CARIBU Facility Research Articles

The LSU-Argonne conversion electron spectrometer: A new detector for the X-Array and SATURN decay station

A new conversion electron detector has been commissioned at the ATLAS/ CARIBU facility at Argonne National Laboratory. The LSU-Argonne Conversion Electron Spectrometer (LACES) is a LN2-cooled Si(Li) detector system designed to be incorporated into a decay station that comprises the dedicated HPGe clover array with a box geometry (X-Array) and the Scintillator and Tape Using Radioactive Nuclei (SATURN) device. This integration enables simultaneous measurements of conversion electrons and gamma-rays in decay experiments, yielding novel information on transition multipolarities, electric monopole transitions, and isomeric states that decay mostly via conversion electrons. A measurement of the energy resolution of LACES yielded 2.3-keV FWHM at 975 keV for electrons and 1.3-keV FWHM at 75 keV for X-rays. A detailed study of the absolute detection efficiency (at 5 mm from the source) was performed, where this quantity was determined experimentally in the range of electron transition energies between 25.5 keV and 1047.8 keV and subsequently simulated using the GEANT4 code. Measurement and simulations are found to be in excellent agreement. A precise characterization, for this type of detector system, of the absolute detection efficiency for such a wide energy range is reported for the first time.

Searching for the origin of the rare-earth peak with precision mass measurements across Ce–Eu isotopic chains

A nuclear mass survey of rare-earth isotopes has been conducted with the Canadian Penning Trap mass spectrometer using the most neutron-rich nuclei thus far extracted from the CARIBU facility. We present a collection of 12 nuclear masses determined with a precision of $\ensuremath{\le}10$ keV/$c{}^{2}$ for $Z=58--63$ nuclei near $N=100$. Independently, a detailed study exploring the role of nuclear masses in the formation of the $r$-process rare-earth abundance peak has been performed. Employing a Markov chain Monte Carlo (MCMC) technique, mass predictions of lanthanide isotopes have been made which uniquely reproduce the observed solar abundances near $A=164$ under three distinct astrophysical outflow conditions. We demonstrate that the mass surface trends thus far mapped out by our measurements are most consistent with MCMC mass predictions given an $r$ process that forms the rare-earth peak during an extended $(n,\ensuremath{\gamma})\ensuremath{\rightleftarrows}(\ensuremath{\gamma},n)$ equilibrium.

A High-Resolution Study of the 110Tc → 110Ru → 110Rh → 110Pd Decay Chain with the GRETINA Array

Spectroscopic data, such as precise γ-ray branching and E2/M1 multipole-mixing ratios, provide vital constraints when performing multi-dimensional Coulomb-excitation analyses. Consequently, as part of our new Coulomb-excitation campaign aimed at investigating the role of exotic non-axial (triaxial) deformations in the unstable refractory Ru-Mo isotopes, additional beta-decay data was obtained. These measurements make use of ANL’s CARIBU facility, which provides intense beams of radioactive refractory isotopes along with the excellent efficiency and angular resolution of the GRETINA γ-ray tracking array. In this article, we report on the analysis of the A = 110 decay chain, focussing on the identification of previously unreported states in 110Ru following the decay of 110Tc.

Charge breeding at GANIL: Improvements, results, and comparison with the other facilities

The 1+/n+ method, based on an ECRIS charge breeder (CB) originally developed at the LPSC laboratory, is now implemented at GANIL for the production of Radioactive Ion Beams (RIBs). Prior to its installation in the middle of the low energy beam line of the SPIRAL1 facility, the 1+/n+ system CB has been modified based on the experiments performed on the CARIBU Facility at Argone National Laboratory. Later, it has been tested at the 1+/n+ LPSC test bench to validate its operation performances. Charge breeding efficiencies as well as charge breeding times have been measured for noble gases and alkali elements. The commissioning phase started at GANIL in the second half-year of 2017. It consisted of a stepwise process to test the upgrade of the SPIRAL1 facility from simple validation [operation of Charge Breeder (CB) as a stand-alone source] up to the production of the first 1+/n+ RIB. Thus, this year, a 38mK/38K RIB has been successfully delivered to a physics experiment over a period of 1 week. The yields on the physics target were in the range of ∼2-4 × 106 pps at 9 MeV/u. The target ion source system (TISS) was made of a FEBIAD ion source connected to a hot graphite target. This is the first time a RIB is accelerated with a cyclotron with the 1+/n+ method. Moreover, a production test with the FEBIAD TISS has confirmed the yields measured previously, which validates the extension of the GANIL/SPIRAL1 catalog for a number of isotopes. In parallel, R&D is being performed on new TISSs (e.g., a fast release one, using surface ionization source). Targets are also a subject of ongoing R&D for yield and release time optimization. This contribution will present the new acceleration scheme of the SPIRAL1 facility, which largely extends the palette of RIBs available for nuclear physicists. It will be compared to the ones used at similar ISOL facilities. This facility is more than a simple ISOL facility, and an overview of the new opportunities offered by the upgraded installation will be also discussed.

β -decay half-lives of Sb134,134m and their isomeric yield ratio produced by the spontaneous fission of Cf252

A number of fission products possess isomeric states which have a nuclear spin significantly different from that of the ground state. The yield ratio of these states following fission is influenced by the angular momentum present in the fissioning system. The $^{134m,134}\mathrm{Sb}$ yield ratio had not been previously measured in the spontaneous fission of $^{252}\mathrm{Cf}$; however, it had previously been observed to favor the (${7}^{\ensuremath{-}}$) isomer over the (${0}^{\ensuremath{-}}$) ground state in $^{235}\mathrm{U}({n}_{th},f$) and $^{232}\mathrm{Th}$(25 MeV $p,f$). Using a mass-separated beam of low-energy $^{134,134m}\mathrm{Sb}$ ions produced by $^{252}\mathrm{Cf}$ spontaneous fission at the CARIBU facility, $\ensuremath{\beta}$ particles and $\ensuremath{\gamma}$ rays were detected using the SATURN/X-Array decay station to determine the fission-yield ratio and $\ensuremath{\beta}$-decay half-lives. The $^{134m}\mathrm{Sb}$ to $^{134}\mathrm{Sb}$ fission yield was determined to be $2.03\ifmmode\pm\else\textpm\fi{}0.05$ and the half-lives of $^{134m}\mathrm{Sb}$ and $^{134}\mathrm{Sb}$ were found to be $9.87\ifmmode\pm\else\textpm\fi{}0.08$ s and $0.674\ifmmode\pm\else\textpm\fi{}0.004$ s, respectively. These results represent the first isomeric yield ratio measurement for this nucleus, and improved measurements of the $^{134}\mathrm{Sb}$ ground state and the $^{134m}\mathrm{Sb}$ isomer half-lives.

Erratum: "Charge breeding of radioactive isotopes at the CARIBU facility with an electron beam ion source" [Rev. Sci. Instrum. 89, 052402 (2018)

First Page

New ion source dramatically improves radioactive beams for CARIBU facility

A new Electron Beam Ion Source Charge Breeder operated with the CARIBU and ATLAS facilities dramatically reduces background contamination in radioactive beams, improving abilities of neutron-rich nuclei.

Charge breeding of radioactive isotopes at the CARIBU facility with an electron beam ion source.

An Electron Beam Ion Source Charge Breeder (EBIS-CB) has been developed at Argonne National Laboratory as part of the californium rare ion breeder upgrade. For the past year, the EBIS-CB has been undergoing commissioning as part of the ATLAS accelerator complex. It has delivered both stable and radioactive beams with A/Q < 6, breeding times <30 ms, low background contamination, and charge breeding efficiencies >18% into a single charge state. The operation of this device, challenges during the commissioning phase, and future improvements will be discussed.

Triaxiality near the 110Ru ground state from Coulomb excitation

A multi-step Coulomb excitation measurement with the GRETINA and CHICO2 detector arrays was carried out with a 430-MeV beam of the neutron-rich 110Ru (t1/2=12s) isotope produced at the CARIBU facility. This represents the first successful measurement following the post-acceleration of an unstable isotope of a refractory element. The reduced transition probabilities obtained for levels near the ground state provide strong evidence for a triaxial shape; a conclusion confirmed by comparisons with the results of beyond-mean-field and triaxial rotor model calculations.

γ-softBa146and the role of nonaxial shapes atN≈90

Low-spin states in the neutron-rich, N = 90 nuclide $^{146}$Ba were populated following $\beta$-decay of $^{146}$Cs, with the goal of clarifying the development of deformation in Ba isotopes through delineation of their non-yrast structures. Fission fragments of $^{146}$Cs were extracted from a 1.7-Ci $^{252}$Cf source and mass-selected using the CARIBU facility. Low-energy ions were deposited at the center of a box of thin $\beta$ detectors, surrounded by a high-efficiency HPGe array. The new $^{146}$Ba decay scheme now contains 31 excited levels extending up to ~2.5 MeV excitation energy, double what was previously known. These data are compared to predictions from the Interacting Boson Approximation (IBA) model. It appears that the abrupt shape change found at N = 90 in Sm and Gd is much more gradual in Ba and Ce, due to an enhanced role of the $\gamma$ degree of freedom.

First operation and mass separation with the CARIBU MR-TOF

The recent installation of a Multi-Reflection Time-of-Flight (MR-TOF) isobar separator at the CARIBU facility has the promising potential to significantly improve the mass separation and selection of short-lived neutron-rich beams. Ions cycled in the km-long isochronous trajectories between two electrostatic mirrors can be separated to high levels of mass-resolving power within a short time (tens of ms). The installation process is described and results from the first operation are discussed. Following an optimization of the mirror voltages a mass-resolving power of 6.8·104 was achieved and a separation of isobars was demonstrated. The higher purity beams provided by the MR-TOF and delivered to the Canadian Penning Trap (CPT) will provide access to further measurements of neutron-rich nuclei along the astrophysical r-process path.

Astrophysics experiments with radioactive beams at ATLAS

Reactions involving short-lived nuclei play an important role in nuclear astrophysics, especially in explosive scenarios which occur in novae, supernovae or X-ray bursts. This article describes the nuclear astrophysics program with radioactive ion beams at the ATLAS accelerator at Argonne National Laboratory. The CARIBU facility as well as recent improvements for the in-flight technique are discussed. New detectors which are important for studies of the rapid proton or the rapid neutron-capture processes are described. At the end we briefly mention plans for future upgrades to enhance the intensity, purity and the range of in-flight and CARIBU beams.

Recent results from HELIOS

Transfer and inelastic scattering reactions using light-ion beams and stable or long-lived targets have traditionally provided detailed information on the structure of nuclei near the line of beta stability. Such studies can now be extended to nuclei away from the line of β -stability as radioactive beams are becoming available at a number of facilities around the world, including the CARIBU facility at Argonne. These measurements must, however, be carried out in inverse kinematics, resulting in a loss of the effective experimental resolution when conventional detection schemes are employed. The HELIOS spectrometer is based on a new concept, that is especially well suited for such studies by reducing the resolution problem, providing simple particle identification, and giving high detection efficiency with moderate Si detector area. In this talk, the HELIOS concept and results from the first series of experiments will be presented.

Radioactive beams from gas catchers: The CARIBU facility

Gas catchers allow the transformation of radioactive recoils from various sources into a good optical quality low-energy radioactive beam that is then available for experiments at low-energy or for further acceleration. The CARIBU project uses such a large gas catcher to create beams of neutron-rich isotopes from a Californium source for post-acceleration through the ATLAS superconducting linac to open new research opportunities for nuclear structure physics and astrophysics. The RF gas catcher developed at Argonne has now demonstrated operation at the high intensity required for this application.