Boundary Layer Clouds Research Articles

Distinctive aerosol–cloud–precipitation interactions in marine boundary layer clouds from the ACE-ENA and SOCRATES aircraft field campaigns

Abstract. The aerosol–cloud–precipitation interactions within the cloud-topped marine boundary layer (MBL) are examined using aircraft in situ measurements from Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) and Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) field campaigns. SOCRATES clouds exhibit a larger number concentration and smaller cloud droplet effective radius (148.3 cm−3 and 8.0 µm) compared to ACE-ENA summertime (89.4 cm−3 and 9.0 µm) and wintertime clouds (70.6 cm−3 and 9.8 µm). The ACE-ENA clouds, especially during the winter, feature stronger drizzle formation via droplet growth through enhanced collision–coalescence that is attributed to a relatively cleaner environment and deeper cloud layer. Furthermore, the aerosol–cloud interaction (ACI) indices from the two aircraft field campaigns exhibit distinct sensitivities, indicating different cloud microphysical responses to aerosols. The ACE-ENA winter season features relatively fewer aerosols, which are more likely activated into cloud droplets under the conditions of sufficient water vapor availability and strong turbulence. The enriched aerosol loading during ACE-ENA summer and SOCRATES generally leads to smaller cloud droplets competing for the limited water vapor and exhibiting a stronger ACI. Notably, the precipitation susceptibilities are stronger during the ACE-ENA than during the SOCRATES campaigns. The in-cloud drizzle behavior significantly alters sub-cloud cloud condensation nuclei (CCN) budgets through the coalescence-scavenging effect and, in turn, impacts the ACI assessments. The results of this study can enhance understanding and aid in future model simulation and assessment of the aerosol–cloud interaction.

Deep-learning-driven simulations of boundary layer clouds over the Southern Great Plains

Abstract. Based on long-term observations at the Southern Great Plains site by the Atmospheric Radiation Measurement (ARM) program for training and validation, a deep-learning model is developed to simulate the daytime evolution of boundary layer clouds (BLCs) from the perspective of land–atmosphere coupling. The model takes ARM measurements (including early-morning soundings and diurnally varying surface meteorological conditions and heat fluxes) as inputs and predicts hourly estimates (including cloud occurrence, the positions of cloud boundaries, and the vertical profile of the cloud fraction) as outputs. The deep-learning model offers good agreement with the observed cloud fields, especially in the accuracy with which cloud occurrence and base height are reproduced. When the inputs are substituted by reanalysis data from ERA5 and MERRA-2, the outputs of the deep-learning model provide a better agreement with observation than the cloud fields extracted from ERA5 and MERRA-2 themselves. Thus, the deep-learning model shows great potential to serve as a diagnostic tool for the performance of physics-based models in simulating stratiform and cumulus clouds. By quantifying biases in clouds and attributing them to the simulated atmospheric state variables versus the model-parameterized cloud processes, this observation-based deep-learning model may offer insights into the directions needed to improve the simulation of BLCs in physics-based models for weather forecasting and climate prediction.

Corrigendum: Towards reliable retrievals of cloud droplet number for non-precipitating planetary boundary layer clouds and their susceptibility to aerosol

Corrigendum: Towards reliable retrievals of cloud droplet number for non-precipitating planetary boundary layer clouds and their susceptibility to aerosol

Airborne measurements of mesoscale divergence at high latitudes during HALO-(AC)3

Abstract Boundary layer cloud transformations at high latitudes play a key role for the Arctic climate and are partially controlled by large-scale dynamics such as subsidence. While measuring large- and mesoscale divergence on spatial scales on the order of 100 km has proven notoriously difficult, recent airborne campaigns in the subtropics have successfully applied measurement techniques using multiple dropsonde releases in circular flight patterns. In this paper it is shown that this method can also be effectively applied at high latitudes, in spite of the considerable differences in atmospheric dynamics compared to the subtropics. To show the applicability, data collected during the airborne HALO-(AC)3 field campaign near Svalbard in Spring 2022 were analysed, where several flight patterns involving multiple dropsonde launches were realized by two aircraft. This study presents a first overview of the results. We find that the method indeed yields reliable estimates of mesoscale gradients in the Arctic, producing robust vertical profiles of horizontal divergence and consequently, subsidence. Sensitivity to aspects of the method is investigated, including dependence on sampling area and the divergence calculation.

How Well Does the DOE Global Storm Resolving Model Simulate Clouds and Precipitation Over the Amazon?

AbstractThis study assesses a 40‐day 3.25‐km global simulation of the Simple Cloud‐Resolving E3SM Model (SCREAMv0) using high‐resolution ground‐based observations from the Atmospheric Radiation Measurement (ARM) Green Ocean Amazon (GoAmazon) field campaign. SCREAMv0 reasonably captures the diurnal timing of boundary layer clouds yet underestimates the boundary layer cloud fraction and mid‐level congestus. SCREAMv0 well replicates the precipitation diurnal cycle, however it exhibits biases in the precipitation cluster size distribution compared to scanning radar observations. Specifically, SCREAMv0 overproduces clusters smaller than 128 km, and does not form enough large clusters. Such biases suggest an inhibition of convective upscale growth, preventing isolated deep convective clusters from evolving into larger mesoscale systems. This model bias is partially attributed to the misrepresentation of land‐atmosphere coupling. This study highlights the potential use of high‐resolution ground‐based observations to diagnose convective processes in global storm resolving model simulations, identify key model deficiencies, and guide future process‐oriented model sensitivity tests and detailed analyses.

Aitken Mode Aerosols Buffer Decoupled Mid‐Latitude Boundary Layer Clouds Against Precipitation Depletion

AbstractAerosol‐cloud‐precipitation interactions are a leading source of uncertainty in estimating climate sensitivity. Remote marine boundary layers where accumulation mode (∼100–400 nm diameter) aerosol concentrations are relatively low are very susceptible to aerosol changes. These regions also experience heightened Aitken mode aerosol (∼10–100 nm) concentrations associated with ocean biology. Aitken aerosols may significantly influence cloud properties and evolution by replenishing cloud condensation nuclei and droplet number lost through precipitation (i.e., Aitken buffering). We use a large‐eddy simulation with an Aitken‐mode enabled microphysics scheme to examine the role of Aitken buffering in a mid‐latitude decoupled boundary layer cloud regime observed on 15 July 2017 during the Aerosol and Cloud Experiments in the Eastern North Atlantic flight campaign: cumulus rising into stratocumulus under elevated Aitken concentrations (∼100–200 mg−1). In situ measurements are used to constrain and evaluate this case study. Our simulation accurately captures observed aerosol‐cloud‐precipitation interactions and reveals time‐evolving processes driving regime development and evolution. Aitken activation into the accumulation mode in the cumulus layer provides a reservoir for turbulence and convection to carry accumulation aerosols into the drizzling stratocumulus layer above. Further Aitken activation occurs aloft in the stratocumulus layer. Together, these activation events buffer this cloud regime against precipitation removal, reducing cloud break‐up and associated increases in heterogeneity. We examine cloud evolution sensitivity to initial aerosol conditions. With halved accumulation number, Aitken aerosols restore accumulation concentrations, maintain droplet number similar to original values, and prevent cloud break‐up. Without Aitken aerosols, precipitation‐driven cloud break‐up occurs rapidly. In this regime, Aitken buffering sustains brighter, more homogeneous clouds for longer.

The Association Between Cloud Droplet Number over the Summer Southern Ocean and Air Mass History

AbstractThe cloud properties and governing processes in Southern Ocean marine boundary layer clouds have emerged as a central issue in understanding the Earth's climate sensitivity. While our understanding of Southern Ocean cloud feedbacks have evolved in the most recent climate model intercomparison, the background properties of simulated summertime clouds in the Southern Ocean are not consistent with measurements due to known biases in simulating cloud condensation nuclei concentrations. This paper presents several case studies collected during the Capricorn 2 and Marcus campaigns held aboard Australian research vessels in the Austral Summer of 2018. Combining the surface‐observed cases with MODIS data along forward and backward air mass trajectories, we demonstrate the evolution of cloud properties with time. These cases are consistent with multi‐year statistics showing that long trajectories of air masses over the Antarctic ice sheet are critical to creating high droplet number clouds in the high latitude summer Southern Ocean. We speculate that secondary aerosol production via the oxidation of biogenically derived aerosol precursor gasses over the high actinic flux region of the high latitude ice sheets is fundamental to maintaining relatively high droplet numbers in Southern Ocean clouds during Summer.

Long‐Term Trends in Aerosols, Low Clouds, and Large‐Scale Meteorology Over the Western North Atlantic From 2003 to 2020

AbstractA continuous decrease in aerosols over the Western North Atlantic Ocean (WNAO) on a decadal timescale provides a long‐term benchmark to evaluate how various natural and anthropogenic processes affect the manifestation of aerosol‐cloud interactions in this region. Furthermore, the WNAO serves as a natural laboratory with diverse aerosol sources, marine boundary layer clouds more variable than those in marine stratocumulus deck regions, and unique flow regimes established by the Gulf Stream and the semi‐permanent Bermuda High. We investigate how satellite‐retrieved macrophysical and microphysical properties of low clouds and the surface shortwave irradiance changed from 2003 to 2020, in tandem with this aerosol decrease. The decadal changes in large‐scale meteorology related to the North Atlantic Oscillation (NAO) are also examined. We find a reduction in low‐cloud optical thickness, accompanied by fewer and larger cloud droplets, yet observe no significant changes in low‐cloud fraction and liquid water path. Despite the reduction in low‐cloud optical thickness together with aerosol decrease, a corresponding increase in the trends of surface shortwave irradiance, also known as surface brightening, is lacking. This absence of brightening is potentially related to concomitant changes found in large‐scale meteorology associated with NAO—Bermuda High strengthening, sea surface warming, and atmospheric moistening— as well as an increase in high‐level cloud fraction that can counteract the surface brightening. Ultimately, our findings suggest that spatial patterns of decadal meteorological variability introduce complexities in the surface cloud radiative effect over the WNAO, thereby complicating the isolation and examination of aerosol‐cloud interactions.

Cloud Properties and Boundary Layer Stability Above Southern Ocean Sea Ice and Coastal Antarctica

AbstractSignificant variability in climate predictions originates from the simulated cloud cover over the Southern Ocean. Historically, Southern Ocean cloud and aerosol properties have been less studied than their northern hemisphere counterparts, and cloud‐sea‐ice interactions over the Southern Ocean also remain largely unexamined. We used data from combined radar, lidar, radiometer, radiosonde, and ERA5 reanalysis profiles to investigate cloud property relationships to cloud temperature, sea‐ice concentration, and boundary layer stability. Our findings show correlations between both cloud macrophysical properties and radiative effects and sea‐ice concentration, and that the marine atmospheric boundary layer is more stable over higher sea‐ice concentrations. Mixed‐phase cloud frequency of occurrence was highest over the sea‐ice zone at 15%, three times higher than over cold water south of the Antarctic Polar Front. For temperatures greater than −15°C, low‐level, single‐layer clouds were more likely to precipitate ice if they were coupled to cold‐water or sea‐ice surfaces than if they were decoupled from these surfaces, with the highest percentage of clouds precipitating ice observed over sea ice. These findings suggest a surface source of ice‐nucleating particles at high southern latitudes that increases cloud glaciation probability. We discuss the implications of our results for future studies into the relationship between cloud properties, aerosols, sea ice, and boundary layer stability at high latitudes over the Southern Ocean.

Assessing CESM2 Clouds and Their Response to Climate Change Using Cloud Regimes

Abstract The Community Earth System Model, version 2 (CESM2), has a very high climate sensitivity driven by strong positive cloud feedbacks. To evaluate the simulated clouds in the present climate and characterize their response with climate warming, a clustering approach is applied to three independent satellite cloud products and a set of coupled climate simulations. Using k-means clustering with a Wasserstein distance cost function, a set of typical cloud configurations is derived for the satellite cloud products. Using satellite simulator output, the model clouds are classified into the observed cloud regimes in both current and future climates. The model qualitatively reproduces the observed cloud configurations in the historical simulation using the same time period as the satellite observations, but it struggles to capture the observed heterogeneity of clouds which leads to an overestimation of the frequency of a few preferred cloud regimes. This problem is especially apparent for boundary layer clouds. Those low-level cloud regimes also account for much of the climate response in the late twenty-first century in four shared socioeconomic pathway simulations. The model reduces the frequency of occurrence of these low-cloud regimes, especially in tropical regions under large-scale subsidence, in favor of regimes that have weaker cloud radiative effects.

Using Satellite and ARM Observations to Evaluate Cold Air Outbreak Cloud Transitions in E3SM Global Storm‐Resolving Simulations

AbstractThis study examines marine boundary layer cloud regime transition during a cold air outbreak (CAO) over the Norwegian Sea, simulated by a global storm‐resolving model (GSRM) known as the Simple Cloud‐Resolving Energy Exascale Earth System Model Atmosphere Model (SCREAM). By selecting observational references based on a combination of large‐scale conditions rather than strict time‐matched comparisons, this study finds that SCREAM qualitatively captures the CAO cloud transition, including boundary layer growth, cloud mesoscale structure, and phase partitioning. SCREAM also accurately locates the greatest ice and liquid in the mesoscale updrafts, however, underestimates supercooled liquid water in cumulus clouds. The model evaluation approach adopted by this study takes advantages of the existing computational‐expensive global simulations of GSRM and the available observations to understand model performance and can be applied to assessments of other cloud regimes in different regions. Such practice provides valuable guidance on the future effort to correct and improve biased model behaviors.

Observation and Reanalysis Derived Relationships Between Cloud and Land Surface Fluxes Across Cumulus and Stratiform Coupling Over the Southern Great Plains

AbstractUnderstanding interactions between low clouds and land surface fluxes is critical to comprehending Earth's energy balance, yet their relationships remain elusive, with discrepancies between observations and modeling. Leveraging long‐term field observations over the Southern Great Plains, this investigation revealed that cloud‐land interactions are closely connected to cloud‐land coupling regimes. Observational evidence supports a dual‐mode interaction: coupled stratiform clouds predominate in low sensible heat scenarios, while coupled cumulus clouds dominate in high sensible heat scenarios. Reanalysis data sets, MERRA‐2 and ERA‐5, obscure this dichotomy owing to a shortfall in representing boundary layer clouds, especially in capturing the initiation of coupled cumulus in high sensible heat scenarios. ERA‐5 demonstrates a relatively closer alignment with observational data, particularly in capturing relationships between cloud frequency and latent heat, markedly outperforming MERRA‐2. Our study underscores the necessity of distinguishing different cloud coupling regimes, essential to the understanding of their interactions for advancing land‐atmosphere interactions.

Assessing Radiative Impacts of African Smoke Aerosols Over the Southeastern Atlantic Ocean

AbstractBiomass burning smoke aerosols are efficient at attenuating incoming solar radiation. The Layered Atlantic Smoke Interactions with Clouds campaign was conducted from June 2016 to October 2017. The U. S. Department of Energy mobile Atmospheric Radiation Measurement site located on Ascension Island (AMF‐ASI) identified several instances of smoke plume intrusions. Increases in surface and column measurements of aerosol loading were directly related to increases in fine mode fraction, number concentrations of aerosols (Na), and cloud condensation nuclei (NCCN). During periods of weak lower tropospheric stability, smoke particles were more likely to be advected downward either by boundary layer turbulence or cloud top entrainment under non‐overcast sky conditions. Backward trajectory analysis illustrated that smoke aerosols reaching the AMF‐ASI site were fine mode, less aged, strongly absorbing, and had shorter boundary layer trajectories while longer boundary layer trajectories denoted mixtures of weakly absorbing smoke and coarse mode marine aerosols. The most polluted smoke cases of August 2016 and 2017 revealed a notable contrast in radiative forcing per unit aerosol optical depth or radiative forcing efficiency (ΔFeff) at the top of the atmosphere (TOA) and near‐surface (BOA). The weakly (strongly) absorbing 2016 cases exhibited weaker (stronger) ΔFeff at the TOA and BOA suggesting a warming (cooling) effect within the boundary layer. The 2017 cases featured the strongest ΔFeff suggesting more of a cooling effect at the TOA and BOA due to mixing of fresh smoke with marine aerosols during transport.

Daytime variation in the aerosol indirect effect for warm marine boundary layer clouds in the eastern North Atlantic

Abstract. Warm boundary layer clouds in the eastern North Atlantic region exhibit significant diurnal variations in cloud properties. However, the diurnal cycle of the aerosol indirect effect (AIE) for these clouds remains poorly understood. This study takes advantage of recent advancements in the spatial resolution of geostationary satellites to explore the daytime variation in the AIE by estimating the cloud susceptibilities to changes in cloud droplet number concentration (Nd). Cloud retrievals for the month of July over 4 years (2018–2021) from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) on Meteosat-11 over this region are analyzed. Our results reveal a significant “U-shaped” daytime cycle in susceptibilities of the cloud liquid water path (LWP), cloud albedo, and cloud fraction. Clouds are found to be more susceptible to Nd perturbations at noon and less susceptible in the morning and evening. The magnitude and sign of cloud susceptibilities depend heavily on the cloud state defined by cloud LWP and precipitation conditions. Non-precipitating thin clouds account for 44 % of all warm boundary layer clouds in July, and they contribute the most to the observed daytime variation. Non-precipitating thick clouds are the least frequent cloud state (10 %), and they exhibit more negative LWP and albedo susceptibilities compared to thin clouds. Precipitating clouds are the dominant cloud state (46 %), but their cloud susceptibilities show minimal variation throughout the day. We find evidence that the daytime variation in LWP and albedo susceptibilities for non-precipitating clouds is influenced by a combination of the diurnal transition between non-precipitating thick and thin clouds and the “lagged” cloud responses to Nd perturbations. The daytime variation in cloud fraction susceptibility for non-precipitating thick clouds can be attributed to the daytime variation in cloud morphology (e.g., overcast or broken). The dissipation and development of clouds do not adequately explain the observed variation in cloud susceptibilities. Additionally, daytime variation in cloud susceptibility is primarily driven by variation in the intensity of cloud response rather than the frequency of occurrence of cloud states. Our results imply that polar-orbiting satellites with an overpass time at 13:30 LT underestimate daytime mean values of cloud susceptibility, as they observe susceptibility daily minima in the study region.

Marine-cloud brightening: an airborne concept

Marine Cloud Brightening (MCB) is a proposed Solar Radiation Modification (SRM) geoengineering technique to enhance Marine Boundary Layer (MBL) cloud albedo. Extant proposals consider 104 − 105 autonomous ships spraying seawater, generating and dispersing sea salt nanoparticles. Alternatively, this paper proposes industrially manufacturing NaCl nanoparticles using ethanol anti-solvent brine precipitation. With desiccation, size optimization and narrowed size distribution, aerosol mass flux reduces by ∼500× (17× for dry mass flux). This facilitates Unmanned Aerial Vehicle delivery (e.g. MQ-9 Reaper Unmanned Aerial Vehicle). Increased speed and wake turbulence improves areal coverage per vehicle versus ships—reducing fleet size. Utilizing extant airframe designs improves vehicle Technology Readiness Level (TRL)—potentially improving system operational cost (est. $40B · yr −1) and lead time. This approach further reduces energy requirements (5× less), technical risk and system complexity. Increased readiness amplifies proliferation risk—particularly for inexpensive regional heatwave and hurricane suppression—making governance more urgent.

Effects of vertical grid spacing on the climate simulated in the ICON-Sapphire global storm-resolving model

Abstract. Global storm-resolving models (GSRMs) use strongly refined horizontal grids compared with the climate models typically used in the Coupled Model Intercomparison Project (CMIP) but employ comparable vertical grid spacings. Here, we study how changes in the vertical grid spacing and adjustments to the integration time step affect the basic climate quantities simulated by the ICON-Sapphire atmospheric GSRM. Simulations are performed over a 45 d period for five different vertical grids with between 55 and 540 vertical layers and maximum tropospheric vertical grid spacings of between 800 and 50 m, respectively. The effects of changes in the vertical grid spacing are compared with the effects of reducing the horizontal grid spacing from 5 to 2.5 km. For most of the quantities considered, halving the vertical grid spacing has a smaller effect than halving the horizontal grid spacing, but it is not negligible. Each halving of the vertical grid spacing, along with the necessary reductions in time step length, increases cloud liquid water by about 7 %, compared with an approximate 16 % decrease for halving the horizontal grid spacing. The effect is due to both the vertical grid refinement and the time step reduction. There is no tendency toward convergence in the range of grid spacings tested here. The cloud ice amount also increases with a refinement in the vertical grid, but it is hardly affected by the time step length and does show a tendency to converge. While the effect on shortwave radiation is globally dominated by the altered reflection due to the change in the cloud liquid water content, the effect on longwave radiation is more difficult to interpret because changes in the cloud ice concentration and cloud fraction are anticorrelated in some regions. The simulations show that using a maximum tropospheric vertical grid spacing larger than 400 m would increase the truncation error strongly. Computing time investments in a further vertical grid refinement can affect the truncation errors of GSRMs similarly to comparable investments in horizontal refinement, because halving the vertical grid spacing is generally cheaper than halving the horizontal grid spacing. However, convergence of boundary layer cloud properties cannot be expected, even for the smallest maximum tropospheric grid spacing of 50 m used in this study.

Comparison of Forecasting Biases Over New York State Mesonet: A Wet Summer Versus a Dry Summer

AbstractExtreme weather events are occurring with increasing frequent due to the climate change. This increasing frequency may introduce more uncertainty in weather forecasting model performance, particularly when considering the intricate relationship of the land surface and atmosphere coupling system. In this study, we utilize data from the sophisticated New York State Mesonet to evaluate the performance of a forecasting system based on WRF Version 4 model, drawing insights from both dry and wet summers. Additionally, the model's performance is assessed on two land surface types: forest and farmland, to provide a comprehensive evaluation of impact of land surface heterogeneity. The surface meteorology, fluxes, and cloud development are assessed. The coupling between surface and atmosphere is diagnosed using a mixing diagram which serves to represent surface thermodynamic properties. The results reveal a systematic increase in warm season dry and warm biases, especially for forested sites during a drought year. The model exhibits heightened sensitivity to drought conditions, resulting in a substantial underestimation of latent heat fluxes during such period. During days with boundary layer clouds, the mixing diagram shows a notably slower growth of moist static energy in the model compared to observation. It is possible that these biases partly attribute to the underestimation of cloud optical depth due to not enough energy for the cloud development.

On the relationship between mesoscale cellular convection and meteorological forcing: comparing the Southern Ocean against the North Pacific

Abstract. Marine atmospheric boundary layer (MABL) clouds cover vast areas over the ocean and have important radiative effects on the Earth's climate system. These radiative effects are known to be sensitive to the local organization, or structure, of the mesoscale cellular convection (MCC). A convolutional neural network model is used to identify the two idealized classes of MCC clouds, namely open and closed, over the Southern Ocean (SO) and Northwest Pacific (NP) from high-frequency geostationary Himawari-8 satellite observations. The results of the climatology show that MCC clouds are evenly distributed over the mid-latitude storm tracks for both hemispheres, with peaks poleward of the 40∘ latitude. Open-MCC clouds are more prevalent than closed MCC in both regions. An examination of the presumed meteorological forcing associated with open- and closed-MCC clouds is conducted to illustrate the influence of large-scale meteorological conditions. We establish the importance of the Kuroshio western boundary current in the spatial coverage of open and closed MCC across the NP, presumably through the supply of strong heat and moisture fluxes during marine cold-air outbreaks events. In regions where static stability is higher, we observe a more frequent occurrence of closed MCCs. This behavior contrasts markedly with that of open MCCs, whose formation and persistence are significantly influenced by the difference in temperature between the air and the sea surface. The occurrence frequency of closed MCC over the SO exhibits a significant diurnal cycle, while the diurnal cycle of closed MCC over the NP is less noticeable.

New Particle Formation Events Can Reduce Cloud Droplets in Boundary Layer Clouds at the Continental Scale

AbstractNew particle formation (NPF) substantially contributes to global cloud condensation nuclei (CCN), and their climate impacts. Individual NPF events are also thought to increase local CCN, cloud droplet number (CDN), and cloud albedo. High resolution simulations however go against the latter, showing that radiatively important stratiform clouds can experience a systematic and substantial decrease in CDN during and after NPF events. CDN drops because particles too small to act as CCN uptake condensable material, and stunt the growth of particles that would otherwise form droplets. Convective clouds however experience modest increases in CDN—consistent with established views on the NPF‐cloud link. Together, these results reshape our conceptual understanding of NPF impacts on clouds, as the newly discovered duality of responses would drive cloud systems in a fundamentally different manner than thought.

Characterizing Ice Nucleating Particles Over the Southern Ocean Using Simultaneous Aircraft and Ship Observations

AbstractSupercooled liquid clouds are ubiquitous over the Southern Ocean (SO), even to temperatures below −20°C, and comprise a large fraction of the marine boundary layer (MBL) clouds. Earth system models and reanalysis products have struggled to reproduce the observed cloud phase distribution and occurrence of cloud ice in the region. Recent simulations found the microphysical representation of ice nucleation and growth has a large impact on these properties, however, measurements of SO ice nucleating particles (INPs) to validate simulations are sparse. This study presents measurements of INPs from simultaneous aircraft and ship campaigns conducted over the SO in austral summer 2018, which include the first in situ observations in and above cloud in the region. Our results confirm recent observations that INP concentrations are uniformly lower than measurements made in the late 1960s. While INP concentrations below and above cloud are similar, higher ice nucleation efficiency above cloud supports model simulations that the dominant INP composition varies with height. Model parameterizations based solely on aerosol properties capture the mean relationship between INP concentration and temperature but not the observed variability, which is likely related to the only modest correlations observed between INPs and environmental or aerosol metrics. Including wind speed in addition to activation temperature in a marine INP parameterization reduces bias but does not explain the large range of observed INP concentrations. Direct and indirect inference of marine INP size suggests MBL INPs, at least during Austral summer, are dominated by particles with diameters smaller than 500 nm.