Bidirectional Emission Research Articles

Unidirectional and highly dispersive grating emitters for silicon photonic beam steerers.

Grating emitters are the key component used in silicon photonic beam steerers to create light emission and allow dispersion-based steering. Conventional grating emitters are inefficient due to bidirectional emission, and their angular dispersion is only on the order of 0.1°/nm. In this paper, we develop unidirectional grating emitters by choosing a top cladding material with a refraction index higher than that of the bottom cladding. The refractive index difference allows the phase-matching condition to be satisfied only for the upward diffraction. We demonstrate experimentally grating emitters with a directionality of 83% and an angular dispersion of 0.79°/nm. These grating emitters have a simple device structure compatible with the standard silicon photonic platform.

Fluorescence and lasing of neutral nitrogen molecules inside femtosecond laser filaments in air: mechanism and applications.

High power femtosecond laser pulses launched in air undergo nonlinear filamentary propagation, featuring a bright and thin plasma channel in air with its length much longer than the Rayleigh length of the laser beam. During this nonlinear propagation process, the laser pulses experience rich and complex spatial and temporal transformations. With its applications ranging from supercontinuum generation, laser pulse compression, remote sensing to triggering of lightning, the underlying physical mechanism of filamentation has been intensively studied. In this review, we will focus on the fluorescence and cavity-free lasing effect of the plasma filaments in air. The different mechanisms underlying the fluorescence of the excited neutral nitrogen molecules will be throughly examined and it is concluded that the electron collision excitation is the dominant channel for the formation of the excited nitrogen molecules. The recently discovered "air lasing" effect, a cavity-free bidirectional lasing emission emitted by the filaments, will be introduced and its main properties will be emphasized. The applications of the fluorescence and lasing effect of the neutral nitrogen molecules will be introduced, with two examples on spectroscopy and detection of electric field. Finally, we discuss the quenching effect of the lasing effect in atmosphere and the mechanisms responsible will be analyzed. An outlook for the achievement of backward lasing in air will be briefly presented.

Anomalous Nernst Effect Induced Terahertz Emission in a Single Ferromagnetic Film.

Despite its important role in understanding ultrafast spin dynamics and revealing novel spin/orbit effects, the mechanism of the terahertz (THz) emission from a single ferromagnetic nanofilm upon a femtosecond laser pump still remains elusive. Recent experiments have shown exotic symmetry, which is not expected from the routinely adopted mechanism of ultrafast demagnetization. Here, by developing a bidirectional pump-THz emission spectroscopy and associated symmetry analysis method, we set a benchmark for the experimental distinction of the THz emission induced by various mechanisms. Our results unambiguously unveil a new mechanism─anomalous Nernst effect (ANE) induced THz emission due to the ultrafast temperature gradient created by a femtosecond laser. Quantitative analysis shows that the THz emission exhibits interesting thickness dependence where different mechanisms dominate at different thickness ranges. Our work not only clarifies the origin of the ferromagnetic-based THz emission but also offers a fertile platform for investigating the ultrafast optomagnetism and THz spintronics.

Preliminary Experimental Research on Split-Cathode-Fed Relativistic Magnetron With Bidirectional Emission Structure

Simulations and experiments of an <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">${S}$ </tex-math></inline-formula> -band TEM-output relativistic magnetron (RM) driven by split cathode (SC) are proposed. In the previous researches on SC, as a result of the space-charge-screening effect of squeeze-state electrons accumulated nearby the emission surface, the diode current is limited, which finally results in low output power. To improve the output performance, a bidirectional emission SC (BSC) is introduced. Experimental results on EPA-90 high-voltage electron beam accelerator demonstrate that when the voltage is around 480 kV and the axial magnetic field is 0.49 T, comparing with a conventional unidirectional emission SC, the output power can be enhanced from 124 to 400 MW by adding an extra downstream emitter. This work lays a foundation for further researches to make the SC-fed RM more practical.

Photon pairs bi-directionally emitted from a resonant metasurface.

Metasurfaces are artificially structured surfaces able to control the properties of light at subwavelength scales. While, initially, they have been proposed as means to control classical optical fields, they are now emerging as nanoscale sources of quantum light, in particular of entangled photons with versatile properties. Geometric resonances in metasurfaces have been recently used to engineer the frequency spectrum of entangled photons, but the emission directivity was so far less studied. Here, we generate photon pairs via spontaneous parametric down conversion from a metasurface supporting a quasi-bound state in the continuum (BIC) leading to remarkable emission directivities. The pair generation rate is enhanced 67 times compared to the case of an unpatterned film of the same thickness and material. At the wavelength of the quasi-BIC resonance, photons are mostly emitted backwards, while their partners, spectrally detuned by only 8 nm, are emitted forwards. This behavior demonstrates fine spectral splitting of entangled photons and their bi-directional emission, never before observed in nanoscale sources. We expect this work to be a starting point for the efficient demultiplexing of photons in nanoscale quantum optics.

Bidirectional phonon emission in two-dimensional heterostructures triggered by ultrafast charge transfer.

Photoinduced charge transfer in van der Waals heterostructures occurs on the 100 fs timescale despite weak interlayer coupling and momentum mismatch. However, little is understood about the microscopic mechanism behind this ultrafast process and the role of the lattice in mediating it. Here, using femtosecond electron diffraction, we directly visualize lattice dynamics in photoexcited heterostructures of WSe2/WS2 monolayers. Following the selective excitation of WSe2, we measure the concurrent heating of both WSe2 and WS2 on a picosecond timescale-an observation that is not explained by phonon transport across the interface. Using first-principles calculations, we identify a fast channel involving an electronic state hybridized across the heterostructure, enabling phonon-assisted interlayer transfer of photoexcited electrons. Phonons are emitted in both layers on the femtosecond timescale via this channel, consistent with the simultaneous lattice heating observed experimentally. Taken together, our work indicates strong electron-phonon coupling via layer-hybridized electronic states-a novel route to control energy transport across atomic junctions.

A robust scheme for unidirectional emission from a hybrid whispering gallery cavity system based on transformation optics.

Using the transformation cavity, a gradient index cavity designed by transformation optics, we propose a hybrid resonator system to extract unidirectional narrow-beam emission from high-Q whispering gallery modes by embedding a transformation cavity inside a deformed uniform index cavity that exhibits unidirectional narrow-beam emission. For effective mode coupling between the transformation cavity and enclosing cavity, the embedded transformation cavity is designed to have bidirectional evanescent emission, which enables most of the emission from the transformation cavity to be laterally incident on the rim of the enclosing deformed cavity. Consequently, ultrahigh-Q resonances of this system can provide a sharp free-space light output, which is difficult to achieve by embedding a homogeneous disk cavity instead of the transformation cavity.

Transformation cavities with a narrow refractive index profile.

Recently, gradient index cavities, or so-called transformation cavities, designed by conformal transformation optics, have been studied to support resonant modes with both high Q-factors and emission directionality. We propose a new, to the best of our knowledge, design method for transformation cavities to realize a narrower width of the refractive index profile, a great advantage in experimental implementations, without losing the benefits of conformal mapping. We study resonant modes with both high Q-factors and directional emission in newly designed transformation cavities, where the refractive index profile is 50% narrower than in previously proposed transformation cavities. By varying a system parameter with a fixed maximal value of the refractive index profile inside the cavity, the width of the refractive index profile narrows, the Q-factors become higher, and the near and far field patterns maintain their properties, namely, conformal whispering gallery modes and bidirectional emission, respectively.

Observation of direction instability in a fiber ring laser

We report on the observation of a new phenomenon occurring in a fiber ring laser. This phenomenon is about the transition from an initially bidirectional emission of a reciprocal fiber ring laser to a unidirectional emission at a certain pump power threshold. In addition, the final direction is not predefined but appears to be randomly chosen every time the threshold is exceeded. Therefore, we term this new phenomenon direction instability. Furthermore, we provide a first discussion of how the instability threshold is influenced by the length and the loss of the cavity. We show that the threshold follows a power times length scaling, indicating a nonlinear origin.

Programmable directional emitter and receiver of itinerant microwave photons in a waveguide

We theoretically demonstrate dynamically selective bidirectional emission and absorption of a single itinerant microwave photon in a waveguide. The proposed device is an artificial molecule composed of two qubits coupled to a waveguide a quarter-wavelength apart. By using simulations based on the input--output theory, we show that upon preparing an appropriate entangled state of the two qubits, a photon is emitted directionally as a result of the destructive interference occurring either at the right or left of the qubits. Moreover, we demonstrate that this artificial molecule possesses the capability of absorbing and transmitting an incoming photon on-demand, a feature essential to the creation of a fully inter-connected one-dimensional quantum network, in which quantum information can be exchanged between any two given nodes.

Soil Biogenic Volatile Organic Compound Flux in a Mixed Hardwood Forest: Net Uptake at Warmer Temperatures and the Importance of Mycorrhizal Associations

AbstractBiogenic volatile organic compounds (bVOCs) play important roles in ecological interactions and Earth system processes, yet the biological and physical processes that drive soil bVOC exchanges remain poorly understood. In temperate forests, nearly all tree species associate with arbuscular mycorrhizal (AM) or ectomycorrhizal (ECM) fungi. Given well‐established differences in soil biogeochemistry between AM‐dominated and ECM‐dominated stands, we hypothesized that bVOC exchanges with the atmosphere would differ between soils from the two stand types. We measured bVOC fluxes at the soil‐atmosphere interface in plots dominated by AM‐ and ECM‐associated trees in a deciduous forest in south‐central Indiana, USA during the early and late vegetative growing season. Soils in both AM‐ and ECM‐dominated plots were a net bVOC sink following leaf‐out and were a greater bVOC sink or smaller source at warmer soil temperatures (Ts). The flux of different bVOCs from ECM plots was often related to soil water content in addition to Ts. Methanol dominated total bVOC fluxes, and ECM soils demonstrated greater uptake relative to AM‐dominated plots, on the order of 170 nmol m−2 hr−1 during the early growing season. Our results demonstrate the importance of soil dynamics characterized by mycorrhizal associations to bVOC dynamics in forested ecosystems and emphasize the need to study bidirectional soil bVOC uptake and emission processes.

氧气对飞秒激光泵浦的氮气分子无腔激光效应的淬灭作用（特邀）

Nitrogen gas pumped by circularly polarized femtosecond laser pulses gives rise to bidirectional lasing emission，which holds unique potential for remote optical sensing application. However，the presence of oxygen molecules strongly suppresses this lasing effect. The influence of O2，Kr，Ar and He on the lasing effect of nitrogen molecules was compared，and the fluorescence of nitrogen molecules in pure nitrogen and ambient air was examined. It is observed that the lasing presents a similar quenching effect with the partial pressure of O2 and Kr，since Kr has a close ionization potential compared to O2. In contrast， for He which has a much higher ionization potential，there is no significant quenching effect. Therefore it is suggested that the quenching effect of O2 on nitrogen molecules mainly stems from the fact that O2 leads to a reduction of the clamped laser intensity inside the plasma filaments，which results in a decrease of the kinetic energy of the free electrons and an inefficient collision excitation.

Bidirectional to unidirectional emission of fluorescence controlled by optical traveling wave antennas

Abstract Tailoring the fluorescence emission of quantum emitters to a desired direction is a crucial issue to achieve high efficient photodetection and realize unique optoelectronic devices. In this study, the directional emission of quantum dots controlled by optical traveling wave antennas based on 1D silver nanowires (NWs) was investigated. Both leaky waves and surface waves on a single NW are utilized for fluorescence emission control, and we show that the coupled fluorescence transforms from bidirectional to unidirectional emission when the surrounding medium changes from air to water. Moreover, in the unidirectional case, we obtain an ultra-narrow half-power bandwidth about 20°. Finite-difference time-domain simulations and Green’s function method in a stratified medium are used to calculate the far-field emission patterns of the hybrid structures, which agree well with the experiments. Further analyses based on typical modes and the dipole-chain model also reveal the mechanism behind the bidirectional and unidirectional fluorescence emission. These results show that the structures have great potential in integrated on-chip, sensing and photon-collection devices.

Dynamical Analysis of Modal Coupling in Rare-Earth Whispering-Gallery-Mode Microlasers

We report on an experimental study of laser regime in erbium-doped whispering gallery mode (WGM) microspheres under modal-coupling between the co- and counter-propagating modes. The evidence of modal coupling has been observed in the relative intensity noise spectrum of several WGM lasers. Cross-correlation measurements have been carried out in order to determine precisely the emission regimes. It is shown that depending on the material constituting the WGM resonator, frequency locked bidirectional emission or self-modulated regime can be reached. The control of the laser emission regime of WGM micro-lasers is of great importance in the aim of applications in microwave optics or optical sensor miniaturization.

Molecular Engineering of Mechanochromic Materials by Programmed C-H Arylation: Making a Counterpoint in the Chromism Trend.

The development of facile methods for screening organic functional molecules through C-H bond activation is a revolutionary trend in materials research. The prediction of mechanochromism as well as mechanochromic trends of luminogens is an appealing yet challenging puzzle. Here, we present a strategy for the design of mechanochromic luminogens based on the dipole moment of donor-acceptor molecules. For this purpose, a highly efficient route to 2,7-diaryl-[1,2,4]triazolo[1,5-a]pyrimidines (2,7-diaryl-TAPs) has been established through programmed C-H arylation, which unlocks a great opportunity to rapidly assemble a library of fluorophores for the discovery of mechanochromic regularity. Molecular dipole moment can be employed to explain and further predict the mechanochromic trends. The 2,7-diaryl-TAPs with electron-donating groups on the 2-aryl and electron-withdrawing groups on the 7-aryl possess a relatively small dipole moment and exhibit a red-shifted mechanochromism. When the two aryls are interchanged, the resulting luminogens have a relatively large dipole moment and display a blue-shifted mechanochromism. Seven pairs of isomers with opposite mechanochromic trends are presented as illustrative examples. The aryl-interchanged congeners with a bidirectional emission shift are structurally similar, which provides an avenue for understanding in-depth the mechanochromic mechanism.

Measurement and Analysis of Bidirectional SIF Emissions in Wheat Canopies

Numerous observations and modeling results have shown that there is noticeable directional variation in the solar-induced chlorophyll fluorescence (SIF), and this has not been well investigated. In this paper, 16 multiangular spectral observations were carried out on winter wheat to assess the bidirectional SIF emission. First, the bidirectional SIF emission was retrieved from the spectral measurements made by a high-performance QE Pro spectrometer and an automatic multiangle observation system using the 3FLD algorithm. The bidirectional shape of the SIF emission was found to be similar to that of the canopy reflectance in the solar principal plane, with a mean correlation coefficient of 0.94 and 0.97 at the O 2 -B and O 2 -A bands, respectively. The modified Rahman-Pinty-Verstraete (MRPV) model, a semiempirical bidirectional reflectance distribution function (BRDF) model, was then employed to describe the bidirectional variation in the SIF and reflectance with a mean root-mean-square-error value of 0.036 and 0.041 mW m -2 sr -1 nm -1 for the SIF at the O 2 -B and O 2 -A bands, respectively. Finally, both the bidirectional reflectance and SIF were BRDF corrected to nadir using the MRPV model. Most of the directional variation was successfully corrected by this method-the mean correction ratios were 87% and 81% for the reflectance at the O 2 -B and O 2 -A bands and 84% and 72% for the SIF at the O 2 -B and O 2 -A bands, respectively. Therefore, the SIF emission cannot be regarded as isotropic, and the high similarity between the bidirectional SIF and reflectance, together with the BRDF correction results, indicates that the bidirectional SIF emission can be adjusted using either the BRDF reflectance models or prior knowledge.

Unidirectional Lasing from Template-Stripped Two-Dimensional Plasmonic Crystals.

Plasmon lasers support cavity structures with sizes below that of the diffraction limit. However, most plasmon-based lasers show bidirectional lasing emission or emission with limited far-field directionality and large radiative losses. Here, we report unidirectional lasing from ultrasmooth, template-stripped two-dimensional (2D) plasmonic crystals. Optically pumped 2D plasmonic crystals (Au or Ag) surrounded by dye molecules exhibited lasing in a single emission direction and their lasing wavelength could be tuned by modulating the dielectric environment. We found that 2D plasmonic crystals were an ideal architecture to screen how nanocavity unit-cell structure, metal material, and gain media affected the lasing response. We discovered that template-stripped strong plasmonic materials with cylindrical posts were an optimal cavity design for a unidirectional laser operating at room temperature.

Spectral narrowing of Yb:YAG waveguide lasers through hybrid integration with ultrafast laser written Bragg gratings.

Laser written waveguides in crystalline materials can be used to make highly efficient, high gain lasers. The bi-directional emission from such lasers however is typically broadband with poor spectral control. Hybridizing a tapered, mode matched laser written Bragg grating with a broadband Yb:YAG crystalline waveguide laser, we demonstrate single longitudinal mode output from one end of the device. Careful control of the grating characteristics led to laser thresholds below 90 mW, slope efficiencies greater than 42% and output powers greater than 20 mW.

Mathematical modeling of basic physical and chemical processes in the production of glass

The main stages of the glass manufacturing process in terms of mathematical modeling were considered. Based on the formulated assumptions, describing the glass manufacturing process physics, equations of continuity, momentum, energy, turbulent kinetic energy, turbulent kinetic energy dissipation in the form of Reynolds-averaged Navier-Stokes equations were described. Initial and boundary conditions needed to solve the mathematical modeling problem were determined. The bi-directional emissivity indicator on the translucent border between the flue gases and molten glass was defined from Fresnel formulas. Temperature distribution simulation was performed by the computational fluid dynamics (CFD) methods. Simulation of turbulent flows was carried out using the κ-e turbulence model. Solution of the radiation energy transfer equation is based on the P1 approximation of the spherical harmonics method for gray two-temperature medium. As a result, the temperature distribution in the glass furnace was obtained. The temperature distribution is an important tool for investigating glass furnace control systems.

Transparent organic light-emitting diodes with different bi-directional emission colors using color-conversion capping layers

We report a study on transparent organic light-emitting diodes (OLEDs) with different bi-directional emission colors, enabled by color-conversion organic capping layers. Starting from a transparent blue OLED with an uncapped Ag top electrode exhibiting an average transmittance of 33.9%, a 4-(dicyanomethylene)-2-methyl-6-(4-dimethylaminostyryl)-4H-pyran (DCM)-doped tris-(8-hydroxy-quinolinato)-aluminum (Alq3) capping layer is applied to achieve color-conversion from blue to orange-red on the top side while maintaining almost unchanged device transmittance. This color-conversion capping layer does not only change the color of the top side emission, but also enhances the overall device efficiency due to the optical interaction of the capping layer with the primary blue transparent OLED. Top white emission from the transparent bi-directional OLED exhibits a correlated color temperature around 6000–7000K, with excellent color stability as evidenced by an extremely small variation in color coordinate of Δ(x,y)=(0.002, 0.002) in the forward luminance range of 100–1000cdm−2. At the same time, the blue emission color of bottom side is not influenced by the color conversion capping layer, which finally results in different emission colors of the two opposite sides of our transparent OLEDs.