In this paper, the synchronization of Chaotic Lur’e systems subject to aperiodic sampling is investigated. It is shown that sampling interval is bounded and nonuniform. A modified free-matrix-based (MFMB) time-dependent Lyapunov functional is developed to capture the information on sampling pattern, which is sufficiently used to analyze stability of Chaotic Lur’e systems. For a special case that the sampled-data controller suffers constant input delay, a discontinuous Lyapunov functional is presented based on the vector extension of Wirtinger’s inequality. The obtained stability condition leads to a less computational complexity than some of existing works. A longer value on the calculation of sampling interval is achieved. Two illustrative examples demonstrate the effectiveness of designed methods and less conservatism of the obtained results.