The complex structural geometry along the northern continental margin of Oman formed during polyphase deformation from the mid-Cretaceous to the Miocene. We focus on the kinematics and tectonics of the Wadi Kabir Fault, which represents an eastern segment of the large-scale, composite Frontal Range fault system that forms the northern boundary of the central Al Hajar Mountains. The most exhumed rocks outcrop in the Saih Hatat window of the Al Hajar Mountains, which occurs in the footwall of the Wadi Kabir Fault. To better understand the tectonic history of the Wadi Kabir Fault, we report three K-Ar illite fault-gouge ages. Sample FG16-1 from a shallowly north-dipping gouge zone of the eastern segment of the Wadi Kabir Fault yielded two consistent ages that overlap within 2σ uncertainties at ∼90 Ma. Sample FG16-2 from the central segment of the fault yielded a K–Ar age of 57.9 ± 2.0 Ma (2σ uncertainties), which is interpreted as a late Paleocene faulting event as it perfectly matches the cooling history of the high-pressure rocks of the Saih Hatat window in the footwall of the Wadi Kabir Fault. We present two tectonic interpretations for the ∼90 Ma fault-gouge age and prefer a synchronous kinematic relationship with the parallel and contractional mid-Cretaceous Yenkit Shear Zone that was active at the distal Arabian Platform since 114 Ma. Because the 57.9 ± 2.0 Ma age is associated with pronounced footwall cooling, we interpret this age to be related to the formation of the Bandar Jissah Basin in the hanging wall of the Wadi Kabir Fault. We conclude that the Frontal Range fault system likely formed during the Paleocene and that its young (≤∼43 Ma) history was accommodated along the western segment of the fault, as there is no evidence of this Eocene fault interval at the Wadi Kabir Fault.