Surface modification by means of textured structures can largely enhance the tribological and wear behavior of components and tools under various environmental conditions. Continuous developments in machining processes, such as the micromilling technology, can be used to manufacture fine-scaled structures on hardened steel tool surfaces. Thus, the adjusted friction behavior, which can affect the tendency of a material to adhere to the surface, is compensated by the small number of contact points between the friction partner and the surface. Accordingly, anisotropic friction properties of such structures can lead to a locally different wear behavior.In this study, a NiCrBSiFe self-fluxing alloy is thermally sprayed onto specimens made of AISI M2 high-speed steel (HSS). Technological and bionic surface structures were applied on thermally sprayed and laser remelted substrates. Based on ball-on-disk tests, the coefficient of friction was determined and compared for different high velocity oxy fuel (HVOF) sprayed NiCrBSiFe coatings and surface textures. These experiments show that functional structures can reduce the coefficient of friction. The bio-inspired surface shows a friction reduction of approximately 35% compared to the as-sprayed and polished sample, and a reduction of 25% when compared to the remelted and smoothened surface. Moreover, the analyzed surface conditions lead to a different wear behavior than the bio-inspired structure, which possesses areas with a reduced oxidational wear and less adhesion when compared to the other surface conditions.