Blockade Radius Research Articles

Ground state of Rydberg-dressed Bose gas confined in a toroidal trap

The experimental realization of Rydberg dressing technology in ultracold atomic systems provides another superior platform for studying novel states of matter and macroscopic quantum phenomena. In this work, based on the mean-field theory, we have investigated the ground-state phases of a two-component Bose–Einstein condensate with Rydberg interaction and confined in a toroidal trap. The effects of the Rydberg interaction and external potential, especially the Rydberg blockade radius, on the ground-state structure of such a system have been investigated in full parameter space. Our results show that the Rydberg blockade radius, which can be regarded as another controllable parameter, can be used to obtain a variety of ground-state phases. More interestingly, it is found that for weak Rydberg interactions, the Rydberg blockade radius breaks the spontaneous rotational symmetry of the system, leading to the formation of a discrete unit cell structure. For strongly interacting cases, it can be used to realize different orders of discrete rotational symmetry breaking.

Trimer quantum spin liquid in a honeycomb array of Rydberg atoms

Quantum spin liquids are elusive but paradigmatic examples of strongly correlated quantum states that are characterized by long-range quantum entanglement. Recently, signatures of a gapped topological Z2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${{\\mathbb{Z}}}_{2}$$\\end{document} spin liquid have been observed in a system of Rydberg atoms; however, the full capability of these platforms to realize quantum spin liquids extends far beyond this state alone. Here, we propose the realization of a different class of spin liquids in a honeycomb array of Rydberg atoms. Exploring the system’s quantum phase diagram using density-matrix renormalization group and exact diagonalization calculations, we identify several density-wave-ordered phases and a trimer spin liquid ground state with an emergent U(1) × U(1) local symmetry. This liquid state originates from superpositions of classical trimer configurations on the dual triangular lattice in the regime where third-nearest-neighbor atoms lie within the Rydberg blockade radius. Finally, we discuss the conditions to enhance the preparation fidelity of this state by a general Rydberg-blockade-based projection mechanism, test the robustness of the trimer spin liquid phase in a range of realistic parameters, and outline methods for its experimental detection.

Floquet-tailored Rydberg interactions

The Rydberg blockade is a key ingredient for entangling atoms in arrays. However, it requires atoms to be spaced well within the blockade radius, which limits the range of local quantum gates. Here we break this constraint using Floquet frequency modulation, with which we demonstrate Rydberg-blockade entanglement beyond the traditional blockade radius and show how the enlarged entanglement range improves qubit connectivity in a neutral atom array. Further, we find that the coherence of entangled states can be extended under Floquet frequency modulation. Finally, we realize Rydberg anti-blockade states for two sodium Rydberg atoms within the blockade radius. Such Rydberg anti-blockade states for atoms at close range enables the robust preparation of strongly-interacting, long-lived Rydberg states, yet their steady-state population cannot be achieved with only the conventional static drive. Our work transforms between the paradigmatic regimes of Rydberg blockade versus anti-blockade and paves the way for realizing more connected, coherent, and tunable neutral atom quantum processors with a single approach.

Rydberg-Rydberg interaction strengths and dipole blockade radii in the presence of Förster resonances.

Achieving a substantial blockade radius is crucial for developing scalable and efficient quantum communication and computation. In this theoretical study, we present the enhancement of the Rydberg blockade radius by utilizing Förster resonance. This phenomenon occurs when the energy difference between two initial Rydberg states closely matches that between the corresponding final Rydberg states, giving rise to a resonant energy transfer process. We employ quantum defect theory to numerically calculate the 87Rb-87Rb Rydberg atomic pair, enabling us to accurately estimate the van der Waals interaction. Our investigation reveals that when the principal quantum numbers of two Rydberg states differ only slightly, the Förster transition is rarely able to achieve a large blockade radius. However, in cases where the principal quantum numbers differ significantly, we substantially improve the Rydberg blockade radius. Most notably, we identify transition channels exhibiting an extensive blockade radius, surpassing 50 μm. This significant increase in the blockade radius enables larger-scale quantum operations and advances quantum technologies, with broad implications for achieving long-range quantum entanglement and robust quantum processes.

Neutral-atom entanglement using adiabatic Rydberg dressing

We revisit the implementation of a two-qubit entangling gate, the M\o{}lmer-S\o{}rensen gate, using the adiabatic Rydberg dressing paradigm for neutral atoms as studied in [A. Mitra et al., Phys. Rev. A 101, 030301(R) (2020)]. We study the implementation of rapid adiabatic passage using a two-photon transition, which does not require the use of an ultraviolet laser, and can be implemented using only amplitude modulation of one field with all laser frequencies fixed. We find that entangling gate fidelities, comparable to the one-photon excitation, are achievable with the two-photon excitation. Moreover, we address how the adiabatic dressing protocol can be used to implement entangling gates outside the regime of a perfect Rydberg blockade. We show that, by using adiabatic dressing, we can achieve scaling of the gate fidelity set by the fundamental limits to entanglement generated by the Rydberg interactions while simultaneously retaining a limited population in the doubly excited Rydberg state. This allows for fast high-fidelity gates for atoms separated beyond the blockade radius.

All-optical quantum information processing via a single-step Rydberg blockade gate.

One of the critical elements in the realization of the quantum internet are deterministic two-photon gates. This CZ photonic gate also completes a set of universal gates for all-optical quantum information processing. This article discusses an approach to realize a high fidelity CZ photonic gate by storing both control and target photons within an atomic ensemble using non-Rydberg electromagnetically induced transparency (EIT) followed by a fast, single-step Rydberg excitation with global lasers. The proposed scheme operates by relative intensity modulation of two lasers used in Rydberg excitation. Circumventing the conventional π-gap-π schemes, the proposed operation features continuous laser protection of the Rydberg atoms from the environment noise. The complete spatial overlap of stored photons inside the blockade radius optimizes the optical depth and simplifies the experiment. The coherent operation here is performed in the region that was dissipative in the previous Rydberg EIT schemes. Encountering the main imperfection sources, i.e., the spontaneous emission of the Rydberg and intermediate levels, population rotation errors, Doppler broadening of the transition lines, storage/retrieval efficiency, and atomic thermal motion induced decoherence, this article concludes that with realistic experimental parameters 99.7% fidelity is achievable.

Gauge theory description of Rydberg atom arrays with a tunable blockade radius

We discuss a Rydberg atom chain with a tunable blockade radius from the gauge theoretic perspective. When the blockade radius is one lattice spacing, this system can be formulated in terms of the PXP model, and there is a $\mathbb{Z}_2$ Ising phase transition known to be equivalent to a confinement-deconfinement transition in a gauge theory, the lattice Schwinger model. Further increasing the blockade radius, one can add a next-nearest neighbor (NNN) interaction into the PXP model. We discuss the interpretation of NNN interaction in terms of the gauge theory and how finite NNN interaction alters the deconfinement behavior and propose a corresponding experimental protocol. When the blockade radius reaches two lattice spacing, the model reduces to the PPXPP model. A novel gauge theory equivalent to the PPXPP model is formulated, and the phases in the two formulations are delineated. These results are readily explored experimentally in Rydberg quantum simulators.

A 509 nm pulsed laser system for Rydberg excitation of cesium atoms

<sec>Single photon source is a non-classical light field with anti-bunching effect, which has a potential applications in the research of fundamental physics problems, quantum precision measurement, quantum communication, quantum computing, etc. The strong interaction between highly excited Rydberg atoms presents an excitation blockade effect. In a dense Rydberg atomic ensemble, the excitation of more than one Rydberg atom within a blockade volume is suppressed, where the interactions of Rydberg atoms shift the atomic states out of resonance with an excitation laser.</sec><sec>We consider here the generation of single photon source by using a four-wave mixing scheme in a room-temperature atomic vapor cell. In a homemade micrometer-sized atomic vapor cell, one-dimensional size is smaller than the radius of Rydberg blockade and the other two-dimensional size is limited by the size of focused laser beam. The blockade radius is on the order of a few micrometers, depending on the Rydberg atom states. An excitation blockade effect can be used to realize single photon source in thermal cesium vapor microcells. The micron cesium-cell is used to spatially localize atomic groups, which results in the atomic decoherence time on the order of microseconds or even nanoseconds. This requires a high-power pulsed laser to prepare the Rydberg atomic state at a nanosecond scale.</sec><sec>Four-photon excitation schemes with narrow linewidth lasers are also used experimentally. The cesium-Rydberg state can usually be excited by the lasers with optical wavelengths 852 and 509 nm, respectively. The laser system is well-stabilized so that the detuning is small compared with the spontaneous linewidth of Rydberg state, while the laser power and temporal mode need to be specified for ns-time coherence in thermal cesium vapor microcells. The 852 nm laser can be achieved by modulating the continuous laser beam with the help of an electro-optic intensity modulator (EOIM). While this remains a technical challenge for 509 nm laser with ns-laser pulse. There is no EOIM to generate the ns-laser pulse with high power.</sec><sec>We demonstrate a novel generation method of 509 nm laser system. In our experiments, a 1018 nm fiber laser is used to produce a continuous laser with a typical linewidth of ～8 kHz and power of 10 mW. The nanosecond pulse is generated with the help of an electro-optic intensity modulator (EOIM) by modifying the continuous laser beam. The peak power of modulated optical pulse is amplified to 4600 W by using a homemade fiber amplifier. The output beam of 1018 nm is then injected into a periodically poled lithium-niobate (PPLN) to generate the second harmonics laser of 509 nm. The typical peak power of 509 nm reaches 173 W by optimizing PPLN phase matching parameters. The pulse repetition frequency of the 509 nm laser can be continuously tuned in a range of 300 kHz–100 MHz, and the pulse width can be continuously tuned in a range of 1–100 ns. Peak power fluctuation of the pulses is about 1.3%. The power 509 nm laser with optimized pulse parameters can be used to excite the cesium atom with GHz bandwidth. Meanwhile the two seed source lasers is well established experimentally, which allows alternating pulses with a different wavelength. This is an essential capability for realizing a single photon source through four-wave mixing.</sec>

Fidelity susceptibility as a diagnostic of the commensurate-incommensurate transition: A revisit of the programmable Rydberg chain

In recent years, programmable Rydberg-atom arrays have been widely used to simulate new quantum phases and phase transitions, generating great interest among theorists and experimentalists. Based on the large-scale density matrix renormalization group method, the ground-state phase diagram of one-dimensional Rydberg chains is investigated with fidelity susceptibility as an efficient diagnostic method. We find that the competition between Rydberg blockade and external detuning produces unconventional phases and phase transitions. As the Rydberg blockade radius increases, the phase transition between disordered and density-wave ordered phases changes from the standard Potts universality class to an unconventional chiral one. As the radius increases further (above Potts point but still close to the tip of the lobe), a very narrow intermediate floating-phase region begins to appear. A concise physical picture is also provided to illustrate the numerical results. Compared with previous studies, this work brings more evidence for commensurate-incommensurate quantum phase transitions in programmable quantum simulators from the perspective of quantum information, showing that fidelity susceptibility can be used to study such phase transitions.

Density-wave-ordered phases of Rydberg atoms on a honeycomb lattice.

Rydberg atom arrays have recently emerged to be a promising platform for the exploration of exotic quantum phases of matter and quantum phenomena. In this work, we map out the ground-state phase diagram of Rydberg atoms on a honeycomb lattice as a function of the Rydberg blockade radius and the laser detuning by performing large-scale finite-size density matrix renormalization group simulations. Apart from a featureless disordered phase, we find five other intricate long-range density-wave-ordered phases within a relatively wide parameter space. The properties of these quantum phases are analyzed by calculating their Rydberg excitation profiles and static structure factors. In addition, a continuous quantum phase transition belonging to the (2+1)-dimensional Ising universality class is explored by a standard finite-size scaling analysis. Our work implies some different physics, such as the possible nontrivial quantum phase transitions and a highly degenerate string ordered phase, that a honeycomb geometry could bring to the Rydberg system and serves as a numerical guide for possible real experiments.

Quantum phases of Rydberg atoms on a frustrated triangular-lattice array.

The neutral atoms coupled to a highly excited Rydberg state on a two-dimensional triangular lattice are investigated by employing the density matrix renormalization group technique in the matrix product state form. The full ground-state phase diagram as a function of blockade radius and the detuning of the exciting laser is determined by the behavior of entanglement entropy. We find several quantum phases including stripe-ordered and symmetry-breaking density-wave-ordered phases featured with regular excitation patterns of different excitation densities ρ = 1/3, 1/4, and 1/7. In addition, a ρ = 2/3 ordered phase and an interesting "order-by-disorder" phase, which has been prepared experimentally, are also observed in this work. Our work provides an exploration of the possible quantum phases that can occur in a triangularly arrayed Rydberg system, and thus could be a faithful theoretical guide for further experimental research.

Microwave Induced Ultralong-Range Charge Migration in a Rydberg Atom

A microwave induced superposition of the 40S 1/2 and 40P 1/2 states of a Cs atom has been investigated in detail. Ultralong-range charge migration which spans a region more than 200 nm has been discovered. As far as we know, this is the first time to discover charge migration in such a long range. This leads to a large dipole moment which oscillates periodically. The present discovery may stimulate new applications such as quantum simulation of many body physics dominated by periodic interactions. In addition, we find an interesting phenomenon that Cs atoms in the superposition of 40S 1/2 and 40P 1/2 have a much larger blockade radius than those of Cs (40S 1/2) or Cs (40P 1/2) atoms.

Quantum Nonlinear Optics Based on Two-Dimensional Rydberg Atom Arrays.

We propose the combination of subwavelength, two-dimensional atomic arrays and Rydberg interactions as a powerful platform to realize strong, coherent interactions between individual photons with high fidelity. The atomic spatial ordering guarantees efficient atom-light interactions without the possibility of scattering light into unwanted directions, allowing the array to act as a perfect mirror for individual photons. In turn, Rydberg interactions enable single photons to alter the optical response of the array within a potentially large blockade radius R_{b}, which can effectively punch a large "hole" for subsequent photons. We show that such a system enables a coherent photon-photon gate or switch, with a significantly better error scaling (∼R_{b}^{-4}) than in a disordered ensemble. We also investigate the optical properties of the system in the limit of strong input intensities and show that this many-body quantum driven dissipative system can be modeled well by a semiclassical model based on holes punched in a classical mirror.

Prediction of Toric Code Topological Order from Rydberg Blockade

The physical realization of Z2 topological order as encountered in the paradigmatic toric code has proven to be an elusive goal. We predict that this phase of matter can be realized in a two-dimensional array of Rydberg atoms placed on the ruby lattice, at specific values of the Rydberg blockade radius. First, we show that the blockade model—also known as a “PXP” model—realizes a monomer-dimer model on the kagome lattice with a single-site kinetic term. This model can be interpreted as a Z2 gauge theory whose dynamics is generated by monomer fluctuations. We obtain its phase diagram using the numerical density matrix renormalization group method and find a topological quantum liquid (TQL) as evidenced by multiple measures including (i) a continuous transition between two featureless phases, (ii) a topological entanglement entropy of ln2 as measured in various geometries, (iii) degenerate topological ground states, and (iv) the expected modular matrix from ground state overlap. Next, we show that the TQL persists upon including realistic, algebraically decaying van der Waals interactions V(r)∼1/r6 for a choice of lattice parameters. Moreover, we can directly access topological loop operators, including the Fredenhagen-Marcu order parameter. We show how these can be measured experimentally using a dynamic protocol, providing a “smoking gun” experimental signature of the TQL phase. Finally, we show how to trap an emergent anyon and realize different topological boundary conditions, and we discuss the implications for exploring fault-tolerant quantum memories.12 MoreReceived 24 November 2020Accepted 19 May 2021DOI:https://doi.org/10.1103/PhysRevX.11.031005Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasTopological phases of matterTopological quantum computingPhysical SystemsRydberg atoms & moleculesCondensed Matter, Materials & Applied Physics

Exact many-body scars and their stability in constrained quantum chains

Quantum scars are non-thermal eigenstates characterized by low entanglement entropy, initially detected in systems subject to nearest-neighbor Rydberg blockade, the so called PXP model. While most of these special eigenstates elude an analytical description and seem to hybridize with nearby thermal eigenstates for large systems, some of them can be written as matrix product states (MPS) with size-independent bond dimension. We study the response of these exact quantum scars to perturbations by analysing the scaling of the fidelity susceptibility with system size. We find that some of them are anomalously stable at first order in perturbation theory, in sharp contrast to the eigenstate thermalization hypothesis. However, this stability seems to breakdown when all orders are taken into account. We further investigate models with larger blockade radius and find a novel set of exact quantum scars, that we write down analytically and compare with the PXP exact eigenstates. We show that they exhibit the same robustness against perturbations at first order.

Depletion imaging of Rydberg atoms in cold atomic gases

We present a depletion imaging technique to map out the spatial and temporal dependency of the density distribution of an ultracold gas of Rydberg atoms. Locally resolved absorption depletion, observed through differential ground state absorption imaging of a 87Rb cloud in presence and absence of pre-excited Rydberg atoms, reveals their projected two-dimensional distribution. By employing a closed two-level optical transition uncoupled from the Rydberg state, the highly excited atoms are preserved during imaging. We measure the excitation dynamics of the state of 87Rb, observing a saturation of the two-dimensional Rydberg density. Such outcome can be explained by the Rydberg blockade effect which prevents resonant excitation of close-by Rydberg atoms due to strong dipolar interactions. By combining the superatom description, where atoms within a blockade radius are represented as collective excitations, with a Monte Carlo sampling, we can quantitatively model the observed excitation dynamics and infer the full three-dimensional distribution of Rydberg atoms, that can serve as a starting point for quantum simulation of many-body dynamics involving Rydberg spin systems.

Anisotropic interactions in electric field polarized ultracold Rydberg gases

We calculate pair potential curves for interacting Rydberg atoms in a constant electric field and use them to determine the effective C3 dipole–dipole and C6 van der Waals coefficients. We compare the C3 and C6 with experiments where the angle of a polarizing electric field is varied with respect to the axis of a quasi-1-dimensional trap at ultracold temperatures. The dipoles produced via polarization of the atoms have an angular dependent dipole–dipole interaction. We focus on the interaction potential of two rubidium Rydberg atoms in states in the blockade regime. For internuclear distances close to the blockade radius, Rbl ≈ 4–6 μm, molecular calculations are in much better agreement with experimental results than those based on the properties of single atoms and independent calculations of C3 and C6 which were used to analyze the original experiment. We find that the calculated C6 coefficient is within 8% of the experimental value while the C3 coefficient is within 20% of the experimental value.

Anderson localization in an oscillating Rydberg-dressed condensate with random disorder

We numerically study the Anderson localization in an oscillating one-dimensional Rydberg-dressed Bose-Einstein condensate with weak random disorder in which the range of the interaction, the blockade radius ${R}_{\mathrm{c}}$, is variable. Without disorder, the uniform system can undergo a superfluid-supersolid transition at ${R}_{\text{c}}={l}_{\mathrm{c}}\ensuremath{\simeq}1.7{\ensuremath{\xi}}_{0}$ with ${\ensuremath{\xi}}_{\text{0}}$ the zero-range healing length. When ${\ensuremath{\xi}}_{0}$ exceeds the disorder correlation length ${\ensuremath{\sigma}}_{\mathrm{D}}$, we show that exponential localization occurs in the equilibrium condensate when ${R}_{\mathrm{c}}\ensuremath{\le}{l}_{\mathrm{c}}$, while Gaussian localization occurs when ${R}_{\mathrm{c}}g{l}_{\mathrm{c}}$. The latter suggests that the $k$ wave for a long-ranged interacting system could decay Gaussianly with weak random disorder.

Analysis of atom–photon quantum interface with intracavity Rydberg-blocked atomic ensemble via two-photon transition

We study the atom-photon quantum interface with intracavity Rydberg-blocked atomic ensemble where the ground-Rydberg transition is realized by two-photon transition. Via theoretical analysis, we report our recent findings of the Jaynes-Cummings model on optical domain and robust atom-photon quantum gate enabled by this platform. The requirement on the implementation is mild which includes an optical cavity of moderately high finesse, typical alkali atoms such as Rb or Cs and the condition that cold atomic ensemble is well within the Rydberg blockade radius. The analysis focuses on the atomic ensemble's collective coupling to the quantized optical field in the cavity mode. We demonstrate its capability to serve as a controlled-PHASE gate between photonic qubits and matter qubits. The detrimental effects associated with several major decoherence factors of this system are also considered in the analysis.

Nonadiabatic holonomic quantum computation with Rydberg superatoms

Nonadiabatic holonomic quantum computation has received increasing attention due to its robustness against control errors as well as high-speed realization. Several schemes of its implementation have been put forward based on various physical systems, each of which has some particular merits. In this paper, we put forward an alternative scheme of nonadiabatic holonomic quantum computation, in which a universal set of quantum gates is realized based on Rydberg superatoms. A Rydberg superatom is a mesoscopic atomic ensemble that allows for only a single Rydberg excitation shared by many atoms within a blockade radius and can be used to generate the collective states to encode the qubits. In our scheme, the qubit is encoded into two collective ground states of Rydberg superatoms and the interaction between two long-range Rydberg superatoms is mediated by a microwave cavity with the aid of two additional collective Rydberg states. Different from the previous schemes,which are based on the systems in the microscope scale, the present scheme is based on atomic ensembles in the mesoscopic scale. Besides the common merits of nonadiabatic holonomic quantum computation such as the robustness and the speediness, the Rydberg-superatom-based scheme has the following particular merits: the long coherence time of Rydberg states and the operability of the mesoscopic systems.