Anisotropic Dispersion Research Articles

All-Dielectric Dual-Band Anisotropic Zero-Index Materials

Zero-index materials, characterized by near-zero permittivity and/or permeability, represent a distinctive class of materials that exhibit a range of novel physical phenomena and have potential for various advanced applications. However, conventional zero-index materials are often hindered by constraints such as narrow bandwidth and significant material loss at high frequencies. Here, we numerically demonstrate a scheme for realizing low-loss all-dielectric dual-band anisotropic zero-index materials utilizing three-dimensional terahertz silicon photonic crystals. The designed silicon photonic crystal supports dual semi-Dirac cones with linear-parabolic dispersions at two distinct frequencies, functioning as an effective double-zero material along two specific propagation directions and as an impedance-mismatched single-zero material along the orthogonal direction at the two frequencies. Highly anisotropic wave transport properties arising from the unique dispersion and extreme anisotropy are further demonstrated. Our findings not only show a novel methodology for achieving low-loss zero-index materials with expanded operational frequencies but also open up promising avenues for advanced electromagnetic wave manipulation.

Shear wave speed, dispersion slope and anisotropy evaluation using cardiac shear wave elastography in patients with Fabry disease

Abstract Background Cardiac shear wave imaging has been proposed to investigate left ventricular myocardial alterations non-invasively. Dispersion slope and anisotropy are fundamental properties that have not been studied in Fabry disease (FD) patients yet. Purpose The aim of this study was to determine and compare shear wave propagation speed, dispersion slope and fractional anisotropy in FD patients and healthy controls. Methods We prospectively included 20 FD patients and 20 healthy controls (HC). Shear wave speed, dispersion slope and fractional anisotropy were measured non-invasively in anteroseptal basal segment using an ultrasound for cardiac shear wave imaging. Echocardiography, electrocardiogram and laboratory evaluations were performed. Results Shear wave propagation speed was higher in FD patients than in HC group (1.46 ± 0.12 m/s and 1.36 ± 0.17 m/s, p = 0.03). No difference was found in dispersion slope (11.4 m/s/kHz in FD group and 11.3 m/s/kHz in HC group, p = 0.6). Fractional anisotropy was 0.05 ± 0.04 in FD group and 0.05 ± 0.04 in HC group, p = 0.4. Conclusion Shear wave speed was higher in FD patients compared to control group. Dispersion slope and fractional anisotropy in FD group did not reveal significant difference to the control group.

Zero momentum topological insulator in 2D semi-Dirac materials

Abstract Semi-Dirac materials in 2D present an anisotropic dispersion relation, linear along one direction and quadratic along the perpendicular one. This study explores the topological properties and the influence of disorder in a 2D semi-Dirac Hamiltonian. Energy-dependent edge states appear only in one direction, localized on either the upper or lower edge of the nanoribbon determined by their particle or hole character. Their topological protection can be rigorously founded on the Zak phase of the one-dimensional reduction of the semi-Dirac Hamiltonian, that depends parametrically on one of the momenta. In general, only a single value of the momentum, corresponding to a zero energy mode, is topologically protected. We explore the dependence on the disorder of the edge states and the robustness of the topological protection in these materials. We also explore the consequences of the topological protection of the zero-momentum state in the transport properties for a two-terminal configuration.

Electronic structure investigation and anisotropic phonon anharmonicity in ternary ZrGeTe4 single crystals

Ternary two-dimensional (2D) transition metal chalcogenides have gained immense attention because of their ability to overcome the intrinsic limitations of their binary counterparts. Layered 2D materials are important for future electronic and photonic devices owing to their low structural symmetry and in-plane anisotropy with tunable bandgap. Herein, the electronic structure and detailed vibrational properties of bulk ZrGeTe4 layered single crystals were investigated using angle-resolved photoemission spectroscopy (ARPES) and Raman scattering (RS). The ARPES results revealed an anisotropic Fermi surface of different momentum along kx and ky from the zone center and an anisotropic band structure with varying band curvatures along the high-symmetry directions. Furthermore, the RS of ZrGeTe4 was investigated under different polarizations and varying temperatures. The polarized RS exhibited twofold and fourfold symmetry orientations in different configurations, revealing the anisotropic phonon dispersions for bulk ZrGeTe4. The observed softening of Raman modes was corroborated with the anharmonic phonon dispersion, which was further supported by our third-order force constant calculations of thermal transport using density functional theory. Low lattice thermal conductivity with increasing temperature is linked with enhanced phonon–phonon scattering, which is evident from the decreased phonon lifetime and peak linewidth. In addition to these fundamental aspects, the anisotropic nature and unique layered structure of such materials reveal their bright future for next-generation nanoelectronic applications.

In-plane anisotropic dispersion property and second-harmonic generation of violet phosphorus with two-dimensional nano-interlocking structure

The unique one-dimensional chain structure of violet phosphorus provides an ideal platform for the study of second-order nonlinear optical properties. This also offers more possibilities for the further development of novel two-dimensional layered nanomaterials in the frequency domain. The research suggest that the highest occupied molecular orbital of monolayer phosphorene is characterized by a small effective mass and high hole mobility, while the lowest unoccupied molecular orbital exhibits opposite properties. This may be attributed to increased lattice scattering or electron-electron interactions in the conduction band. Monolayer violet phosphorus exhibits strong absorption capabilities in the near-ultraviolet light range, which can be utilized in UV spectroscopy technology for detecting harmful substances in water and air. Besides, its second harmonic generation response is also very strong within the visible light spectrum, and this response significantly varies with changes in angle. This provides theoretical guidance for optimizing the different stacking directions and heterojunction structures of violet phosphorus, more importantly, the sensitivity and directional selectivity of sensors can be improved. The work not only deepens the understanding of the electro-optical performance of violet phosphorus materials but also lays a theoretical foundation and guidance for the design and application of devices based on violet phosphorus.

Effects of background elastic and permeability anisotropy on dynamic seismic signatures of a fluid-saturated porous rock with aligned fractures

Seismic dispersion, attenuation, and frequency-dependent anisotropy due to wave-induced fluid flow (WIFF) in fluid-saturated porous and fractured rocks have been widely studied. However, most of these studies do not consider the effects of background elastic and permeability anisotropy. In this work, we study such effects by considering a fluid-saturated porous rock with penny-shaped fractures embedded in the isotropic plane of a transversely isotropic (TI) background. Starting with P-waves propagating perpendicularly to the fracture plane, we obtain the wavefields in the fluid-saturated porous TI background scattered from a single fracture. This allows for the calculation of effective P-wavenumber through the Foldy approximation and the derivation of a frequency-dependent fracture compliance matrix. The angle-dependent seismic dispersion and attenuation, as well as frequency-dependent anisotropy, can thus be calculated. Using this model, we study a fractured tight sandstone with a TI background. The results show that the background elastic anisotropy primarily affects the seismic frequency-dependent anisotropy, while the background permeability anisotropy not only affects seismic frequency-dependent anisotropy but also influences seismic dispersion and attenuation. In particular, the background permeability anisotropy alters the rate of change in seismic velocities and velocity anisotropy parameters with frequencies and the peaks of seismic attenuation and attenuation anisotropy parameters. By comparing the theoretical predictions of our model to other theories and also to two sets of experimental data, our model is validated. Our model can be applied to characterize the fractured, layered earth.

Tailoring Dispersion Property and Anisotropy of Second-Harmonic Generation by Strain Engineering in Monolayer GeSe

Tailoring Dispersion Property and Anisotropy of Second-Harmonic Generation by Strain Engineering in Monolayer GeSe

Tailoring Phonon Dispersion of a Genetically Designed Nanophononic Metasurface.

Phonon engineering at the nanoscale holds immense promise for a myriad of applications. However, the design of phononic devices continues to rely on regular shapes chosen according to long-established simple rules. Here, we demonstrate an inverse design approach to create a two-dimensional phononic metasurface exhibiting a highly anisotropic phonon dispersion along the main axes of the Brillouin zone. A partial hypersonic bandgap of approximately 3.5 GHz is present along one axis, with gap closure along the orthogonal axis. Such a level of control is achieved through genetically optimized unit cells, with shapes exceeding conventional intuition. We experimentally validated our theoretical predictions using Brillouin light scattering, confirming the effectiveness of the inverse design method. Our approach unlocks the potential for automated engineering of phononic metasurfaces with on-demand functionalities, thus leading toward innovative phononic devices beyond the limitations of traditional design paradigms.

Investigation on particle slug flow using large eddy simulation combined a particle kinetic energy model

In this study, an investigation on particle hydrodynamic behaviors of gas-particle slug flow is modeled and numerically simulated. A novelty particle kinetic energy model at subgrid-scale level is developed to consider the effect of gas turbulence on particle movement and a four-way coupling approach is combined. Anisotropic particle dispersions and the multiphase interactions is revealed by using a second-order moment turbulence model and large eddy simulation is performed to solve the Euler-Euler two-fluid transport equations, Predictions are well agreed with the experimental data and reported results by discrete particle model built-in the multiphase flow model with interphase exchanges code. Bubble motions have great effects on the particle dynamics due to bubble entrainment. Flow patterns of particle circulation are generated between higher and lower concentrations. The largest frequency of power spectrum density at center of top surface is approximately 4.5 times larger than that of wall region. Bubblelike granular temperatures are much larger than smaller-scale particle granular temperature. At the top surface, maximum value of vertical bubblelike Reynolds stress is found at x/W = 0.28, it is 4.0 times larger than that of the lateral x-direction. In addition, the mean values, and the standard deviation of SGS particle kinetic energy at center are both approximately 3.5 times larger than those of z = 10.0 cm. For particle shear stress at middle section, maximum ratios of mean value and standard deviation at central regions to those of walls reach up to 8.0 and 11.0.

Thermoelectric effects in ballistic junctions of 2D-Weyl semimetals

Two dimensional Weyl semimetals are a variant of topological materials in two dimensions, which are realized in three atomic layer materials. These materials possess isotropic or anisotropic dispersions around Weyl nodes and present some common physical properties with their 3D counterparts. We study the thermoelectric effects in a ballistic junction of 2D-Weyl semimetal with isotropic or anisotropic dispersions around the Weyl points. We demonstrate that these two types of 2D-Weyl semimetals exhibit different thermoelectric responses at low chemical potentials of the leads. The Weyl semimetal layer’s physical characteristics can significantly affect these junctions’ thermoelectric properties. Moreover, significant Seebeck coefficient and thermoelectric figure of merit of these junctions are only observed at the low chemical potential of the leads. In particular, we unveil that thermoelectric effects in the ballistic junction of 2D-Weyl semimetals are not as efficient as their 3D counterparts.

The Rotation of Classical Bulges in Barred Galaxies in the Presence of Gas

Barred galaxies often develop a box/peanut pseudobulge, but they can also host a nearly spherical classical bulge, which is known to gain rotation due to the bar. We aim to explore how the presence of gas impacts the rotation of classical bulges. We carried out a comprehensive set of hydrodynamical N-body simulations with different combinations of bulge masses and gas fractions. In these models, both massive bulges and high gas content tend to inhibit the formation of strong bars. For low-mass bulges, the resulting bar is stronger in cases of low gas content. In the stronger bar models, bulges acquire more angular momentum and thus display considerable rotational velocity. Such bulges also develop anisotropic velocity dispersions and become triaxial in shape. We found that the rotation of the bulge becomes less pronounced as the gas fraction is increased from 0 to 30%. These results indicate that the gas content has a significant effect on the dynamics of the classical bulge, because it influences bar strength. Particularly in the case of the low-mass bulges (10% bulge mass fraction), all of the measured rotational and structural properties of the classical bulge depend strongly and systematically on the gas content of the galaxy.

Vacancy modulation dramatically enhances the thermoelectric performance of InTe single crystal

InTe single crystals have demonstrated great promise in the field of thermoelectric materials, particularly when oriented along the [110] direction. This specific crystal orientation exhibits higher electronic conductivity and lower thermal conductivity compared to other orientations of InTe. Through first-principles calculations, we identified the anisotropic valence band and phonon dispersion as the underlying factors. Moreover, reducing the density of In+ vacancies in InTe was found to lower the band effective mass and modulate carrier scattering, enhancing the material quality factor (B). To explore these findings, we systematically grew InTe single crystals, achieving exceptional thermoelectric performance. A record-breaking power factor of 12.0 μW·cm−1·K−2 and a dimensionless figure of merit (zT) of 0.5 at room temperature were obtained. Notably, InTe crystals oriented along [110] with low In+ vacancy density exhibited the highest average zT of 0.63 among InTe-based thermoelectric materials within the 300–473 K temperature range. Furthermore, we introduced an effective method of reducing In+ vacancies through Indium vapor annealing, resulting in the highest reported carrier mobility of 182 cm2·V−1·s−1 for InTe. Our study highlights the potential for improving InTe's thermoelectric performance near room temperature through vacancy modulation and crystal orientation.

Spin-wave self-imaging: Experimental and numerical demonstration of caustic and Talbot-like diffraction patterns

Extending the scope of the self-imaging phenomenon, traditionally associated with linear optics, to the domain of magnonics, this study presents the experimental demonstration and numerical analysis of spin-wave (SW) self-imaging in an in-plane magnetized yttrium iron garnet film. We explore this phenomenon using a setup in which a plane SW passes through a diffraction grating, and the resulting interference pattern is detected using Brillouin light scattering. We have varied the frequencies of the source dynamic magnetic field to discern the influence of the anisotropic dispersion relation and the caustic effect on the analyzed phenomenon. We found that at low frequencies and diffraction fields, the caustics determine the interference pattern. However, at large distances from the grating, when the waves of high diffraction order and number of slits contribute to the interference pattern, the self-imaging phenomenon and Talbot-like patterns are formed. This methodological approach not only sheds light on the behavior of SW interference under different conditions but also enhances our understanding of the SW self-imaging process in both isotropic and anisotropic media.

Modeling and simulation of pollution transport in the Mediterranean Sea using enriched finite element method

This paper presents a novel numerical method for simulating the transport and dispersion of pollutants in the Mediterranean sea. The governing mathematical equations consist of a barotropic ocean model with friction terms, bathymetric forces, Coriolis and wind stresses coupled to an advection–diffusion equation with anisotropic dispersion tensor and source terms. The proposed numerical solver uses a multilevel adaptive semi-Lagrangian finite element method that combines various techniques, including the modified method of characteristics, finite element discretization, coupled projection scheme based on a rotational pressure correction algorithm, and an adaptive L2-projection. The approach employs the gradient of the concentration as an error indicator for enrichment adaptations and increasing the number of quadrature points where needed without refining the mesh. The method is shown to provide accurate and efficient simulations for pollution transport in the Mediterranean sea. The proposed approach distinguishes itself from the well-established adaptive finite element methods for incompressible viscous flows by retaining the same structure and dimension of linear systems during the adaptation process.

Assessment of white matter microstructure integrity in subacute postconcussive vestibular dysfunction using NODDI

Abstract Vestibular symptoms, such as dizziness and balance impairment, are frequently reported following mild traumatic brain injury (mTBI) and are associated with a protracted recovery, yet the underlying neuroanatomical substrates remain unclear. The present study utilized advanced diffusion MRI (dMRI) techniques including both conventional diffusion tensor imaging (DTI) and neurite orientation dispersion and density imaging (NODDI) to investigate microstructural white matter integrity in individuals with postconcussive vestibular dysfunction (PCVD) within the subacute injury period (median of 35 days from injury; IQR of 23). Study participants included 23 individuals with subacute PCVD and 37 healthy control subjects who underwent imaging and comprehensive clinical vestibular testing. Between-group voxelwise analysis of differences in white matter revealed areas of higher intra-neurite volume fraction (VIn) and isotropic volume fraction (VIso) within PCVD subjects compared to controls, which involved overlapping regions within the left hemisphere of the brain. Affected areas of higher VIn and VIso included the superior longitudinal fasciculus (SLF) and superior and posterior corona radiata (SCR and PCR, respectively). We examined the relationship between clinical vestibular measures and diffusion metrics including DTI (fractional anisotropy [FA], mean diffusivity [MD], radial diffusivity [RD] and axial diffusivity [AD]) and NODDI (intraneurite volume fraction [VIn], isotropic volume fraction [VIso], dispersion anisotropy [DA], orientation dispersion indexTotal/Primary/Secondary [ODIT/P/S]) within 32 regions-of-interest. Clinical vestibular measures included self-reported measures, including the Dizziness Handicap Inventory, Visual Vertigo Analog Scale, and Vestibular/Ocular-Motor Screening, as well as objective vestibular testing using the sensory organization test. Significant correlations were found with clinical measures across all diffusion maps (except DA), within various regions of interest (ROIs), including SLF, SCR, and PCR. These results implicate several important association bundles that may potentiate sensory processing dysfunction related to PCVD. Whether these neuroanatomical differences found within the subacute phase of PCVD are in response to injury or represent preexisting structural variations that increase vulnerability to sensory processing dysfunction is unclear and remains an active area of study.

Anisotropic dielectric dispersions and thermal behaviors in highly textured BN thin films for heat self-dissipating electronics

Mainstream high-k gate materials, such as SiO2, Al2O3, and HfZrO2, are in demand for modern electronics. However, these dielectrics possess lower thermal conductivity, significantly limiting thermal dissipation in electronic devices. Herein, we propose the utilization of complementary metal-oxide semiconductor- (CMOS) compatible high power impulse magnetron sputtering (HiPIMS) for the mass production of highly textured hexagonal boron nitride (h-BN) on (100)-, (110)-, and (111)-oriented SrTiO3 substrates. The as-prepared films exhibit distinct vertical alignments, as evidenced by HRTEM and FTIR analysis. Notably, the R value, ranging from 0.46 to 0.50, is associated with the stress in the film. Importantly, distinct anisotropies in thermal conductivity, dielectric constant, and optical band gap are observed. Furthermore, the values of thermal conductivity in these highly textured h-BN films are 4.5, 5.7, and 5.3 Wm−1K−1, which is almost three times larger than those of SiO2 (1.4 Wm−1K−1) and Al2O3 (1.35 Wm−1K−1), and even an order of magnitude larger than that of HfZrO2 (0.67 Wm−1K−1). The combination of excellent dielectric characteristics, favorable thermal conductivity, and superior stability over a broad temperature range makes this novel material outperform conventional dielectric gate materials in high-power electronics applications.

Extraordinary Polarization and Thickness Dependences of Photocarrier Dynamics in PdSe2 Ribbons.

Pentagonal palladium diselenide (PdSe2) stands out for its exceptional optoelectronic properties, including high carrier mobility, tunable bandgap, and anisotropic electronic and optical responses. Herein, we systematically investigate photocarrier dynamics in PdSe2 ribbons using polarization-resolved optical pump-probe spectroscopy. In thin PdSe2 ribbons with a semiconductor phase, the photocarrier dynamics are found to be dominated by intraband hot-carrier cooling, interband recombination, and the exciton effect, showing weak crystalline orientation dependences. Conversely, in thick semimetal-phase PdSe2 ribbons, the photocarrier relaxations governed by the electron-optical/acoustic phonon scattering strongly depend on the sample orientation, albeit with a degradation in in-plane anisotropy following hot-carrier cooling. Furthermore, we analyze the correlations between photocarrier dynamics and anisotropic energy dispersions of electronic structures across a wide range in k space, as well as the contributions from the anisotropic electron-phonon couplings. Our study provides crucial insights for developing polarization-sensitive photoelectronic devices based on PdSe2.

Anisotropic Klemens model for the thermal conductivity tensor and its size effect

With the constraint from Onsager reciprocity relations, here we generalize the Klemens model for intrinsic phonon-phonon scattering from isotropic to anisotropic. Combined with the anisotropic Debye dispersion, this anisotropic Klemens model leads to analytical expressions for heat transfer along both ab-plane (κab) and c-axis (κc), suitable for both layered and chainlike materials with any anisotropy ratio of the dispersion and the scattering. This combination of dispersion and scattering is further applied to the equation of phonon radiative transfer to model heat conduction across anisotropic thin films. The model is compared to experimental κab and κc of bulk graphite at high temperatures (T≥0.1×max(θD,ab,θD,c), where θD,ab and θD,c are the two Debye temperatures), leading to best-fit scattering parameters that capture the harmonic and anharmonic nature of the intra- and inter-layer bonding of graphite. With no further adjusting of these parameters, the anisotropic scattering model performs at least 9 times better than the isotropic one at explaining the experimental κc of graphite thin films. This size effect is further justified by comparing the accumulation function of κc.

Dynamic polarization, quantum spectral function and effective mass for black phosphorous: Random phase approximation approach at finite temperature

In this work, the finite-temperature dynamic polarization function of black phosphorus is obtained using the random phase approximation (RPA) for the lower band of the corresponding effective Hamiltonian. The maximum temperature-dependent polarization of the orthorhombic honeycomb structure of black phosphorus is observed at ω=0.54eV for wavectors at the Fermi level. Several peaks are thus observed indicating that an overall Fermi-liquid behavior is present but with different kinds of quasiparticles. These quasiparticles appear due to the highly anisotropic energy dispersion. Experiments conducted on black phosphorous at a temperature of 10 K have a tremendous effect on the scattering mechanism. Subsequently, the quasiparticle behavior is studied through the spectral function and the effective mass, each resolved on the three components of the wave number. The resulting effective mass anisotropy causes the plasmon to disperse completely, leading to a lower resonant frequency when there is a larger mass along one of the axes. At large wavelengths, the RPA result is almost identical to that obtained from the classical plasmon dispersion.

Phonon-Driven Femtosecond Dynamics of Excitons in Crystalline Pentacene from First Principles.

Nonradiative exciton relaxation processes are critical for energy transduction and transport in optoelectronic materials, but how these processes are connected to the underlying crystal structure and the associated electron, exciton, and phonon band structures, as well as the interactions of all these particles, is challenging to understand. Here, we present a first-principles study of exciton-phonon relaxation pathways in pentacene, a paradigmatic molecular crystal and optoelectronic semiconductor. We compute the momentum- and band-resolved exciton-phonon interactions, and use them to analyze key scattering channels. We find that both exciton intraband scattering and interband scattering to parity-forbidden dark states occur on the same ∼100 fs timescale as a direct consequence of the longitudinal-transverse splitting of the bright exciton band. Consequently, exciton-phonon scattering exists as a dominant nonradiative relaxation channel in pentacene. We further show how the propagation of an exciton wave packet is connected with crystal anisotropy, which gives rise to the longitudinal-transverse exciton splitting and concomitant anisotropic exciton and phonon dispersions. Our results provide a framework for understanding the role of exciton-phonon interactions in exciton nonradiative lifetimes in molecular crystals and beyond.