Argon Dark Matter Research Articles

Prospects for measuring the time variation of astrophysical neutrino sources at dark matter detectors

We study the prospects for measuring the time variation of solar and atmospheric neutrino fluxes at future large-scale xenon and argon dark matter detectors. For solar neutrinos, a yearly time variation arises from the eccentricity of Earth’s orbit and, for charged current interactions, from a smaller energy-dependent day-night variation due to flavor regeneration as neutrinos travel through Earth. For a 100-ton xenon detector running for ten years with a xenon-136 fraction of ≲0.1%, in the electron recoil channel a time-variation amplitude of about 0.8% is detectable with a power of 90% and the level of significance of 10%. This is sufficient to detect time variation due to eccentricity, which has amplitude of ∼3%. In the nuclear recoil channel, the detectable amplitude is about 10% under current detector resolution and efficiency conditions, and this generally reduces to about 1% for improved detector resolution and efficiency, the latter of which is sufficient to detect time variation due to eccentricity. Our analysis assumes both known and unknown periods. We provide scalings to determine the sensitivity to an arbitrary time-varying amplitude as a function of detector parameters. Identifying the time variation of the neutrino fluxes will be important for distinguishing neutrinos from dark matter signals and other detector-related backgrounds and extracting properties of neutrinos that can be uniquely studied in dark matter experiments. Published by the American Physical Society 2024

Study of low-energy nuclear recoils in liquid argon with the ReD experiment

Liquid Argon (LAr) Time Projection Chambers (TPC) operating in double-phase can detect the nuclear recoils (NR) possibly caused by the elastic scattering of WIMP dark matter particles via light signals from both scintillation and ionization processes. In the scenario of a low-mass WIMP (< 2 GeV/c2), the energy range for the NRs would be below 20 keV, thus making it crucial to characterize the ionization response in LAr TPCs as the lone available detection channel at such low energy. The Recoil Directionality (ReD) project, within the Global Argon Dark Matter Collaboration, aims to measure the ionization yield of a LAr TPC in the recoil energy range of 2–5 keV. The measurement was performed in winter 2023 at the INFN Sezione of Catania and the analysis is ongoing.

The DarkSide-20k experiment

The DarkSide-20k experiment represents the present goal of the Global Argon Dark Matter Collaboration program. Bringing together the experience from previous argon-based detectors, as well as the knowledge gained on large volume membrane cryostats developed within the DUNE program, the community is now building a dual-phase LAr-TPC equipped with SiPM arrays for light readout. The main goal of the experiment is to discover or to extend the current sensitivity limits on the search for dark matter WIMP-like particles. Currently, the experiment has entered the construction phase and the external cryostat is being put in place at Laboratori Nazionali del Gran Sasso (LNGS), Italy. Detector construction will follow, and data taking is expected to start in late 2026. This contribution will introduce the DarkSide detector and goals, and it will report on the ongoing construction of the underground infrastructure at LNGS. Finally, it will concentrate on the current activities on large arrays of silicon light detectors, that are at the base of the construction of the detector light readout system.

Directionality for nuclear recoils in a Liquid Argon TPC

Directional sensitivity to nuclear recoils would provide a smoking gun for a possible discovery of dark matter in the form of WIMPs (Weakly Interacting Massive Particles). A hint of directional dependence of the response of a dual-phase argon Time Projection Chamber (TPC) was found in the SCENE experiment. Given the potential importance of such a capability in the framework of dark matter searches, a new dedicated experiment, ReD (Recoil Directionality), was designed by the Global Argon Dark Matter Collaboration, in order to scrutinise this hint. A small dual-phase argon TPC was irradiated with neutrons produced by the p(7Li,7Be)n reaction using the 15 MV TANDEM accelerator of the INFN - Laboratori Nazionali del Sud, Catania, Italy, so as to produce argon nuclear recoils in the range (20 - 100) keV of interest for dark matter searches. Energy and direction of nuclear recoils are inferred by the detection of the elastically-scattered neutron by a set of scintillation detectors. Events were selected by gating of the associated 7Be, which is detected by a telescope of Si detectors.

Comparison of Different Detection Paradigm for WMIPs

Based on astrophysics observation, dark matter accounts for approximately 84% of all matter in the universe, with the remaining 16% being ordinary matter. According to the prevailing scientific model, dark matter particles are supersymmetric particles with a mass of 100 GeV (about the mass of 100 protons) with the density about 5000 particles m-3. Yet such a dominant substance dominates the universe, but one has not detected yet. Among various candidate, WIMPs are one of the most appealing one that plenty of facilities aim to detect. In this essay, the detection principles and some recent results of two representatives of the state-of-art mainstream detection methods were presented, i.e., the ‘Wukong’ astronomical satellite (DAMPE) and the Jinping Mountains of Sichuan Province, China (CJPL). It was shown that ‘Wukong’ has successfully detected an electron-positron pairs at an energy of 0.9 Tev. In Jinping, experiments are proposed to detect liquid argon dark matter. In this review, the two methods of detecting dark matter will be compared and the advantages, disadvantages will be analyzed. These results shed light on guiding further exploration of dark matter.

The Recoil Directionality (ReD) Experiment

Directional sensitivity to nuclear recoils would provide a smoking gun for a possible discovery of dark matter in the form of WIMPs (Weakly Interacting Massive Particles). A hint of directional dependence of the response of a dual-phase argon Time Projection Chamber (TPC) was found in the SCENE experiment. Given the potential importance of such a capability in the framework of dark matter searches, a new dedicated experiment, ReD (Recoil Directionality), was designed by the Global Argon Dark Matter Collaboration, in order to scrutinize this hint. Prior to the irradiation with a neutron beam, the ReD TPC underwent a long campaign of characterization and optimization: some selected results are presented in this contribution.

Atmospheric neutrinos in next-generation xenon and argon dark matter experiments

We study the sensitivity of future xenon- and argon-based dark matter and neutrino detection experiments to low-energy atmospheric neutrinos. Not accounting for experimental backgrounds, the primary obstacle for identifying nuclear recoils induced by atmospheric neutrinos is the tail of the electron recoil distribution due to $pp$ solar neutrinos. We use the NEST code to model the solar and atmospheric neutrino signals in a xenon detector and find that an exposure of 700 tonne-years will produce a $5\sigma$ detection of atmospheric neutrinos. We explore the effect of different detector properties and find that a sufficiently long electron lifetime is essential to the success of such a measurement.

Status of the DEAP-3600 experiment

DEAP-3600 is a single-phase liquid argon (LAr) dark matter detector, located 2 km underground at SNOLAB in Sudbury, Canada, which started taking data in 2016. The detector is sensitive to nuclear recoils induced by scattering of dark matter particles, which would cause emission of prompt scintillation light. DEAP-3600 demonstrated excellent performance, holds the leading WIMP exclusion among LAr detectors, and published several physics results. The WIMP sensitivity of the detector is currently limited by backgrounds induced by alpha activity at the LAr inlet, in a shadowed region of detector. The ongoing hardware upgrade aims at fixing that limitation and, in consequence, at reaching the full WIMP sensitivity. This paper summarizes the latest results from DEAP-3600 and details of the upgrade.

Position reconstruction using photon timing for the DEAP-3600 dark matter experiment

DEAP-3600 is a single-phase liquid argon dark matter detector being operated 2 km underground at SNOLAB, Sudbury, Canada. The detector consists of 3.3 tonnes of ultra-pure liquid argon in a spherical acrylic cryostat instrumented with 255 photomultiplier tubes. Natural radioactive contamination in the acrylic vessel or TPB wavelength shifter can alpha-decay. Reconstruction of the position of the interactions taking place in the detector uses information about the number of photoelectrons detected in each PMT and when they were detected. Including this information in our suite of cuts allows us to identify and remove almost all surface background events. A method of event position reconstruction emphasizing photon timing is presented here.

Technique for surface background rejection in liquid argon dark matter detectors using layered wavelength-shifting and scintillating thin films

A technique using layered wavelength shifting, scintillating and non-scintillating films is presented to achieve discrimination of surface α events from low-energy nuclear recoils in liquid argon detectors. A discrimination power greater than 108, similar to the discrimination possible for electronic recoils in argon, can be achieved by adding a 50μm layer of scintillator with a suitably slow decay time, approximately 300 ns or greater, to a wavelength-shifter coated surface. The technique would allow suppression of surface α events in a very large next-generation argon dark matter experiment (with hundreds of square meters of surface area) without the requirement for position reconstruction, thus allowing utilization of more of the instrumented mass in the dark matter search. The technique could also be used to suppress surface backgrounds in compact argon detectors of low-energy nuclear recoils, for example in measurements of coherent neutrino–nucleus scattering or for sensitive measurements of neutron fluxes.

DArT, a detector for measuring the 39Ar depletion factor

One of the most powerful techniques for direct detection of dark matter via elastic scattering of galactic WIMPs is the use of liquid argon time projection chambers. Atmospheric argon (AAr) has a naturally occurring radioactive isotope, 39Ar, of cosmogenic origin. The use of argon extracted from underground wells, deprived of 39Ar, is key to the physics potential of these experiments. The DarkSide-20k (DS-20k) dark matter search experiment will operate with 50 tonnes of radio-pure underground argon (UAr), extracted from the Urania plant in Cortez (U.S.A.) and purified in the Aria distillation plant (Sardinia, Italy). Assessing the radio-purity of UAr in terms of 39Ar is crucial for the success of DS-20k, as well as for future experiments of the Global Argon Dark Matter Collaboration (GADMC), and will be done with the experiment named DArT in ArDM. DArT is a small chamber that will contain the argon under test. The detector will be immersed in the LAr active volume of the ArDM detector, located at the Canfranc Underground Laboratory (LSC) in Spain, which will act as active veto for background events coming from photons from detector materials and surrounding rock radioactivity.

Design and construction of a new detector to measure ultra-low radioactive-isotope contamination of argon

Large liquid argon detectors offer one of the best avenues for the detection of galactic weakly interacting massive particles (WIMPs) via their scattering on atomic nuclei. The liquid argon target allows exquisite discrimination between nuclear and electron recoil signals via pulse-shape discrimination of the scintillation signals. Atmospheric argon (AAr), however, has a naturally occurring radioactive isotope, 39Ar, a β emitter of cosmogenic origin. For large detectors, the atmospheric 39Ar activity poses pile-up concerns. The use of argon extracted from underground wells, deprived of 39Ar, is key to the physics potential of these experiments. The DarkSide-20k dark matter search experiment will operate a dual-phase time projection chamber with 50 tonnes of radio-pure underground argon (UAr), that was shown to be depleted of 39Ar with respect to AAr by a factor larger than 1400. Assessing the 39Ar content of the UAr during extraction is crucial for the success of DarkSide-20k, as well as for future experiments of the Global Argon Dark Matter Collaboration (GADMC). This will be carried out by the DArT in ArDM experiment, a small chamber made with extremely radio-pure materials that will be placed at the centre of the ArDM detector, in the Canfranc Underground Laboratory (LSC) in Spain. The ArDM LAr volume acts as an active veto for background radioactivity, mostly γ-rays from the ArDM detector materials and the surrounding rock. This article describes the DArT in ArDM project, including the chamber design and construction, and reviews the background required to achieve the expected performance of the detector.

Triplet lifetime in gaseous argon

MiniCLEAN is a single-phase liquid argon dark matter experiment. During the initial cooling phase, impurities within the cold gas ($<$140 K) were monitored by measuring the scintillation light triplet lifetime, and ultimately a triplet lifetime of 3.480 $\pm$ 0.001 (stat.) $\pm$ 0.064 (sys.) $\mu$s was obtained, indicating ultra-pure argon. This is the longest argon triplet time constant ever reported. The effect of quenching of separate components of the scintillation light is also investigated.

Directional modulation of electron-ion pairs recombination in liquid argon

Motivated by the ongoing study of a possible directional signal in liquid argon dark matter detectors, we introduce a new model describing the recombination of electron-ion pairs in ionizing tracks in liquid argon in the presence of a drift field. The emphasis is on the three-dimensional distribution of electrons and ions and on their orientation relative to that of the electric field. We successfully apply our model to describe the angular dependence of the ionization signal of protons recently reported in measurements performed by the ArgoNeuT Collaboration with a liquid argon time projection chamber.

First measurement of surface nuclear recoil background for argon dark matter searches

One major background in direct searches for weakly interacting massive particles (WIMPs) comes from the deposition of radon progeny on detector surfaces. The most dangerous surface background is the $^{206}$Pb recoils produced by $^{210}$Po decays. In this letter, we report the first characterization of this background in liquid argon. The scintillation signal of low energy Pb recoils is measured to be highly quenched in argon, and we estimate that the 103keV $^{206}$Pb recoil background will produce a signal equal to that of a ~5keV (30keV) electron recoil ($^{40}$Ar recoil). In addition, we demonstrate that this dangerous $^{210}$Po surface background can be suppressed by a factor of ~100 or higher using pulse shape discrimination methods, which can make argon dark matter detectors near background-free and enhance their potential for discovery of medium- and high-mass WIMPs. We also discuss the impact on other low background experiments.

Commissioning of the ArDM experiment at the Canfranc underground laboratory: first steps towards a tonne-scale liquid argon time projection chamber for Dark Matter searches

The Argon Dark Matter (ArDM) experiment consists of a liquid argon (LAr) time projection chamber (TPC) sensitive to nuclear recoils, resulting from scattering of hypothetical Weakly Interacting Massive Particles (WIMPs) on argon targets. With an active target mass of 850 kg ArDM represents an important milestone towards developments for large LAr Dark Matter detectors. Here we present the experimental apparatus currently installed underground at the Laboratorio Subterráneo de Canfranc (LSC), Spain. We show data on gaseous or liquid argon targets recorded in 2015 during the commissioning of ArDM in single phase at zero E-field (ArDM Run I). The data confirms the overall good and stable performance of the ArDM tonne-scale LAr detector.

Improving photoelectron counting and particle identification in scintillation detectors with Bayesian techniques

Many current and future dark matter and neutrino detectors are designed to measure scintillation light with a large array of photomultiplier tubes (PMTs). The energy resolution and particle identification capabilities of these detectors depend in part on the ability to accurately identify individual photoelectrons in PMT waveforms despite large variability in pulse amplitudes and pulse pileup. We describe a Bayesian technique that can identify the times of individual photoelectrons in a sampled PMT waveform without deconvolution, even when pileup is present. To demonstrate the technique, we apply it to the general problem of particle identification in single-phase liquid argon dark matter detectors. Using the output of the Bayesian photoelectron counting algorithm described in this paper, we construct several test statistics for rejection of backgrounds for dark matter searches in argon. Compared to simpler methods based on either observed charge or peak finding, the photoelectron counting technique improves both energy resolution and particle identification of low energy events in calibration data from the DEAP-1 detector and simulation of the larger MiniCLEAN dark matter detector.

Characterization of the R5912-02 MOD photomultiplier tube at cryogenic temperatures

Hamamatsu's R5912-02 MOD is an 8 inch diameter cryogenic photomultiplier tube of interest for light detection in large liquid noble dark matter and neutrino detectors. The R5912-02 MOD will be used in the MiniCLEAN single phase liquid argon dark matter detector and has been tested and characterized at cryogenic temperatures in the single photoelectron regime. A detailed model of the single photoelectron timing properties, pulse shape, and charge distribution will be described. The model extracts these parameters from fits to the unique multi-component timing structure of the R5912-02 MOD pulses.

Study of nuclear recoils in liquid argon with monoenergetic neutrons

In the framework of developments for liquid argon dark matter detectors we assembled a laboratory setup to scatter neutrons on a small liquid argon target. The neutrons are produced mono-energetically (Ekin = 2.45 MeV) by nuclear fusion in a deuterium plasma and are collimated onto a 3" liquid argon cell operating in single-phase mode (zero electric field). Organic liquid scintillators are used to tag scattered neutrons and to provide a time-of-flight measurement. The setup is designed to study light pulse shapes and scintillation yields from nuclear and electronic recoils as well as from alpha particles at working points relevant for dark matter searches. Liquid argon offers the possibility to scrutinise scintillation yields in noble liquids with respect to the population strength of the two fundamental excimer states. Here we present experimental methods and first results from recent data towards such studies.

Depleted Argon from Underground Sources

Argon is a powerful scintillator and an excellent medium for detection of ionization. Its high discrimination power against minimum ionization tracks, in favor of selection of nuclear recoils, makes it an attractive medium for direct detection of WIMP dark matter. However, cosmogenic 39Ar contamination in atmospheric argon limits the size of liquid argon dark matter detectors due to pile-up. The cosmic ray shielding by the earth means that Argon from deep underground is depleted in 39Ar. In Cortez Colorado a CO2 well has been discovered to contain approximately 500 ppm of argon as a contamination in the CO2. In order to produce argon for dark matter detectors we first concentrate the argon locally to 3-5% in an Ar, N2, and He mixture, from the CO2 through chromatographic gas separation. The N2 and He will be removed by continuous cryogenic distillation in the Cryogenic Distillation Column recently built at Fermilab. In this talk we will discuss the entire extraction and purification process; with emphasis on the recent commissioning and initial performance of the cryogenic distillation column purification.