Abstract To obtain the mechanical mechanism of shear-type cavitation water jet dissociating flake graphite to improve the grinding technology of flake graphite, the motion state of flake graphite particles in shear-type cavitation water jet, the micro-jet impact process, the high-pressure elastic potential energy pressure release process, and the water wedge stretching process have been analyzed using the theory of hydraulic transport of liquid-solid two-phase, the theory of jets, the cavitation primordial principle, the principle of capacity conversion, and the water wedge action. The primary mechanical mechanism of shear cavitation water jet dissociation of flake graphite is collision friction effect, micro-jet impact, pressure release, and water wedge stretching effect, under these four kinds of loads individually or jointly, to achieve the purpose of removing the surface of flake graphite particles of the veinstone minerals to realize the dissociation of flake graphite. Moreover, the collision friction, pressure release, and water wedge stretching effects destroy the material under tensile stress to remove the veinstone minerals, and the micro-jet impact effect is the destruction of the material under compressive stress to remove the veinstone minerals.