All-optical Helicity-dependent Switching Research Articles

Single-shot all-optical switching of magnetization in TbFe

Thermally induced magnetization switching (TIMS) relying solely on a single laser without any applied magnetic field is a key research direction of current spintronics. Most studies on TbFe so far have focused on helicity-dependent all-optical switching (HD-AOS). In this work, we observe the TIMS on TbFe alloys excited by atomic spin dynamics simulations combined with a two-temperature model. The results show that the magnetization switching of TbFe can be found under certain damping conditions. In addition, we further investigated the reasons why energy density leads to the opposite switching time behavior of Tb and Fe, and our research results also found that changes in damping can affect the concentration and energy density range of the switching, as well as the maximum pulse duration. The dynamic behavior indicates that TbFe switching in 2 ps or less. Our findings widen the basis for fast optical switching of magnetization and break new ground for engineered materials that can be used for nonvolatile ultrafast switching using ultrashort pulses of light.

Multiphysics Modeling of Plasmon-Enhanced All-Optical Helicity-Dependent Switching.

In this work, we propose a multiphysics approach to simulate all-optical helicity-dependent switching induced by the local hot spots of plasmonic nanostructures. Due to the plasmonic resonance of an array of gold nanodisks, strong electromagnetic fields are generated within the magnetic recording media underneath the gold nanodisks. We construct a multiphysics framework considering the opto-magnetic and opto-thermal effects, and then model the magnetization switching using the Monte Carlo method. Our approach bridges the gap between plasmonic nanostructure design and magnetization switching modeling, allowing for the simulation of helicity-dependent, nanoscale magnetization switching in the presence of localized surface plasmons.

Optically Induced Magnetization Switching in NiCo2O4 Thin Films Using Ultrafast Lasers

All-optical magnetization control has recently been garnering considerable attention to realize next-generation ultrafast magnetic information devices. Here, employing a magneto-optical Kerr effect (MOKE) microscope, we observed the laser-induced magnetization switching of ferrimagnetic oxide NiCo2O4 (NCO) epitaxial thin films with perpendicular magnetic anisotropy, where the sample was pumped by 1030 nm laser pulses, and magnetic domain images were acquired via the MOKE microscope with a white light emitting diode. Laser pulses irradiated the NCO thin film at various temperatures from 300 to 400 K while altering the parameters of pulse interval, fluency, and the number of pulses in the absence of the external magnetic field. We observed accumulative all-optical helicity-dependent switching above 380 K. Our observation of oxide NCO thin films facilitates the realization of magnetization switching using ultrafast lasers without applying a magnetic field.

Plasmonic dichroism and all-optical magnetization switching in nanophotonic structures with GdFeCo.

We report on a phenomenon of plasmonic dichroism observed in magnetic materials with transverse magnetization under excitation of surface plasmon polariton waves. The effect originates from the interplay of the two magnetization-dependent contributions to the material absorption, both of which are enhanced under plasmon excitation. Plasmonic dichroism is similar to circular magnetic dichroism, which is at the base of all-optical helicity-dependent switching (AO-HDS) but observed for linearly polarized light, and the dichroism acts upon in-plane magnetized films, where AO-HDS does not take place. We show by electromagnetic modeling that laser pulses exciting counter-propagating plasmons can be used to write +M or -M states in a deterministic way independent of the initial magnetization state. The presented approach applies to various ferrimagnetic materials with in-plane magnetization, exhibiting the phenomenon of all-optical switching of a thermal nature and broadens the horizons of their applications in data storage devices.

Magnetization manipulation using ultra-short light pulses

In this review, we discuss the different results demonstrating deterministic magnetization switching using ultra-fast laser pulses, named all-optical switching (AOS). The response of these magnetic systems can be separated into two groups depending on whether the helicity of the incident light affects the switching behaviour. All optical helicity-independent switching (AO-HIS) occurs after a single laser pulse and is mostly observed in Gd-based alloys and multilayers while all optical helicity-dependent switching (AO-HDS) occurs following multiple laser pulses and is observed in a diverse range of magnetic thin films. Our discussion focuses on the experimental and theoretical aspects of AO-HIS from Gd-based systems and other emerging materials. For AO-HDS, we highlight recent progress on the influence of domain size, state diagrams, mechanisms, and interlayer coupling. Finally, we discuss the potential application of all-optical switching in data-storage and logic devices, such as magnetic tunnel junctions, racetrack memories, and logic computation.

Timescales and contribution of heating and helicity effect in helicity-dependent all-optical switching

The heating and helicity effects induced by circularly polarized laser excitation are entangled in the helicity-dependent all-optical switching (HD-AOS), which hinders understanding the magnetization dynamics involved. Here, applying a dual-pump laser excitation, first with a linearly polarized (LP) laser pulse followed by a circularly polarized (CP) laser pulse, the timescales and contribution from heating and helicity effects in HD-AOS were identified with a Pt/Co/Pt triple-layer. When the LP laser pulses preheat the sample to a nearly fully demagnetized state, the CP laser pulses with a power reduced by 80% switch the sample’s magnetization. By varying the time delay between the two pump pulses, the results show that the helicity effect, which gives rise to the deterministic helicity-induced switching, arises almost instantly within 200 fs close to the pulse width upon laser excitation. The results reveal that the transient magnetization state upon which CP laser pulses impinge is the key factor for achieving HD-AOS, and importantly, the tunability between heating and helicity effects with the unique dual-pump laser excitation approach will enable HD-AOS in a wide range of magnetic material systems having wide-ranging implications for potential ultrafast spintronics applications.Graphical abstract

All-optical frequency-dependent magnetic switching in metal-insulator-metal stub structures.

Many attempts to switch magnetization with optical pulses were based on free-space coupling schemes of circularly polarized light pulses, so-called all-optical helicity-dependent magnetic switching; however, waveguide coupling schemes are promising for on-chip all-optical magnetic switching. Metal-insulator-metal (MIM) stub structures provide a promising platform for highly integrated photonic circuits, thanks to their compact size, on-chip compatibility, and ease of fabrication. We found clockwise and counterclockwise ring-like modes in the MIM stub structure, which can act as effective magnetic fields with two opposite directions due to the inverse Faraday effect. Effective magnetic field spectra inside the MIM stub have dual resonant peaks at which the effective magnetic field intensity reaches its extreme values with opposite signs, corresponding to binary magnetic states. Switching between the binary magnetic states can be achieved by altering the optical pump frequency. The all-optical frequency-dependent magnetic switching in the MIM stub may provide a chip-compatible and ultracompact tool for ultrafast switching of magnetic order.

Efficient All-Optical Helicity Dependent Switching of Spins in a Pt/Co/Pt Film by a Dual-Pulse Excitation

All-optical helicity dependent switching (AO-HDS), deterministic control of magnetization by circularly polarized laser pulses, allows to efficiently manipulate spins without the need of a magnetic field. However, AO-HDS in ferromagnetic metals so far requires many laser pulses for fully switching their magnetic states. Using a combination of a short, 90-fs linearly polarized pulse and a subsequent longer, 3-ps circularly polarized pulse, we demonstrate that the number of pulses for full magnetization reversal can be reduced to four pulse pairs in a single stack of Pt/Co/Pt. The obtained results suggest that the dual-pulse approach is a potential route towards realizing efficient AO-HDS in ferromagnetic metals.

Magneto-optical design of anomalous Nernst thermopile

The introduction of spin caloritronics into thermoelectric conversion has paved a new path for versatile energy harvesting and heat sensing technologies. In particular, thermoelectric generation based on the anomalous Nernst effect (ANE) is an appealing approach as it shows considerable potential to realize efficient, large-area, and flexible use of heat energy. To make ANE applications viable, not only the improvement of thermoelectric performance but also the simplification of device structures is essential. Here, we demonstrate the construction of an anomalous Nernst thermopile with a substantially enhanced thermoelectric output and simple structure comprising a single ferromagnetic material. These improvements are achieved by combining the ANE with the magneto-optical recording technique called all-optical helicity-dependent switching of magnetization. Our thermopile consists only of Co/Pt multilayer wires arranged in a zigzag configuration, which simplifies microfabrication processes. When the out-of-plane magnetization of the neighboring wires is reversed alternately by local illumination with circularly polarized light, the ANE-induced voltage in the thermopile shows an order of magnitude enhancement, confirming the concept of a magneto-optically designed anomalous Nernst thermopile. The sign of the enhanced ANE-induced voltage can be controlled reversibly by changing the light polarization. The engineering concept demonstrated here promotes effective utilization of the characteristics of the ANE and will contribute to realizing its thermoelectric applications.

Optoelectronic domain-wall motion for logic computing

Logic computing in magnetic domain walls is investigated using the interplay of all-optical helicity-dependent switching and current-induced spin–orbit torque switching. By simultaneously controlling current and laser pulses, logic functions of AND, OR, NAND, and NOR are experimentally demonstrated through the anomalous Hall effect and verified by micromagnetic simulations. The optoelectronic domain-wall motion is energy-efficient compared to the traditional all-current approach and provides another degree of freedom for the realization of logic applications.

All‐Optical Helicity‐Dependent Switching in Hybrid Metal–Ferromagnet Thin Films

AbstractOver the past decades, optical manipulation of magnetization by ultrafast laser pulses has attracted extensive interest. It not only shows intriguing fundamental science arising from the interactions between spins, electrons, phonons, and photons, but also manifests the potential to process and store data at a speed that is three orders of magnitude faster than the current technologies. In this paper, all‐optical helicity‐dependent switching (AO‐HDS) in hybrid metal–ferromagnet thin films, which consist of Co/Pt multilayers with perpendicular magnetic anisotropy and an Au film capping layer on the top, is experimentally demonstrated. The switching behaviors of the hybrid Co/Pt–Au material, with various laser repetition rates, scanning speeds, and fluencies, are systematically studied. In comparison with bare Co/Pt multilayers, the hybrid metal–ferromagnet thin films show pronounced AO‐HDS when the number of laser pulses per μm along the scanning direction gradually increases. In addition, the AO‐HDS effect is very robust against laser fluences. A possible mechanism is further proposed based on numerical simulations of the optomagnetic coupling model. These findings promise a new material system that exhibits stable AO‐HDS phenomena, and hence can transform future magnetic storage devices, especially with the addition of plasmonic nanostructures made of noble metals.

Fully controllable three-dimensional light-induced longitudinal magnetization using a single objective lens.

With features of fast and energy-efficient data writing, all-optical helicity-dependent switching (AO-HDS) has emerged as a competitive technology to satisfy the demand for the next-generation volume data storage. Unfortunately, to switch the magnetizations in different positions of the magnetic-optic film, the laser beam, the objective lens, or the magnetic recording film should be moved, limiting the advantage of AO-HDS in fast data writing. To achieve on-the-fly magnetization switching, the induced magnetization should be fully controllable. In this Letter, by focusing an azimuthally polarized vortex beam (APVB) and introducing an additional phase, a feasible strategy constructing subwavelength light-induced pure longitudinal multi-magnetization spots is proposed. In addition, the position of the multi-magnetization spots can be dynamically controlled. The distributions of the focused APVBs with different orbital angular momentum, and the induced magnetizations are surveyed. We believe that this is a practical and flexible three-dimensional magnetic recording technique with dynamic control of the recording position.

Micromagnetic Modeling of All Optical Switching of Ferromagnetic Thin Films: The Role of Inverse Faraday Effect and Magnetic Circular Dichroism

There is a lot of experimental evidence of All Optical Switching (AOS) by applying ultrashort laser pulses on ferromagnetic thin films with perpendicular magnetic anisotropy. However, the physical origin behind these processes remains under debate. In addition to the heating caused by the laser pulses, the Inverse Faraday Effect (IFE) and Magnetic Circular Dichroism (MCD) have been proposed as the most probable phenomena responsible for the observations of helicity-dependent AOS. Here, we review the influence of both phenomena by means of realistic micromagnetic simulations based on the Landau–Lifshitz–Bloch equation coupled to the heat transport caused by the laser heating. The analysis allows us to reveal the similarities and differences between both effects. While both mechanisms may lead to the local inversion of the initial magnetic state of a ferromagnetic sample submitted to a train of circularly polarized laser pulses, the Inverse Faraday Effect proves to be more efficient for nucleation and domain wall movement and it reproduces more accurately the different magnetic configurations that the experiments report for different values of the fluence of the laser beam.

Magneto-optical painting of heat current

Active control of heat flow is crucial for the thermal management of increasingly complex electronic and spintronic devices. In addition to conventional heat transport engineering, spin caloritronics has received extensive attention as a heat control principle owing to its high controllability and unique thermal energy conversion symmetry. Here we demonstrate that the direction of heat currents generated by spin-caloritronic phenomena can be changed simply by illuminating magnetic materials with visible light. The optical control of heat currents is realized through a combination of the spin-driven thermoelectric conversion called an anomalous Ettingshausen effect and all-optical helicity-dependent switching of magnetization. This approach enables not only pinpoint manipulation and flexible design of the heat current distribution by patterning the illuminating light but also on/off control of the resulting temperature modulation by tuning the light polarization. These versatile heat control functionalities will open up a pathway for nanoscale thermal energy engineering.

Multi-layer magnetic recording driven by a tunable laser

All-optical magnetization switching with features of low-power consumption and high writing speed is a promising road map to satisfy the demand for volume data storage. To promote denser and faster magnetic recording technologies, herein, all-optical helicity-dependent switching (AO-HDS) in multi-layer magnetic recording is proposed based on the chromatic aberration of an optical lens (Thorlabs’s N-BK7 plano-convex uncoated lens). The power of the incident beams and the thickness of the multi-layer magnetic recording film are designed carefully. Besides, the uniformity of this multi-layer magnetic recording is optimized. At last, a prototype system of information multiplexing based on this multi-layer magnetic recording technology is constructed as well. Flexible and controllable magnetization reversals in different layers are also demonstrated by tuning the wavelength and helicity of working beams. We believe that such a prototype system can pave the way for increasing the storage density in an effective and low-cost mode.

Controlling All-Optical Helicity-Dependent Switching in Engineered Rare-Earth Free Synthetic Ferrimagnets.

All‐optical helicity‐dependent switching in ferromagnetic layers has revealed an unprecedented route to manipulate magnetic configurations by circularly polarized femtosecond laser pulses. In this work, rare‐earth free synthetic ferrimagnetic heterostructures made from two antiferromagnetically exchange coupled ferromagnetic layers are studied. Experimental results, supported by numerical simulations, show that the designed structures enable all‐optical switching which is controlled, not only by light helicity, but also by the relative Curie temperature of each ferromagnetic layer. Indeed, through the antiferromagnetic exchange coupling, the layer with the larger Curie temperature determines the final orientation of the other layer and so the synthetic ferrimagnet. For similar Curie temperatures, helicity‐independent back switching is observed and the final magnetic configuration is solely determined by the initial magnetic state. This demonstration of electrically‐detected, optical control of engineered rare‐earth free heterostructures opens a novel route toward practical opto‐spintronics.

From single to multiple pulse all-optical switching in GdFeCo thin films

All-optical switching refers to the magnetization reversal induced by ultrashort laser pulses. Both single-pulse all-optical helicity-independent switching and multiple pulses all-optical helicity-dependent switching have been reported for GdFeCo thin films. In this paper, we demonstrate that for two GdFeCo compositions, the transition between these two behaviors can appear by increasing the thickness of the Pt capping or by tuning the laser fluence. The two types of switching cannot be observed for the same set of parameters, which supports that their mechanisms are uncorrelated. Our calculations indicate that the transition may be induced by a strong inhomogeneity of the electronic temperature within the thickness of the GdFeCo layer in the subpicosecond timescale.

From Multiple- to Single-Pulse All-Optical Helicity-Dependent Switching in Ferromagnetic Co/Pt Multilayers

All-optical helicity-dependent switching in ferromagnetic Co/Pt multilayers is investigated using magneto-optical microscopy and anomalous Hall effect measurements. A state diagram is built by studying the effect of pulse duration, fluence, and spot size. We use numerical solutions of the three-temperature model to explain that the all-optical helicity-dependent switching mechanism relies on the spin bath reaching temperatures close to the Curie point. Further insights into the reversal process are provided by the experimental demonstration of significant helicity-dependent reversal after a single laser pulse that reveals the involvement of direct angular momentum transfer. Moreover, based on the observation that longer pulse durations and larger spot sizes lead to enhanced reversal efficiency, we identify experimental conditions that lead to saturated magnetization reversal after just a few tens of laser pulses.

All-optical helicity-dependent magnetic switching by first-order azimuthally polarized vortex beams

In this letter, a method to realize all-optical helicity-dependent magnetic switching (AO-HDS) using a first-order azimuthally polarized vortex (FAPV) beam is demonstrated. Numerical calculations of the focal fields of FAPV beams reveal that left-handed and right-handed circular polarizations are generated due to the interaction between the polarization singularity and the helical wave front. Its feasibility for AO-HDS is experimentally demonstrated in Gd27Fe63.87Co9.13 under low numerical aperture (NA) conditions and within a narrow fluence window. It is numerically predicted that under high NA conditions, the lateral size of magnetic bits recorded by FAPV beams can be nearly 30% smaller than that obtained by circularly polarized beams, which opens a promising route to realize ultrafast and ultrahigh-density magnetic recording.

Suppression of all-optical switching in He+ -irradiated Co/Pt multilayers: influence of the domain-wall energy

The observation of all-optical helicity-dependent switching (AO-HDS) in ferri- and ferro-magnetic materials depends not only on the saturation magnetization, but on the magnetic domain size which takes into account the competition between the demagnetizing energy and the domain wall (DW) energy. In this paper, we study the optical response of Co/Pt multilayers for which perpendicular magnetic anisotropy can be tuned using He+ -irradiation. This allows us to correlate the observation of AO-HDS with the magnetic properties of the He+ -irradiated multilayer. These results give direct evidence of the crucial role of the DW energy in the laser-induced switching process.