Field observations and U–Pb zircon data yield evidence that the Kaintaleck Complex represents a distinct crystalline basement unit of the eastern Greywacke Zone and contrasts partly with other pre-Alpine basement complexes of the Eastern Alps. The age data indicate possible Late Archean rock formation, several magmatic and metamorphic events in the Early Palaeozoic (ca. 520–490 and ca. 400–360 Ma), and low-grade metamorphic overprint in the Cretaceous. Zircons from a garnet gneiss layer in a plagioclase gneiss and amphibolite sequence yield an upper intercept age of ca. 2.55 Ga which is interpreted as a possible protolith age. The lower intercept age at 514 Ma represents either (1) a magmatic event or (2) a metamorphic overprint within amphibolite facies conditions. Magmatic zircons derived from granitic orthogneiss boulders of the Kalwang Conglomerate, which covers the crystalline basement, crystallised at ca. 500 Ma. The lower discordia intercepts of the orthogneiss boulders mark the Cretaceous low-grade metamorphic overprint. The lower intercept age of paragneiss zircons from another slice of the Kaintaleck Complex suggests a likely Devonian metamorphic event at ca. 390–400 Ma. The new data demonstrate that the Kaintaleck Complex experienced several stages of tectonothermal evolutions, which are in contrast to the evolution of the main mass of the Austroalpine basement. The data constrain linkages of this part of the Austroalpine basement to the Cordillere Ligerienne and Cadomian block within West-European Variscides.