This paper presents a study on the double-loop controller design technique for a single-phase power factor correction (PFC) three-level (TL) boost converter. Designing a double-loop controller using conventional methods is challenging due to the 120 Hz voltage ripple in the output voltage. This study proposes new double-loop control design methods using a band-stop filter and MATLAB SISOTOOL, detailed in a step-by-step sequence. A band-stop filter with a 120 Hz stop band is applied to the double-loop controller design. Modeling based on the state-space equation, applicable to the full duty range, is constructed to obtain the transfer function. The double-loop controller structure is then designed, and optimal gains that satisfy the design requirements are obtained through automatic tuning using the MATLAB SISOTOOL library. The simulation results demonstrate the performance of the proposed method, which is further verified by experimental results.