Aqueous Mineral Carbonation Research Articles

Direct aqueous mineral carbonation of secondary materials for carbon dioxide storage

Mineral carbonation of secondary materials offers an innovative way of storing carbon dioxide in materials that instead would mostly go to waste. This study investigates the carbonation efficiency (CE) of 11 different secondaries from refractory production, waste incineration, and the paper industry compared to untreated and thermally activated serpentinite. To determine the chemical and mineralogical composition of the materials, various analytical methods, like X-ray fluorescence, X-ray diffraction, scanning electron microscopy, Brunauer-Emmet-Teller and thermogravimetric analysis have been employed, both before and after the direct aqueous carbonation process. Each material was examined over reaction times of 6 & 10 hours at 180 °C and a starting pressure of 20 bar in a 0.6 L stainless steel batch reactor. The received results were then compared to the theoretical CO2 uptake, defined as the maximum carbon dioxide storage potential achievable if all Ca, Fe and Mg ions were converted to carbonates. The findings indicate carbonation efficiencies of 14–65 % for secondary materials, compared to 0.7–14 % observed in the serpentinite samples. The highest uptakes were achieved by the refractory materials, primarily due to their high metal oxide content. However, a negative impact was observed from graphite-based carbon binders in the refractories, with increased leaching of these binders leading to a decrease in carbonation efficiency. Materials with higher SiO2 content showed reduced performance, suggesting a passivation layer buildup during carbonation.

Enhancing aqueous carbonation via co-milled serpentine and wollastonite: Effects of mechanochemical activation

Carbon dioxide (CO2) storage through aqueous mineral carbonation is recognized as a promising technology for geochemical carbon removal. Previous studies predominantly focused on individual alkaline earth silicates, such as wollastonite or serpentine, overlooking their interactive effects on carbonation processes. To address this knowledge gap, we conducted aqueous carbonation tests using individually ball-milled serpentine (m-serpentine), wollastonite (m-wollastonite), mixtures of ball-milled serpentine and wollastonite (m-serpentine + m-wollastonite), and the co-milled serpentine and wollastonite (m-(serpentine + wollastonite)). The carbonation of (m-serpentine + m-wollastonite) involved the formation of a combination of calcite (CaCO3) and magnesite (MgCO3), suggesting that no significantly interactive effect between the serpentine and wollastonite. In contrast, carbonating m-(serpentine + wollastonite) results in the precipitation of Mg-bearing calcite ((Mg, Ca)CO3). Upon quantification, the carbonation degrees of m-(serpentine + wollastonite) is relatively higher than that of (m-serpentine + m-wollastonite). During the carbonation of m-(serpentine + wollastonite), the combination of serpentine and wollastonite facilitates mutual dissolution, leading to the release of more cations. However, these released ions do not diffuse into the bulk carbonating solution; instead, carbonation occurs exclusively at the mineral-water interface. Consequently, the co-milling process, merging Ca-rich wollastonite into Mg-rich serpentine, induces the formation of (Mg, Ca)SiO3. These novel insights into aqueous carbonation using a combination of Mg-containing and Ca-containing minerals underscore the significant role of mineral-mineral reactions in CO2 mineralization.

Aqueous mineral carbonation of three different industrial steel slags: Absorption capacities and product characterization

Heavy carbon industries produce solid side stream materials that contain inorganic chemicals like Ca, Na, or Mg, and other metals such as Fe or Al. These inorganic compounds usually react efficiently with CO2 to form stable carbonates. Therefore, using these side streams instead of virgin chemicals to capture CO2 is an appealing approach to reduce CO2 emissions. Herein, we performed an experimental study of the mineral carbonation potential of three industrial steel slags via aqueous, direct carbonation. To this end, we studied the absorption capacities, reaction yields, and physicochemical characteristics of the carbonated samples. The absorption capacities and the reaction yields were analyzed through experiments carried out in a reactor specifically designed to work without external stirring. As for the physicochemical characterization, we used solid-state Fourier Transform Infrared Spectroscopy (FTIR), X-ray diffraction (XRD), and scanning electron microscope (SEM). Using this reactor, the absorption capacities were between 5.8 and 35.3 g/L and reaction yields were in the range of 81–211 kg CO2/ton of slag. The physicochemical characterization of the solid products with solid FTIR, XRD and SEM indicated the presence of CaCO3. This suggests that there is potential to use the carbonated products in commercial applications.

Elution of Divalent Cations from Iron Ore Mining Waste in an Indirect Aqueous Mineral Carbonation for Carbon Capture and Storage

Mining waste is generated in vast quantities globally, which can have negative environmental consequences. This study highlights the utilization of iron ore mining waste as feedstock material in the preparatory step of an indirect aqueous mineral carbonation for carbon sequestration. The role of reactive cations (Ca2+, Mg2+, and Fe2+) was investigated in view of their elution behavior to improve carbonation efficiency. An elution experiment was carried out for the divalent cations using different acids (oxalic, HCl, acetic, and formic acid) at different concentration solutions (up to 1.5 M) and times (up to 100 min) at ambient temperature. The initial analysis confirmed the presence of divalent cations in the sample. The elution approach at ambient temperature resulted in the elution efficiency of Fe2+ (30.4%), Mg2+ (54%) using oxalic acid, and Ca2+ (98%) using HCl at a relatively short time between 50 and 100 min. It was found that for the iron ore mining waste, oxalic acid and HCl were best suited as elution agents for the Fe2+ and Mg2+, and Ca2+, respectively. The CO2 sequestration potential was calculated to be 131.58 g CO2/kg residue. A further carbonation step using a complexing agent (1,10 phenanthroline) confirmed the formation of siderite and magnesite along with phenanthroline hydrates. Findings have shown that the indirect mineral carbonation of the iron mining waste with complexing agent might improve carbonation efficiency, thus indicating that this material is useful for long-term carbon capture and storage applications.

Indirect Aqueous Mineral Carbonation of Samples of Linz–Donawitz Slag from the Steel Industry in Eastern India

Indirect Aqueous Mineral Carbonation of Samples of Linz–Donawitz Slag from the Steel Industry in Eastern India

Enhancing Aqueous Carbonation of Calcium Silicate through Acid and Base Pretreatments with Implications for Efficient Carbon Mineralization.

Carbon dioxide (CO2) mineralization based on aqueous carbonation of alkaline earth silicate minerals is a promising route toward large-scale carbon removal. Traditional aqueous carbonation methods largely adopt acidification-based approaches, e.g., using concentrated/pressurized CO2 or acidic media, to accelerate mineral dissolution and carbonation. In this study, we designed and tested three distinctive routes to evaluate the effect of pretreatments under different pH conditions on aqueous carbonation, using amorphous calcium silicate (CS) as an example system. Pretreating CS with high concentrations (100 mM) of HCl (Route I) or NaOH (Route II and III) enhanced their carbonation degrees. However, NaOH pretreatment overall yielded higher carbonation degrees than the HCl pretreatment, with the highest carbonation degree achieved through Route III, where an extra step is taken after the NaOH pretreatment to remove the solution containing dissolved silica prior to carbonation. The HCl and NaOH pretreatments formed different intermediate silica products on the CS surface. Silica precipitated from the HCl pretreatment had a minimal effect on the carbonation degree. The high Ca/Si ratio intermediate phases formed from the NaOH, on the other hand, can be readily carbonated. In contrast to commonly utilized acidification-based approaches, basification offers a more promising route to accelerate aqueous carbonation as it can mitigate the need for costly pH swing and high-concentration/pressurized CO2. The key to aqueous carbonation under basic conditions, as suggested by this study, is the control of aqueous silica species that have a suppressing effect on carbonation. Overall, this study highlights the critical needs for investigations of aqueous mineral carbonation in a broader pH region.

Direct aqueous mineral carbonation of carbide slag in a bubble column reactor under ambient conditions

The accelerated carbonation technology utilizing the alkaline minerals or alkaline wastes incurs high operation and investment costs low conversion efficiency and high energy consumption. Due to the strong alkalinity of the carbide slag, good feedstock availability and great performance of the bubble column reactor, the direct aqueous mineral carbonation of the carbide slag in a bubble column at ambient conditions is evaluated. The impact mechanism of the liquid to solid ratio (5 mL/g−50 mL/g) and gas velocity (0.0041 m/s−0.205 m/s) on the reactions are investigated. The flow patterns are identified by empirical mode decomposition (EMD) energy entropy, and carbonation efficiencies at different flow regimes are compared and illustrated. It is found that this route has a high carbonation efficiency and short reaction time. The maximum carbonation efficiency is 100% and the capture capacity is 214.05 g CO2 / kg carbide slag. The discrete bubble regime (DBR) and bubble coalescence regime (BCR) are observed, and the increase of the L/S ratio can promote the bubble coalescence. The hydrodynamics can influence the processes of the CO2 mass transfer from gas to liquid phase, Ca(OH)2 dissolution, reactant diffusion, collision and ionic reactions. At small L/S ratio, the greater carbonation efficiency is achieved in discrete bubble regime attributing to the longer gas residence time, larger gas–liquid interfacial area and better CO2 mass transfer than that in BCR. At large L/S ratio, the greater carbonation efficiencies are achieved both in DBR and BCR. It has good CO2 mass transfer in DBR and has the strong liquid turbulence intensity in BCR which is good for the reactant diffusion and collision. The enhancement factor increases when enhancing the L/S ratio in DBR. The 30 mL/g and the gas velocity operated in the discrete bubble regime are recommended considering the better three-phase contact, good carbonation conversion and low energy consumption.

Kinetic analysis on CO2 sequestration from flue gas through direct aqueous mineral carbonation of circulating fluidized bed combustion fly ash

In this work, the suitability of fly ash from 600 MW circulating fluidized bed boiler for CO2 sequestration through direct aqueous route was evaluated. The circulating fluidized bed combustion fly ash exhibited favorable carbon capture characteristics with a maximum CO2 sequestration capacity of 0.128 g CO2/g CFA and a corresponding carbonation efficiency of 78.17 %. A modified shrinking core model incorporated gaseous CO2 dissolution and time-dependent effective coefficient of internal diffusion was proposed to determine the gas–liquid-solid carbonation kinetics. The key kinetic parameters were assessed as a function of various carbonation conditions including reaction temperature, solid–liquid (S/L) ratio, energy input and superficial gas velocity. The mass diffusion through the liquid film near the gas–liquid interface was the rate-controlling step during the initial period of time, while diffusion through the expanded passivation layer constituted the controlling mechanism at the final stage. The model provides a more accurate representation of the gas–liquid-solid carbonation process and can be generalized to describe the carbonation of other solid wastes of interest.

Mineral carbonation of New Caledonian ultramafic mine slag: Effect of glass and secondary silicates on the carbonation yield

New Caledonian nickel (Ni) mines produces ∼12 million metric tons of mine slag every year, that are considered undesired and uneconomic waste materials. However, due to the high content of Mg2+ and Fe2+, these slags exhibit a potential of carbon dioxide (CO2) storage by ex-situ aqueous mineral carbonation. We conducted laboratory batch experiments at 200 °C/ 150 bar, 250 °C/ 300 bar, 300 °C/ 300 bar, in CO2-saturated water to better understand the slag dissolution, secondary mineral formation at the fluid-mineral interface, and the effect of the secondary silicates on the carbonation yield. The slag contains olivine (45 wt%) and glass (55 wt%). Olivine in the slag dissolves faster than glass, contributing to carbonate precipitation (Fe-rich magnesite) at 200 °C/150 bar. At 250 °C/ 300 bar, olivine is almost completely dissolved while glass dissolves only partially, both contributing to the highest recorded carbonation yields of the slag of 44 wt%. Although both olivine and glass are completely dissolved at 300 °C/ 300 bar, the carbonate yield drops at a value half of that at 250 °C/ 300 bar. This is due to formation of large quantity of Mg-bearing phyllosilicates that reduces the amount of Mg2+ available for carbonation. These results emphasize that increasing temperature above 250 °C would not increase the carbonate yield of New Caledonian mine slags. However, as glass only partially reacts at T < 250 °C, mobilizing Mg2+ in glass could potentially increase the carbonation yield, for example by adding suitable organic ligands. Mg-bearing phyllosilicates and amorphous silica that are formed in these experiments do not exhibit passivation properties, and therefore do not affect the carbonation rate.

Evaluation of the kinetics of direct aqueous mineral carbonation of wood combustion ash using modified shrinking core models.

The direct aqueous mineral carbonation of wood combustion ash (WCA), which is a representative high-calcium waste from combustion process, was systematically investigated by varying complex operating conditions, including reaction time, liquid-to-solid ratio (L/S), CO2 concentration, and particle size. The WCA exhibited high CO2 sequestration characteristics with an optimal carbonation efficiency of 76.4%, corresponding to a CO2 sequestration capacity of 0.314g CO2/g WCA. In addition to solid carbonates, dry residues from liquid products with high potassium contents are potential feedstocks for quality potash fertilizer. Modified shrinking core models based on diffusion-controlled mechanism were proposed to evaluate the carbonation process. The theoretical framework assumes a contracting interface mechanism where active CaO reacts with CO2 to form a product layer. The effective diffusion coefficient of CO2 through the product layer decreases over time, giving deficient carbonation efficiency. The newly proposed models corresponding to different geometrical dimensions provided more perfect fit to the experimental data when compared with the most commonly used kinetic equations. The low apparent activation energy of the carbonation reaction demonstrated the diffusion-controlled mechanism. This work is useful for improving the economics and feasibility of bioenergy carbon capture and storage (CCS) technology chain.

Carbon dioxide sequestration of iron ore mining waste under low-reaction condition of a direct mineral carbonation process.

Mining waste that is rich in iron-, calcium- and magnesium-bearing minerals can be a potential feedstock for sequestering CO2 by mineral carbonation. This study highlights the utilization of iron ore mining waste in sequestering CO2 under low-reaction condition of a mineral carbonation process. Alkaline iron mining waste was used as feedstock for aqueous mineral carbonation and was subjected to mineralogical, chemical, and thermal analyses. A carbonation experiment was performed at ambient CO2 pressure, temperature of 80°C at 1-h exposure time under the influence of pH (8-12) and particle size (< 38-75µm). The mine waste contains Fe-oxides of magnetite and hematite, Ca-silicates of anorthite and wollastonite and Ca-Mg-silicates of diopside, which corresponds to 72.62% (Fe2O3), 5.82% (CaO), and 2.74% (MgO). Fe and Ca carbonation efficiencies were increased when particle size was reduced to < 38µm and pH increased to 12. Multi-stage mineral transformation was observed from thermogravimetric analysis between temperature of 30 and 1000°C. Derivative mass losses of carbonated products were assigned to four stages between 30-150°C (dehydration), 150-350°C (iron dehydroxylation), 350-700°C (Fe carbonate decomposition), and 700-1000°C (Ca carbonate decomposition). Peaks of mass losses were attributed to ferric iron reduction to magnetite between 662 and 670°C, siderite decarbonization between 485 and 513°C, aragonite decarbonization between 753 and 767°C, and calcite decarbonization between 798 and 943°C. A 48% higher carbonation rate was observed in carbonated products compared to raw sample. Production of carbonates was evidenced from XRD analysis showing the presence of siderite, aragonite, calcite, and traces of Fe carbonates, and about 33.13-49.81g CO2/kg of waste has been sequestered from the process. Therefore, it has been shown that iron mining waste can be a feasible feedstock for mineral carbonation in view of waste restoration and CO2 emission reduction.

Aqueous carbonation of peridotites for carbon utilisation: a critical review.

Peridotite and serpentinites can be used to sequester CO2 emissions through mineral carbonation. Olivine dissolution rate is directly proportional with temperature, presence of CO2, surface area of mineral particles and presence of ligands and is inversely proportional to pH. Olivine dissolution is better under air flow and increases seven times when rock-inhibiting fungus (Knufia petricola) is used. Olivine dissolution retards as silica layers form during reaction. Sonication, acoustic and concurrent grinding using various grinding medias have been used to artificially break these silica layers and achieve high magnesium extraction. Wet grinding using 50 wt.% ethanol enhanced CO2 uptake of dunite 6.9 times and CO2 uptake of harzburgite by 4.5 times. The best economical process is single-stage concurrent grinding at 130 bar, 185 °C, 15 wt.% solids and 50 wt.% grinding media (zirconia) using 0.64 M NaHCO3. Ratio of grinding media to feed should not be less than 3:1. Yield increases with temperature, pressure, time of reaction, pH and rpm and using additives and grinding media and reducing particle size. This review aims to investigate the progress from 1970s to 2021 on aqueous mineral carbonation of olivine and its naturally available rocks (harzburgite and dunite). This paper comprehensively reviews all aspects of olivine carbonation including olivine dissolution kinetics, effects of grinding and concurrent grinding, thermal activation of olivine feedstock (dunites and harzburgites) as well as chemistry of olivine mineral carbonation. The effects of different reaction parameters on the carbonation yield, role of mineral carbonation accelerators and costs of mineral carbonation process are discussed.

Carbon mineralization with concurrent critical metal recovery from olivine

Carbon dioxide utilization for enhanced metal recovery (EMR) during mineralization has been recently developed as part of CCUS (carbon capture, utilization, and storage). This paper describes fundamental studies on integrating CO2 mineralization and concurrent selective metal extraction from natural olivine. Nearly 90% of nickel and cobalt extraction and mineral carbonation efficiency are achieved in a highly selective, single-step process. Direct aqueous mineral carbonation releases Ni2+ and Co2+ into aqueous solution for subsequent recovery, while Mg2+ and Fe2+ simultaneously convert to stable mineral carbonates for permanent CO2 storage. This integrated process can be completed in neutral aqueous solution. Introduction of a metal-complexing ligand during mineral carbonation aids the highly selective extraction of Ni and Co over Fe and Mg. The ligand must have higher stability for Ni-/Co- complex ions compared with the Fe(II)-/Mg- complex ions and divalent metal carbonates. This single-step process with a suitable metal-complexing ligand is robust and utilizes carbonation processes under various kinetic regimes. This fundamental study provides a framework for further development and successful application of direct aqueous mineral carbonation with concurrent EMR. The enhanced metal extraction and CO2 mineralization process may have implications for the clean energy transition, CO2 storage and utilization, and development of new critical metal resources.

Direct Air Capture and Sequestration of CO2 by Accelerated Indirect Aqueous Mineral Carbonation under Ambient Conditions

Mineralization of gaseous carbon dioxide into solid carbonates using alkaline industrial residues such as coal fly ash has a dual advantage of reducing the carbon dioxide footprint of coal power plants and improving ash utilization. However, the slow mineral carbonation rate under atmospheric conditions is a major challenge, especially when using natural minerals or industrial residues for direct air capture (DAC) of CO2. In this study, using coal fly ash samples and concentrated alkali carbonate aqueous solutions as a recyclable solvent, we show the feasibility of coupling mineral carbonation with DAC under atmospheric conditions. Findings show that carbonation efficiency is best under alkaline conditions, achieving as high as ∼80% conversion to calcium carbonates within 1 h in a 1.9 M sodium carbonate solution. Based on the experimental results, a process coupling DAC and mineral carbonation that operates entirely under ambient conditions is proposed. The techno-economic and life cycle assessments for the proposed process project a levelized cost of $116–133/t-CO2-sequestered (US $2019) and process carbon emissions (GWP) in the range of 0.03–0.25 t-CO2e/t-CO2-sequestered. Considering the low cost, simplicity, and gigaton-scale sequestration potential, we believe that DAC based on alkaline industrial residue carbonation can be considered a “low-hanging fruit” in the pursuit of negative emissions to combat climate change.

Glycine-induced synthesis of vaterite by direct aqueous mineral carbonation of desulfurization gypsum

Glycine-induced synthesis of vaterite by direct aqueous mineral carbonation of desulfurization gypsum

Characteristics of carbide slag slurry flow in a bubble column carbonation reactor

Abstract The direct aqueous mineral carbonation of carbide slag was investigated. The flow characteristics of carbide slag-CO2-water reaction system in a bubble column were studied, which included the bubble Sauter mean diameter, gas holdup, bubble residence time, and the gas-liquid interfacial area. Bubble flow behaviors in the reactor were characterized by analyzing the bed pressure signals. The effects of the gas velocity (U g ) and liquid to solid ratio (L/S ratio) were discussed and analyzed. The results showed that the larger bubbles were easy to form at the larger L/S ratio, which indicated that the bubble coalescence was promoted. The gas holdup was larger when increasing U g or reducing the L/S ratio. The better gas-liquid interfacial areas were found in a wide range of L/S ratio at U g = 0.082 m/s. The optimum conditions were found at U g = 0.082 m/s and L/S ratio = 15–30 mL/g for the better gas-liquid interfacial area and the higher carbide slag conversion. The work provided the theoretical basis for the direct aqueous carbonation of the carbide slag and the operation condition optimization.

Kinetic modeling of direct aqueous mineral carbonation using carbide slag in a stirred tank reactor

Direct aqueous mineral carbonation by carbide slag at various temperatures, power inputs, superficial gas velocities, and CO2 partial pressures in a stirred tank reactor were systematically studied. Based on the Two-Film Theory, a novel kinetic model that exhibited extraordinary agreement with the experimental data was proposed to express the relationship between carbonation efficiency and reaction time. Carbonation efficiencies of more than 90% were achieved in all the experiments. The rate-controlling step of the reaction was gas-liquid mass transfer initially, although solid-liquid mass transfer was the rate-controlling step at the final stage. Changes in the mineralogy and morphology of the carbide slag before and after carbonation confirmed the reaction mechanism. The effect of various operating parameters on gas-liquid mass transfer was quantitatively investigated using an empirical equation. The present study contributes to the large-scale, rational utilization of energy, operation optimization of CO2 mineral carbonation in gas-liquid-solid reaction systems.

Application of concurrent grinding in direct aqueous carbonation of magnesium silicates

Formation of silica-rich passivation layers formed on the periphery of reacting feed particles is one of the primary obstacles in obtaining high magnesite yields during direct aqueous mineral carbonation of peridotites and serpentinites. The disruption of the silica-rich layer around partially reacted grains as a result of concurrent grinding on the degree of carbonation (magnesite yield) was investigated in this work. Three types of naturally-occurring magnesium silicate feedstocks, dunite, olivine and lizardite, as well as three types of grinding media, were examined.Discrete size fractions of feed samples, with and without grinding media, were carbonated. SEM readily disclosed the formation of a silica-rich shell around a magnesium rich core during carbonation. EDS analysis was employed to study the elemental composition of reacted particles’ shell and core. The method confirmed that during concurrent grinding these silica-rich layers were removed and continuously produced a fresh surface available for further reaction. The removal of the silica-rich layer was shown to significantly improve magnesite yields up to a 600 % increase in yield. Among the three different grinding media used in this work, zirconia and stainless steel media resulted in similar and highest magnesite yields, which is believed to be due to a combination of their high densities and hardness. The findings of this research showed that enhanced magnesite yields could be achieved for all feedstock without the need for energy intensive pre-treatment steps (e.g. ultrafine grinding and heat-activation). Moreover, concurrent grinding resulted in a magnesite yield when raw lizardite was carbonated.

Feasibility of a Mineral Carbonation Technique Using Iron-Silicate Mining Waste by Direct Flue Gas CO2 Capture and Cation Complexation Using 2,2′-Bipyridine

Mineral carbonation is gaining increasing attention for its ability to sequester CO2. The main challenge is doing it economically and energy-efficiently. Recently, many studies have focused on the aqueous reaction of carbon dioxide with the alkaline earth minerals such as serpentine, Mg-rich olivine and wollastonite. Nevertheless, Fe-rich olivines have been poorly studied because of their high energy demand, which make them unfeasible for industrial implementation. This article describes the feasibility of an indirect mineral carbonation process using silicic, Fe-rich mining waste with direct flue gas CO2 via iron complexation using 2,2′-bipyridine. The overall process was performed in three main steps: leaching, iron complexation, and aqueous mineral carbonation reactions. The preferential parameters resulted in a recirculation scenario, where 38% of Fe cations were leached, complexed, and reacted under mild conditions. CO2 uptake of 57.3% was achieved, obtaining a Fe-rich carbonate. These results are promising for the application of mineral carbonation to reduce CO2 emissions. Furthermore, the greenhouse gas balance had a global vision of the overall reaction’s feasibility. The results showed a positive balance in CO2 removal, with an estimated 130 kg CO2/ton of residue. Although an exhaustive study should be done, the new and innovative mineral carbonation CO2 sequestration approach in this study is promising.

Aqueous mineral carbonation of ultramafic material: a pre-requisite to integrate into mineral extraction and tailings management operation.

Ex situ aqueous mineral carbonation of ultramafic mining waste is an evolving technology for the CO2 sequestration from small- to medium-scale emitters. The mineral ores or mine wastes of associated ultramafic mineralogy are a suitable feedstock for mineral carbonation. The aqueous mineral carbonation at ambient temperature is motivating and attractive from an energy-saving perspective. This study has investigated the CO2 sequestration potential of a locally available ultramafic material generated from a nickel ore mine with a futuristic scope of integrating the method into an ongoing mineral extraction and/or tailing management operation. The mineral characterization and experimental results indicate that the tested material has CO2 sequestration potential and underwent carbonation at ambient temperature. The carbonate conversion efficiencies obtained for Ca and Mg from the dissolved ionic forms at optimum conditions are 60% and 25%, respectively. The material was able to sequestrate about 0.12 gCO2 per g solid at this efficiency. Aragonite and hydromagnesite are the major products that evolved out from the aqueous carbonation. Based on the mineral carbonation results, the novel concept of integrating the evolved method to existing mineral extraction and/or tailings management operation is discussed.