splitting of the lower hybrid mode is much stronger than that of the upper hybrid mode. On further investigation, it is seen that one of the hybrid modes remains unchanged while other mode undergoes significant change with varying the cavity medium. This nature of the hybrid modes has been utilized for designing self-referenced refractive index sensors for sensing different analytes. For η= 1.333 and N= 10 in a hybrid structure, the sensitivity increases from 51 to 201 nm RIU−1 with increasing cavity thickness from 170 to 892 nm. For the fixed cavity thickness of 892 nm, the sensitivity increases from 201 to 259 nm RIU−1 by increasing η from 1.333 to 1.605. The sensing parameters such as detection accuracy, quality factor, and figure of merit for two different hybrid structures [(η = 1.333, N = 10) and (η = 1.605, N = 6)] have been evaluated and compared. The value of resonant reflectivity of one of the hybrid modes changes considerably with varying analyte medium which can be used for refractive index sensing.