Array Of Atoms Research Articles

Emergent Glassy Behavior in a Kagome Rydberg Atom Array.

We present large-scale quantum MonteCarlo simulation results on a realistic Hamiltonian of kagome-lattice Rydberg atom arrays. Although the system has no intrinsic disorder, intriguingly, our analyses of static and dynamic properties on large system sizes reveal emergent glassy behavior in a region of parameter space located between two valence bond solid phases. The extent of this glassy region is demarcated using the Edwards-Anderson order parameter, and its phase transitions to the two proximate valence bond solids-as well as the crossover towards a trivial paramagnetic phase-are identified. We demonstrate the intrinsically slow (imaginary) time dynamics deep inside the glassy phase and discuss experimental considerations for detecting such a quantum disordered phase with numerous nearly degenerate local minima. Our proposal paves a new route to the study of real-time glassy phenomena and highlights the potential for quantum simulation of a distinct phase of quantum matter beyond solids and liquids in current-generation Rydberg platforms.

Dark-State Enhanced Loading of an Optical Tweezer Array.

Neutral atoms and molecules trapped in optical tweezers have become a prevalent resource for quantum simulation, computation, and metrology. However, the maximum achievable system sizes of such arrays are often limited by the stochastic nature of loading into optical tweezers, with a typical loading probability of only 50%. Here we present a species-agnostic method for dark-state enhanced loading (DSEL) based on real-time feedback, long-lived shelving states, and iterated array reloading. We demonstrate this technique with a 95-tweezer array of ^{88}Sr atoms, achieving a maximum loading probability of 84.02(4)% and a maximum array size of 91 atoms in one dimension. Our protocol is complementary to, and compatible with, existing schemes for enhanced loading based on direct control over light-assisted collisions, and we predict it can enable close-to-unity filling for arrays of atoms or molecules.

Accelerating the Assembly of Defect-Free Atomic Arrays with Maximum Parallelisms

Defect-free atomic arrays have been demonstrated as a scalable and fully-controllable platform for quantum simulations and quantum computations. To push the qubit size limit of this platform further, we design an integrated measurement and feedback system, based on field programmable gate array (FPGA), to quickly assemble two-dimensional defect-free atomic array using maximum parallelisms. The total time cost of the rearrangement is first reduced by processing atom detection, atomic occupation analysis, rearrangement strategy formulation, and acousto-optic deflectors (AOD) driving signal generation in parallel in time. Then, by simultaneously moving multiple atoms in the same row (column), we save rearrangement time by parallelism in space. To best utilize these parallelisms, we propose a new algorithm named Tetris algorithm to reassemble atoms to arbitrary target array geometry from two-dimensional stochastically loaded atomic arrays. For an $L \times L$ target array geometry, the number of moves scales as $L$, and the total rearrangement time scales at most as $L^2$. We present the overall performance for different target geometries, and demonstrate a significant reduction in rearrangement time and the potential to scale up defect-free atomic array system to thousands of qubits.

Dynamic population of multiexcitation subradiant states in incoherently excited atomic arrays

The authors theoretically investigate the creation of subradiant states with multiple excitations in dense arrays of quantum emitters, which is a long-lasting challenge due to the complexity of the system and the experimental limitations in state-of-the-art platforms. The authors analyze the effects of trapping geometry and correlations on the subradiant-state formation and provide insights for controlling and utilizing subradiant states in quantum technologies.

Scalable Multilayer Architecture of Assembled Single-Atom Qubit Arrays in a Three-Dimensional Talbot Tweezer Lattice.

We report on the realization of a novel platform for the creation of large-scale 3D multilayer configurations of planar arrays of individual neutral-atom qubits: a microlens-generated Talbot tweezer lattice that extends 2D tweezer arrays to the third dimension at no additional costs. We demonstrate the trapping and imaging of rubidium atoms in integer and fractional Talbot planes and the assembly of defect-free atom arrays in different layers. The Talbot self-imaging effect for microlens arrays constitutes a structurally robust and wavelength-universal method for the realization of 3D atom arrays with beneficial scaling properties. With more than 750 qubit sites per 2D layer, these scaling properties imply that 10 000 qubit sites are already accessible in 3D in our current implementation. The trap topology and functionality are configurable in the micrometer regime. We use this to generate interleaved lattices with dynamic position control and parallelized sublattice addressing of spin states for immediate application in quantum science and technology.

Topology and Polarization of Optical Vortex Fields from Atomic Phased Arrays

We developed a theoretical formalism for the generation of optical vortices by phased arrays of atoms. Using the Jacobi–Anger expansion, we demonstrated the resulting field topology and determined the least number of individual atoms necessary for the generation of vortices with a given topological charge. Vector vortices were considered, taking into account both the spin and orbital angular momenta of electromagnetic fields. It was found for the vortex field that, in the far field limit, the spatial variation in spin-density matrix parameters—orientation and alignment—is independent of the distance to the radiation source.

Precisely Orientating Atomic Array in One-Dimension Tellurium Microneedles Enhances Intrinsic Piezoelectricity for an Efficient Piezo-Catalytic Sterilization.

Comprehensively understanding the interdependency between the orientated atomic array and intrinsic piezoelectricity in one-dimension (1D) tellurium (Te) crystals will greatly benefit their practical piezo-catalytic applications. Herein, we successfully synthesized the various 1D Te microneedles by precisely orientating the atomic growth orientation by tuning (100)/(110) planes ratios (Te-0.6, Te-0.3, Te-0.4) to reveal the secrets of piezoelectricity. Explicitly, the theoretical simulations and experimental results have solidly validated that the Te-0.6 microneedle grown along the [110] orientation possesses a stronger asymmetric distribution of Te atoms array causing the enhanced dipole moment and in-plane polarization, which boosts a higher transfer and separation efficiency of the electron and hole pairs and a higher piezoelectric potential under the same stress. Additionally, the orientated atomic array along the [110] has p antibonding states with a higher energy level, resulting in a higher CB potential and a broadened band gap. Meanwhile, it also has a much lower barrier toward the valid adsorption of H2O and O2 molecules over other orientations, effectively conducive to the production of reactive oxygen species (ROS) for the efficient piezo-catalytic sterilization. Therefore, this study not only broadens the fundamental perspectives in understanding the intrinsic mechanism of piezoelectricity in 1D Te crystals but also provides a candidate 1D Te microneedle for practical piezo-catalytic applications.

Distributed Quantum Computing with Photons and Atomic Memories

AbstractThe promise of universal quantum computing requires scalable single‐ and inter‐qubit control interactions. Currently, three of the leading candidate platforms for quantum computing are based on superconducting circuits, trapped ions, and neutral atom arrays. However, these systems have strong interaction with environmental and control noises that introduce decoherence of qubit states and gate operations. Alternatively, photons are well decoupled from the environment and have advantages of speed and timing for quantum computing. Photonic systems have already demonstrated capability for solving specific intractable problems like Boson sampling, but face challenges for practically scalable universal quantum computing solutions because it is extremely difficult for a single photon to “talk” to another deterministically. Here, a universal distributed quantum computing scheme based on photons and atomic‐ensemble‐based quantum memories is proposed. Taking the established photonic advantages, two‐qubit nonlinear interaction is mediated by converting photonic qubits into quantum memory states and employing Rydberg blockade for the controlled gate operation. Spatial and temporal scalability of this scheme is demonstrated further. These results show photon‐atom network hybrid approach can be a potential solution to universal distributed quantum computing.

Maximally entangled Rydberg-atom pairs via Landau-Zener sweeps

We analyze the formation of maximally entangled Rydberg atom pairs subjected to Landau-Zener sweeps of the atom-light detuning. Though the populations reach a steady value at longer times, the phases evolve continuously, leading to periodic oscillations in the entanglement entropy. The local unitary equivalence between the obtained maximally entangled states and the Bell states is verified by computing the polynomial invariants. Finally, we study the effect of spontaneous emission from the Rydberg state of rubidium atoms on the correlation dynamics and show that the oscillatory dynamics persists for high-lying Rydberg states. Our study may offer novel ways to generate maximally entangled states, quantum gates and exotic quantum matter in arrays of Rydberg atoms through Landau Zener sweeps.

Characteristics of 1D ordered arrays of optical centers in solid-state photonics

Collective interaction of emitter arrays has lately attracted significant attention due to its role in controlling directionality of radiation, spontaneous emission and coherence. We focus on light interactions with engineered arrays of solid-state emitters in photonic resonators. We theoretically study light interaction with an array of emitters or optical centers embedded inside a microring resonator and discuss its application in the context of solid-state photonic systems. We discuss how such arrays can be experimentally realized and how the inhomogeneous broadening of mesoscopic atomic arrays can be leveraged to study broadband collective excitations in the array.

Measuring Arbitrary Physical Properties in Analog Quantum Simulation

A central challenge in analog quantum simulation is to characterize desirable physical properties of quantum states produced in experiments. However, in conventional approaches, the extraction of arbitrary information requires performing measurements in many different bases, which necessitates a high level of control that present-day quantum devices may not have. Here, we propose and analyze a scalable protocol that leverages the ergodic nature of generic quantum dynamics, enabling the efficient extraction of many physical properties. The protocol does not require sophisticated controls and can be generically implemented in analog quantum simulation platforms today. Our protocol involves introducing ancillary degrees of freedom in a predetermined state to a system of interest, quenching the joint system under Hamiltonian dynamics native to the particular experimental platform, and then measuring globally in a single, fixed basis. We show that arbitrary information of the original quantum state is contained within such measurement data, and can be extracted using a classical data-processing procedure. We numerically demonstrate our approach with a number of examples, including the measurements of entanglement entropy, many-body Chern number, and various superconducting orders in systems of neutral atom arrays, bosonic and fermionic particles on optical lattices, respectively, only assuming existing technological capabilities. Our protocol excitingly promises to overcome limited controllability and, thus, enhance the versatility and utility of near-term quantum technologies.

Nanoporous N/O:sp2-C films functionalized at nonbonding electrons of a biogenic husk (green chili) with deep UV-visible light absorption-emission for photocatalysis and other applications

The wastewater, which is released at industries, depleting aquatic ecology, and stringent pollution regulations, is a global issue of safety of the green nature. There is an urgent need for developing sustainable materials for pollutant removal from the polluted ground and/or surface water. In this purview, a sp2_C (a synergistic photocatalyst) offers a special remedy to degrade toxics in the potable water. It is nontoxic and ecological, and readily adsorbs the pollutants in water. Here, we explore synthesis of a biogenic N/O doped C-sp2 (p-GNO) of a nanoporous husk (green chili) of many electron film-shaped particles. Nonbonding n1, n2 → π* electron transitions (≤ 3.0 eV) at N/O mediate to coherently excite p-GNO to its π → π* excited states (5.0 eV) via an up-energy conversion. That lead to separate the electron-hole ‘e−–h+’ pairs so to degrade the pollutants at the redox reactions. The p-GNO exhibits a prominent (002) XRD peak as it consists of (002) sp2-C layers of thin films (2 −5 nm thickness). Two allotropes coexist − one ρc = 2.11 g/cm3 density and other a higher ρc = 2.41 g/cm3, at atomic arrays twisted at the pores at 2 → 5 nm sizes (335.2 m2/g surface area). Small twins are shown at a 2−5 nm scale at the HRTEM images, with atomic thin interfaces at 3 → 25° slips. As tested at two pollutants methylene blue (MB) and 2-chlorophenol (2-CP), as much as 92.5% (87.5 % at 2-CP) ‘degradation removal efficiency’ is obtained at a 3.1 × 10−3 min−1 rate for MB under the identical conditions. So, p-GNO exhibits better features over many high grade photocatalysts. The mechanism of energy-transfer is described with models at n1, n2 ↔ π* energy-conversions at harmonics in deep UV-visible regions. The results are useful to design and develop value aided sp2-C and related hybrids for adsorption, photocatalysis, photonics, and other applications.

Quantum nonlinear metasurfaces from dual arrays of ultracold atoms

Atoms in a sub-wavelength lattices have remarkable optical properties that have become of high scientific and technological significance. Here, we show how the coupling of light to more than a single atomic array can expand these perspectives into the domain of quantum nonlinear optics. While a single array transmits and reflects light in a largely linear fashion, the combination of two arrays is found to induce strong photon-photon interactions that can convert an incoming classical beam into highly antibunched light. Such quantum metasurfaces open up new possibilities for coherently generating and manipulating nonclassical light, from optical quantum information processing to exploring quantum many-body phenomena in two-dimensional systems of strongly interacting photons.

Multichannel waveguide QED with atomic arrays in free space

We study light scattering off a two-dimensional array of atoms driven to Rydberg levels. We show that the problem can be mapped to a generalized model of waveguide QED, consisting of multiple one-dimensional photonic channels (transverse modes), each of which is directionally coupled to a corresponding Rydberg surface mode of the array. In the Rydberg blockade regime, collective excitations of different surface modes block each other, leading to multichannel correlated photonic states. Using an analytical approach, we characterize interchannel quantum correlations, and elucidate the role of collective two-photon resonances of the array. Our results open new possibilities for multimode many-body physics and quantum information with photons in a free-space platform.

Simulating the generation of spin squeezing in a Rydberg atomic array for quantum metrology via a dissipative discrete truncated Wigner approximation

An atomic ensemble with many-body entanglement is desirable for precision measurement. As a type of such quantum state, the spin squeezed state has been pursued in both cold and warm atoms for applications of a quantum-enhanced atomic clock, interferometer, and magnetometer. Here, we report the numerical simulation of many-body dynamics in a Rydberg atomic array with dipole–dipole interaction, and evaluate the generation of spin squeezing. The method builds on the dissipative discrete truncated Wigner approximation, which combines the mean-field dynamics of a spin ensemble with Monte Carlo sampling. By taking into account experimental imperfections such as spin decoherence, we apply this approach to the dynamics in both strontium and rubidium Rydberg atomic arrays with the current available scale. This offers the possibility to accurately simulate the many-body dynamics of interacting quantum systems in achievable platforms for application of quantum simulation and quantum metrology.

Synthesis and Structural Studies of Complexes of Bis(pentafluorophenyl)mercury with Di(phosphane oxide) Ligands

The reaction of bis(pentafluorophenyl)mercury with the ligands bis(diphenylphosphano) methane P,P’-dioxide ({Ph2P(O)}2CH2) (1), bis{2-(N,N,N’N’-tetraethyldiaminophosphano) imidazol-1-yl} methane P,P’-dioxide ({2-PO(NEt2)2C3N2H2}2CH2) (2) and bis (2-diphenylphosphanophenyl) ether P,P’-dioxide ({2-PPh2(O)C6H4}2O) (3) afforded crystalline σ-donor complexes [{Hg(C6F5)2}2{Ph2P(O)}2CH2] (1Hg), [Hg(C6F5)2{2-PO(NEt2)2C3N2H2}2CH2]n (2Hg) and [Hg(C6F5)2{2-PPh2(O)C6H4}2O] (3Hg), respectively. The molecular structures of 1Hg, 2Hg and 3Hg show considerable differences. In complex 1Hg, a single bridging bidentate ligand connects two three-coordinate T-shape mercury atoms with a near linear C-Hg-C atom array. Complex 2Hg is a one-dimensional coordination polymer in which adjacent four-coordinate mercury atoms with a linear C-Hg-C atom array are linked by bridging bidentate O,O’- ligands, whilst in complex 3Hg a T-shape three-coordinate mercury atom is ligated by (3) in a monodentate fashion. The Hg-O bond lengths of complexes 1Hg, 2Hg and 3Hg differ substantially (range 2.5373(14)-2.966(3) Å) owing to structural and bonding differences.

Fully packed quantum loop model on the square lattice: Phase diagram and application for Rydberg atoms

The quantum dimer and loop models attract great attentions, partially because the fundamental importance in the phases and phase transitions emerging in these prototypical constrained systems, and partially due to their intimate relevance toward the on-going experiments on Rydberg atom arrays in which the blockade mechanism naturally enforces the local constraint. Here we show, by means of the sweeping cluster quantum Monte Carlo method, the complete ground state phase diagram of the fully packed quantum loop model on the square lattice. We find between the lattice nematic (LN) phase with strong dimer attraction and the staggered phase (SP) with strong dimer repulsion, there emerges a resonating plaquette (RP) phase with off-diagonal translational symmetry breaking. Such a quantum phase is separated from the LN via a first order transition and from the SP by the famous Rokhsar-Kivelson point. Our renormalization group analysis reveals the different flow directions, fully consistent with the order parameter histogram in Monte Carlo simulations. The realization and implication of our phase diagram in Rydberg experiments are proposed.

Parallel Assembly of Arbitrary Defect-Free Atom Arrays with a Multitweezer Algorithm

Defect-free atom arrays are a precursor for quantum information processing and quantum simulation with neutral atoms. Yet, large-scale defect-free atom arrays can be challenging to realize, due to the losses encountered when rearranging stochastically loaded atoms to achieve a desired target array. Here, we demonstrate a parallel rearrangement algorithm that uses multiple mobile tweezers to independently sort and compress atom arrays in a way that naturally avoids atom collisions. With a high degree of parallelism, our algorithm offers a reduced move complexity compared to both single-tweezer algorithms and existing multitweezer algorithms. We further determine the optimal degree of parallelism to be a balance between an algorithmic speedup and multitweezer inhomogeneity effects. The defect-free probability for a 225-atom array is demonstrated to be as high as 33(1)% in a room-temperature setup after multiple cycles of rearrangement. The algorithm presented here can be implemented for any target array geometry with an underlying periodic structure.Received 13 September 2022Revised 15 December 2022Accepted 19 January 2023DOI:https://doi.org/10.1103/PhysRevApplied.19.034048Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasCooling & trappingQuantum algorithmsQuantum information with atoms & lightQuantum simulationPhysical SystemsLatticesNanotechnologyTechniquesOptical tweezersAtomic, Molecular & OpticalQuantum InformationCondensed Matter, Materials & Applied Physics

Optical tweezers throw and catch single atoms

Single atoms movable from one place to another would enable a flying quantum memory that can be useful for dynamic quantum computing architectures. Guided atoms, e.g., by optical tweezers, provide a partial solution, but the benefit of flying qubits could be lost if they still interact with the guiding means. Here we propose and experimentally demonstrate freely flying atoms that are not guided but instead thrown and caught by optical tweezers. We provide a set of proof-of-principle flying atom demonstrations, which include atom transport through optical tweezers, atom arrangements by flying atoms, and atom scattering off optical tweezers. In experiments, cold rubidium atoms at 40 µK temperature are thrown by accelerating optical tweezers, freely fly with up to a speed of 0.65 m/s and free-flying distance of 4.2 µm, and are recaptured and stopped by decelerating optical tweezers at a transportation efficiency of 94(3)%. Flying atoms suggest possible applications such as defect correction in a tweezer trap atom array, fast atom-array formation, Rydberg-atom collision studies, and dynamic quantum computing architectures.

Robust phase-controlled gates for scalable atomic quantum processors using optical standing waves

A simple scheme is presented for realizing robust optically controlled quantum gates for scalable atomic quantum processors by driving the qubits with optical standing waves. Atoms localized close to the antinodes of the standing wave can realize phase-controlled quantum operations that are potentially more than an order of magnitude less sensitive to the local optical phase and atomic motion than corresponding travelling wave configurations. The scheme is compatible with robust optimal control techniques and spatial qubit addressing in atomic arrays to realize phase controlled operations without the need for tight focusing and precise positioning of the control lasers. This will be particularly beneficial for quantum gates involving Doppler sensitive optical frequency transitions and provides an all optical route to scaling up atomic quantum processors.