The slab dynamic processes, such as roll-back during oceanic subduction and break-off during collision orogenesis, would affect the movement of mantle material and the interaction between crust and mantle, accompanied by significant amounts of magmatism. Providing accurate depictions for these processes are extremely difficult, especially in the case of ancient orogens. Here, we present an integrated study of petrology, geochronology, geochemistry and Sr–Nd–Hf isotopes for Early Paleozoic granitoids from the Duojielaka, Ledu and Binglingsi plutons of the southeastern Qilian orogen. Our LA-ICP-MS UPb zircon data show that these granitoids were emplaced at 476–432 Ma. The petrological and geochemical data suggest that the ~476 Ma Duojielaka porphyritic syenogranites formed by feldspar-dominated fractionation from relatively K-rich basaltic rock-derived adakitic parental magma. The ~454 Ma Duojielaka biotite monzogranites are highly fractionated I-type granites and were derived from basement orthogneisses mixed with minor mafic rocks. The Ledu fine- and medium-grained quartz diorites (~446 and ~452 Ma) are high-K calc-alkaline to shoshonitic and were produced by partial melting of relatively old K-rich mafic crust followed by minor mixing with mantle-derived magmas. The ~432 Ma Binglingsi biotite monzogranites with adakitic characteristics most likely originated by partial melting of thickened mafic lower crust. Based on the new data, in combination with previously published data, we suggest that the roll-back of the South Qilian oceanic slab occurred during the Middle Cambrian to early Middle Ordovician. The Duojielaka porphyritic syenogranites represented crustal anatexis in an arc front associated with slab roll-back. The Late Ordovician–early Middle Silurian intrusive rocks probably resulted from diachronous slab break-off in the post-collisional stage. The rocks record the opening of the break-off window from east to west and the gradual heat propagation from the central part to the southern and northern margins of the eastern Central Qilian due to the widening of break-off window and asthenospheric upwelling. We propose that complex geodynamic processes and their thermal effects can be traced by a comprehensive consideration of the petrogenetic, temporal and spatial evolution of related magmatism.
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