African Dust Research Articles

Coarse-mode mineral dust size distributions, composition and optical properties from AER-D aircraft measurements over the tropical eastern Atlantic

Abstract. Mineral dust is an important component of the climate system, affecting the radiation balance, cloud properties, biogeochemical cycles, regional circulation and precipitation, as well as having negative effects on aviation, solar energy generation and human health. Dust size and composition has an impact on all these processes. However, changes in dust size distribution and composition during transport, particularly for coarse particles, are poorly understood and poorly represented in climate models. Here we present new in situ airborne observations of dust in the Saharan Air Layer (SAL) and the marine boundary layer (MBL) at the beginning of its transatlantic transport pathway, from the AERosol Properties – Dust (AER-D) fieldwork in August 2015, within the peak season of North African dust export. This study focuses on coarse-mode dust properties, including size distribution, mass loading, shape, composition, refractive indices and optical properties. Size distributions from 0.1 to 100 µm diameter (d) are presented, fully incorporating the coarse and giant modes of dust. Within the MBL, mean effective diameter (deff) and volume median diameter (VMD) were 4.6 and 6.0 µm respectively, giant particles with a mode at 20–30 µm were observed, and composition was dominated by quartz and alumino-silicates at d > 1 µm. Within the SAL, particles larger than 20 µm diameter were always present up to 5 km altitude, in concentrations over 10−5 cm−3, constituting up to 40 % of total dust mass. Mean deff and VMD were 4.0 and 5.5 µm respectively. Larger particles were detected in the SAL than can be explained by sedimentation theory alone. Coarse-mode composition was dominated by quartz and alumino-silicates; the accumulation mode showed a strong contribution from sulfate-rich and sea salt particles. In the SAL, measured single scattering albedos (SSAs) at 550 nm representing d < 2.5 µm were 0.93 to 0.98 (mean 0.97). Optical properties calculated for the full size distribution (0.1 < d < 100 µm) resulted in lower SSAs of 0.91–0.98 (mean 0.95) and mass extinction coefficients of 0.27–0.35 m2 g−1 (mean 0.32 m2 g−1). Variability in SSA was mainly controlled by variability in dust composition (principally iron) rather than by variations in the size distribution, in contrast with previous observations over the Sahara where size is the dominant influence. It is important that models are able to capture the variability and evolution of both dust composition and size distribution with transport in order to accurately represent the impacts of dust on climate. These results provide a new SAL dust dataset, fully representing coarse and giant particles, to aid model validation and development.

Limited impact of eolian and riverine sources on the biogeochemical cycling of Cd in the tropical Atlantic

We present coupled cadmium (Cd) concentrations and Cd isotopic compositions (expressed as δ114Cd) in seawater profiles along the northeast-southwest GEOTRACES GA11 section in the tropical Atlantic Ocean. The GA11 section encompasses three contrasting regions including the Amazon River plume, the North African dust plume, and the Guinea Dome oxygen deficient zone (ODZ). Given the long oceanic residence time of Cd (104 to 105 yr), local inputs such as atmospheric and riverine sources are generally considered to be of little importance for the open ocean Cd budget, and the limited Cd isotope dataset available thus far has prevented any unambiguous conclusions on the importance of these processes. The GA11 section is ideally located for assessing the influence of external, natural and anthropogenic riverine and eolian inputs, as well as internal processes, on the Cd mass balance in the tropical Atlantic Ocean. As in previous Cd isotope studies, this dataset documents that both surface consumption–regeneration of micronutrients within the water column and deep water mass mixing exert the prime control on the cycling of Cd. However, we do observe some near-surface samples with lower-than-expected δ114Cd signatures along the western section of the transect. Surface waters sampled at the margin of the Amazon freshwater plume show no resolvable difference in [Cd] and δ114Cd compared to waters outside of the plume, suggesting that the Amazon River is not an important source of Cd to the open ocean. Although the eastern GA11 transect is directly downwind of the Saharan dust plume, atmospheric Cd deposition accounts for <1% of the inferred upwelling flux, indicating that atmospheric inputs to the surface North Atlantic Ocean, even within the main Saharan dust plume, only have a relatively minor influence on the Cd budget. In the subsurface tropical Atlantic (100–200 m water depth), there is a clear deviation from a tight linear Cd-PO4 correlation toward lower Cd concentrations for a given PO4 concentration. Our new Cd data show that this Cd-PO4 decoupling is likely a feature of the entire tropical Atlantic and may possibly reflect PO4 enrichment via preferential re-mineralization of organically-bound phosphorus. Alternatively, the decoupling may arise from subsurface Cd depletion caused by precipitation of Cd sulphide within sinking organic particulate microenvironments, as has been suggested in recent studies.This article is part of a special issue entitled: “Cycles of trace elements and isotopes in the ocean – GEOTRACES and beyond” - edited by Tim M. Conway, Tristan Horner, Yves Plancherel, and Aridane G. González.

Polar Jet Associated Circulation Triggered a Saharan Cyclone and Derived the Poleward Transport of the African Dust Generated by the Cyclone

AbstractIn this study, we identify a new mechanism by which dust aerosols travel over long distances across the eastern side of the North Atlantic Ocean toward the Arctic. The meandering polar jet was at the origin of both dust emission through cyclogenesis over Northwest Africa and poleward transport of the uplifted dust toward the Arctic, through cut‐off circulation. The dust emission was associated with an intense Saharan cyclone that formed over Northwest Africa in early April 2011. The formation of the cyclone was caused by the intrusion into subtropics, of a high‐latitude‐upper‐level trough, linked to the meandering polar jet. The trough initiated cyclogenesis over Northwest Africa after orographic blocking by the Anti‐Atlas Mountains. The still meandering polar jet led to the formation of a cut‐off low further south with which the Saharan dust‐cyclone merged 2 days later and moved northward with the main stream. Beside satellite observations, a simulation at high resolution was performed using the prognostic‐dust permitting model MesoNH. The total dust load carried during this event to areas located north of 40 N was estimated by the model to be 38 Tg and dust deposition was estimated to be 1.3 Tg. The Saharan dust reaching Greenland was accompanied by warm and moist air masses that caused a rise in surface temperature of about 10C for more than 3 consecutive days over the southeastern Greenland. Ice melt over this area of Greenland was detected in the brightness temperature observations.

Science questions and knowledge gaps to study microbial transport and survival in Asian and African dust plumes reaching North America

The Sahara in North Africa and the Gobi and Taklamakan deserts in Asia are the primary sources of mobilized dust in the atmosphere, with regional or global airborne transport estimated at 2 to 5 billion tonnes per year. Annual Asian dust plumes take about 7 to 10 d to cross the Pacific Ocean, and often reach the northwest USA between late February and May. In contrast, the peak season for the movement of African dust storms to the southeastern USA is typically June to August, and dust plumes take about 5 to 7 d to reach Florida. Although studies have documented that a wide range of bacteria, fungi, archaea, and viruses in dust plumes reach the USA each year, little is known about temporal and spatial variability in the microbial biodiversity in transoceanic dust plumes, or the effect on the deposition environments. A scoping study (called the Transoceanic Aerobiology Biodiversity Study) was conducted to develop field-based campaigns centered on examining the abundance, diversity, survival, and impact of microorganisms in transoceanic dust plumes arriving in the continental USA from Asia and Africa. This effort identified Science Questions (SQs) and Knowledge Gaps (KGs) that are highly relevant toward an understanding of the microbial diversity, transport, survival, and dispersal in transoceanic dusts. Science Questions were defined as broad science topics in transoceanic dust plume microbiology that were underexplored by the aerobiology community. Knowledge Gaps were defined as specific project-level research questions for each SQ that represented important topics in the study of transoceanic aerobiology.

Platinum Group Elements, Lanthanoids and Other Metals of Concern in Road Dust and Airborne Particles in Houston, TX

Metal-content of inhalable fine particulate matter (PM2.5 &amp;#8804; 2.5 µm in diameter) can increase the risk of adverse health outcomes while simultaneously providing clues to their origins. A unique aspect of Houston aerosols is their lanthanoid enrichment emanating from crude oil-cracking units in petroleum refineries with smaller contributions from oil combustion and shipping activities. Similarly, concentration pattern of platinum group of elements (PGE) used as unique markers of tailpipe emissions from light-duty vehicles is distorted from the crust in heavily trafficked areas, e.g., Texas. Evidence is also provided for transatlantic North African desert dust and its impact on mass and elemental composition of atmospheric aerosols during summers through detailed elemental analysis. Consequently, comprehensive characterization of airborne particulates for a wide range of elements will assist in identifying and apportioning various natural and anthropogenic sources. Our analytical method recently optimized for simultaneous measurement of three PGEs of Rh, Pd, and Pt, 14 lanthanoids, and numerous other trace- to major-elements will be briefly described in this presentation along with a summary of our measurements in source and receptor particulates in the greater Houston area. Our focus will be on road dust and airborne particulate matter, two important compartments of environmental PGEs, lanthanoids, and other anthropogenically polluted elements. Possible sources of primary particulate emissions and their contributions to PM2.5 mass concentrations in Houston air will also be summarized from source apportionment studies based on elementally characterized receptor data. Finally, compositional differences in ambient PM2.5 under the influence of different source emissions will be discussed using ternary diagrams and abundance pattern of lanthanoids.

North African mineral dust across the tropical Atlantic Ocean: Insights from dust particle size, radiogenic Sr-Nd-Hf isotopes and rare earth elements (REE)

Abstract Large amounts of mineral dust are exported from North Africa across the Atlantic Ocean, impacting the atmosphere and ocean during transport and after deposition through biogeochemical processes. In order to characterize the isotopic signature of dust from different seasons and years, in relation to their bulk particle size, and to obtain a general idea of its provenance, Saharan dust was collected using subsurface sediment traps moored in the tropical North Atlantic Ocean in 2012–2013, and by shipboard aerosol collection during three trans-Atlantic research cruises in 2005, 2012 and 2015. The samples were analysed for radiogenic Strontium (Sr), Neodymium (Nd), and Hafnium (Hf) isotopes, rare earth element (REE; La-Lu) abundances and particle size. In addition, soil sediments from Mauritania, a potential source area, were analysed and compared to the Atlantic dust samples. The results indicate no relation between Sr and Nd isotopic compositions and dust particle size. In contrast, Hf isotopic compositions show a strong relation with particle size, associated to the so-called zircon effect. We explored alternative sources of lithogenic particles to the sediment traps such as Amazon River sediments. Our results reveal that the sediment-trap samples bear distinctly different geochemical signatures from sediments from the Amazon Basin and Amazon River tributaries, and confirm that the primary source of lithogenic particles is northern Africa. The collected dust samples show close relations to African dust aerosols collected at Barbados and samples from the Bodele Depression, although differences between seasons are observed, which we relate to differences in source areas.

The implementation of NEMS GFS Aerosol Component (NGAC) Version 2.0 for global multispecies forecasting at NOAA/NCEP – Part 2: Evaluation of aerosol optical thickness

Abstract. An accurate representation of aerosols in global numerical weather prediction (NWP) models is important to predict major air pollution events and to also understand aerosol effects on short-term weather forecasts. Recently the global aerosol forecast model at NOAA, the NOAA Environmental Modeling System (NEMS) GFS Aerosol Component (NGAC), was upgraded from its dust-only version 1 to include five species of aerosols (black carbon, organic carbon, sulfate, sea salt and dust). This latest upgrade, now called NGACv2, is an in-line aerosol forecast system providing three-dimensional aerosol mixing ratios along with aerosol optical properties, including aerosol optical thickness (AOT), every 3 h up to 5 days at global 1∘×1∘ resolution. In this paper, we evaluated nearly 1.5 years of model AOT at 550 nm with available satellite retrievals, multi-model ensembles and surface observations over different aerosol regimes. Evaluation results show that NGACv2 has high correlations and low root mean square errors associated with African dust and also accurately represented the seasonal shift in aerosol plumes from Africa. Also, the model represented southern African and Canadian forest fires, dust from Asia, and AOT within the US with some degree of success. We have identified model underestimation for some of the aerosol regimes (particularly over Asia) and will investigate this further to improve the model forecast. The addition of a data assimilation capability to NGAC in the near future is expected to provide a positive impact in aerosol forecast by the model.

Application of satellite observations in conjunction with aerosol reanalysis to characterize long-range transport of African and Asian dust on air quality in the contiguous U.S.

A methodology utilizing multiple aerosol measurements and reanalysis was developed to analyze the long-range transport (LRT) of North African and Asian dust events and their effect on contiguous U.S. (CONUS) air quality.Two events in 2015, that originated inland from North Africa and Asia, were detected with aerosol optical depth (AOD) greater than 0.8 over the Gulf of Mexico (June 21) and west coast of Oregon and Washington (April 19). Large amounts of dust were rising over Sahara-Sahel and Taklamakan deserts during these events. For the North African dust event, dust remained the dominant aerosol species transporting from North Africa to CONUS. For Asian dust, before the Taklamakan dust outbreak traveled across the Pacific Ocean, it mixed with sulfate from East China and organic carbons from Siberia. The trans-Atlantic North African dust emerged and compressed below 5 km over the Azores High, whereas the trans-Pacific Asian dust entered the westerlies (5–10 km) along with the mid-latitude frontal system.For the two cases examined, the North African dust event tended to have more influence on CONUS air quality. During the LRT periods, there were 4 of 17 rural and suburban stations (with AOD > 0.5 as the LRT dust approached) in Texas and Louisiana reporting PM2.5 daily maximum observations greater than 36.3 μg m−3. In contrast, the Asian dust stayed above ground level, and all of the 4 rural and suburban stations (with AOD > 0.5 as the LRT dust approached) in Washington and Oregon observed daily maximum PM2.5 below 22.4 μg m−3. The integration of measurements and modeling was able to successfully characterize the sources and transport patterns of the LRT dust events, and differentiate their influence on CONUS air quality. Even though there was high AOD from the Asian LRT dust detected over the western CONUS, significant impacts on surface air quality was not observed as the dust remained aloft.

Characterizing the Impact of Aerosols on Pre-Hurricane Sandy

This study focuses on the role that African dust over the Atlantic had on the persistence of the tropical system that eventually became Hurricane Sandy in October 2012. On October 8, a Saharan dust event in the Mauritania region of West Africa transported significant amounts of mineral dust into the troposphere and along the path of an easterly wave created by a break in the Intertropical Convergence Zone (ITCZ). The Terra/Aqua-MODIS satellite observations clearly define the spatial distribution of the coarse/fine aerosols, while the CALIPSO observations of the total attenuated backscatter at 532 nm provide a detailed view of the vertical structure and aerosol types in the dust-laden layer. European Centre for Medium-Range Weather Forecasts and Modern-Era Retrospective Analysis for Research and Applications, Version 2 reanalysis data show the distribution of aerosols along the path of the pre-Sandy wave as well as a second wave that formed north of the ITCZ under different condition. The second wave, which started in an area of relatively larger aerosol optical depth (AOD), moved into an area with abnormally low convective available potential energy and AOD, subsequently dying out, while the wave that became Sandy had light aerosol loading (AOD between 0.15–0.5) along a majority of its path. The evidence suggests that aerosols played a nontrivial role in the maintenance of this system until it moved into an environment favorable for cyclogenesis.

Day by day evolution of a vigorous two wave Saharan dust storm – Thermal and air quality impacts

This paper conducts a day-by-day analysis of an intense Saharan dust storm that struck Athens (Greece) during April 2008 and consisted of two main dust waves (the first from 10/04/2008 to 14/04/2008 and the second from 19/04/2008 to 22/04/2008). Daily satellite data (1o × 1o resolution) of aerosol optical depth (AOD) were used, in order to follow the course of two dust plumes originated in North Africa through the eastern Mediterranean. Ground based measurements of particle concentrations (PM 10 and PM 2.5 ) and meteorological parameters (wind speed, air temperature, relative humidity and visibility) were also studied. The time intervals before and after each dust wave were taken under consideration, aiming to identify the atmospheric circulation that generated the dust storm and also the clearing mechanisms that removed the African dust from the Athenian atmosphere. Backward air mass trajectories isolated the source of the two dust plumes over Libya and Tunisia, where extreme daily AOD values were recorded. The transportation of dust in the Greek region, during both dust waves, was associated with south westerlies airflows attributed to the advent of low pressure systems from the Atlantic. The impact of both dust waves in Athens was interrupted by the prevalence of a strong north westerlies air stream, which carried the particles eastwards through Turkey, Cyprus and the Middle East. During this dust event, air quality in Athens was severely downgraded, but no thermal discomfort has occurred, according to the estimation of a Pollution Index (PI) and a Discomfort Index (DI), respectively. A drop in visibility was also reported.

Seasonal radiogenic isotopic variability of the African dust outflow to the tropical Atlantic Ocean and across to the Caribbean

In order to assess the impact of mineral dust on climate and biogeochemistry, it is paramount to identify the sources of dust emission. In this regard, radiogenic isotopes have recently been used successfully for tracing North African dust provenance and its transport across the tropical Atlantic to the Caribbean. Here we present two time series of radiogenic isotopes (Pb, Sr and Nd) in dusts collected at the Cape Verde Islands and Barbados in order to determine the origin of the dust and examine the seasonality of westerly dust outflow from Northern Africa. Aerosol samples were collected daily during two campaigns – February 2012 (winter) and June–July 2013 (summer) – at the Cape Verde Atmospheric Observatory (CVAO) on the island of São Vicente (16.9°N, 24.9°W). A one-year-long time series of aerosols from Barbados (13.16°N, 59.43°W) – a receptor region in the Caribbean – was sampled at a lower, monthly resolution.Our results resolve a seasonal isotopic signal at Cape Verde shown by daily variations, with a larger radiogenic isotope variability in winter compared to that in summer. This summer signature is also observed over Barbados, indicating similar dust provenance at both locations, despite different sampling years. This constrains the isotope fingerprint of Saharan Air Layer (SAL) dust that is well-mixed during its transport. This result provides unequivocal evidence for a permanent, albeit of variable strength, long-range transport of African dust to the Caribbean and is in full agreement with atmospheric models of North African dust emission and transport across the tropical Atlantic in the SAL.The seasonal isotopic variability is related to changes in the dust source areas – mainly the Sahara and Sahel regions – that are active all-year-round, albeit with variable contributions in summer versus the winter months. Our results provide little support for much dust contributed from the Bodélé Depression in Chad – the “dustiest” place on Earth – reaching Cape Verde and Barbados during the summer, while contributions during the winter months are likely patchy and minor at most.Importantly, a short-term isotopic excursion is resolved in the Cape Verde winter record during a dust outbreak on 06–08 February 2012. This features a highly radiogenic Pb and Sr and unradiogenic Nd signature, marking a clear shift in dust provenance relative to that of normal days. As the dust storm waned, continuous gradual changes are observed, reflecting mixing and progressive dilution with dust typical of normal days. These inferences from radiogenic isotope tracers are corroborated by both satellite images (CALIPSO and MODIS) and back-trajectory analyses. The radiogenic isotope fingerprinting of these presently-active North African dust sources, and especially the Saharan Air Layer, will prove invaluable in studies of past dust emission from Northern Africa, where imagery and back trajectory analysis are unavailable.

Supporting Weather Forecasters in Predicting and Monitoring Saharan Air Layer Dust Events as They Impact the Greater Caribbean

AbstractDuring the spring and summer months, the greater Caribbean region typically experiences pulses of moderate to heavy episodes of airborne African dust concentrations that originate over the Sahara Desert and propagate westward across the tropical North Atlantic basin. These dust episodes are often contained within the Saharan air layer (SAL), an elevated air mass (between 850–500 hPa) marked by very dry and warm conditions within the lowest levels. During its westward transport, the SAL’s distinct environmental characteristics can persist well into the Gulf of Mexico and southern United States. As a result, the Caribbean population is susceptible to airborne dust levels that often exceed healthy respiratory limits. One of the major responsibilities within the National Weather Service in San Juan, Puerto Rico (NWS-PR), is preparing the public within their area of responsibility (AOR) for such events. The Naval Research Laboratory Marine Meteorology Division (NRL-MMD) is sponsored by the National Oceanic and Atmospheric Administration (NOAA) to support the NWS-PR by providing them with an invaluable “one stop shop” web-based resource (hereafter SAL-WEB) that is designed to monitor these African dust events. SAL-WEB consists of near-real-time output generated from ground-based instruments, satellite-derived imagery, and dust model forecasts, covering the extent of dust from North Africa, westward across the Atlantic basin, and extending into Mexico. The products within SAL-WEB would serve to augment the Advanced Weather Interactive Processing System (AWIPS-II) infrastructure currently in operation at the NWS-PR. The goal of this article is to introduce readers to SAL-WEB, along with current and future research underway to provide improvements in African dust prediction capabilities.

Surface Winds and Dust Biases in Climate Models

AbstractAn analysis of North African dust from models participating in the Fifth Climate Models Intercomparison Project (CMIP5) suggested that, when forced by observed sea surface temperatures, these models were unable to reproduce any aspects of the observed year‐to‐year variability in dust from North Africa. Consequently, there would be little reason to have confidence in the models' projections of changes in dust over the 21st century. However, no subsequent study has elucidated the root causes of the disagreement between CMIP5 and observed dust. Here I develop an idealized model of dust emission and then use this model to show that, over North Africa, such biases in CMIP5 models are due to errors in the surface wind fields and not due to the representation of dust emission processes. These results also suggest that because the surface wind field over North Africa is highly spatially autocorrelated, intermodel differences in the spatial structure of dust emission have little effect on the relative change in year‐to‐year dust emission over the continent. I use these results to show that similar biases in North African dust from the NASA Modern Era Retrospective analysis for Research and Applications (MERRA) version 2 surface wind field biases but that these wind biases were not present in the first version of MERRA.

Sr–Nd–Hf isotopic fingerprinting of transatlantic dust derived from North Africa

Long-range transport of African dust plays an important role in understanding dust-climate relationships including dust source areas, dust pathways and associated atmospheric and/or oceanic processes. Clay-sized Sr–Nd–Hf isotopic compositions can be used as geochemical fingerprints to constrain dust provenance and the pathways of long-range transported mineral dust. We investigated the clay-sized Sr–Nd–Hf isotopic composition of surface samples along four transects bordering the Sahara Desert. The transects are from Mali, Niger/Benin/Togo, Egypt and Morocco. Our results show that the Mali transect on the West African Craton (WAC) produces lower εNd (εNd-mean = −16.38) and εHf (εHf-mean = −9.59) values than the other three transects. The Egyptian transect exhibits the lowest 87Sr/86Sr ratios (87Sr/86Srmean = 0.709842), the highest εHf (εHf-mean = −0.34) and εNd values of the four transects. Comparison of the clay-sized Sr–Nd–Hf isotopic values from our North African samples to transatlantic African dust collected in Barbados demonstrates that the dust's provenance is primarily the western Sahel and Sahara as well as the central Sahel. Summer emission dust is derived mainly from the western Sahel and Sahara regions. The source of transatlantic dust in spring and autumn is more varied than in the summer and includes dust not only from western areas, but also south central areas. Comparison of the Sr–Nd–Hf isotopic fingerprints between the source and sink of transatlantic dust also suggests that a northwestward shift in dust source occurs from the winter, through the spring and into the summer. The isotopic data we develop here provide another tool for discriminating changes in dust archives resulting from paleoenvironmental evolution of source regions.

Linking Barbados Mineral Dust Aerosols to North African Sources Using Elemental Composition and Radiogenic Sr, Nd, and Pb Isotope Signatures

AbstractLarge quantities of African dust are carried across the Atlantic to the Caribbean Basin and southern United States where it plays an important role in the biogeochemistry of soils and waters and in air quality. Dusts' elemental and isotopic composition was comprehensively characterized in Barbados during the summers of 2013 and 2014, the season of maximum dust transport. Although total suspended insoluble particulate matter (TSIP) mass concentrations varied significantly daily and between the two summers, the abundances (μg element/g TSIP) of 50 elements during “high‐dust days” (HDD) were similar. Aerosols were regularly enriched in Na, Cu, Zn, As, Se, Mo, Cd, Sn, Sb, and W relative to the upper continental crust. Enrichment of these elements, many of which are anthropogenically emitted, was significantly reduced during HDD, attributed to mixing and dilution with desert dust over source regions. Generally, Ti/Al, Si/Al, Ca/Al, Ti/Fe, Si/Fe, and Ca/Fe ratios during HDD differed from their respective values in hypothesized North African source regions. Nd isotope composition was relatively invariant for “low‐dust days” (LDD) and HDD. In contrast, HDD‐aerosols were more radiogenic exhibiting higher 87Sr/86Sr, 206Pb/204Pb, 207Pb/204Pb, and 208Pb/204Pb ratios compared to LDD. Generally, Barbados aerosols' composition ranged within narrow limits and was much more homogeneous than that of hypothesized African source soils. Our results suggest that summertime Barbados aerosols are dominated by a mixture of particles originating from sources in the Sahara‐Sahel regions. The Bodélé Depression, long suspected as a major source, appears to be an insignificant contributor of summertime western Atlantic dust.

Performance Evaluation of WRF-CHEM in Simulating Harmattan Dust over West Africa

In this study, we investigated the ability of Weather Research and Forecasting model coupled with the Chemistry option (WRF-Chem) using the GOCART dust scheme in capturing the spatial and temporal distribution of a severe dust storm which occurred in March 2006 over West Africa. The period (5th - 14th March, 2006) also coincided with the African Monsoon Multidisciplinary Analysis (AMMA) Special Observing Period (SOP) and some observed datasets from other platforms were also used. The WRF-Chem simulation was performed on a two-way nested domain in order to resolve the dust episode on high horizontal resolution dataset. From the 5th March, a dust storm raised in northern Algeria, which propagated southward spreading to the west and east on the subsequent days. Over the Gulf of Guinea, an intense dust haze was transported southward thereby generating an aerosol optical thickness (AOT) greater than 4 over Nigeria. Qualitative and quantitative characterizations between observations and WRF-Chem simulations demonstrated that the WRF-Chem model is highly efficient and can be recommended to simulate the spatial and temporal distribution of harmattan dust over West Africa. We discovered that the WRFChem modelled Aerosol Optical Depth (AOD) underestimated the AOD from AERONET as a result of all other aerosols like black carbon integrated into the observed which is not yet captured by model. The quantitative and qualitative analysis of the model output ascertain the capability of WRF-Chem to reasonably reproduce West African harmattan dust haze from the time and location of being raised to its transportation and propagation and hence its final settling or disappearance over the continental area of West Africa. Model simulation was able to partition the dust particles into five different sizes. It was discovered that dust particles of sizes 1.4 μm, 2.4 μm and 4.5 μm are more prevalent among other sizes from the raised and transported dust over West Africa.

Analysis of the Impact of African Dust Storms on the Presence of Enteric Viruses in the Atmosphere in Tenerife, Spain

ABSTRACT Airborne viruses and their relation to dust storms, as a possible route for dispersion, have not been widely investigated. There are, however, studies that have described the airborne dispersal of pathogenic viruses and their potential impact on public and agronomical health. Atmospheric samples were collected in an urban area of Tenerife during 2009, 2010, 2012 and 2013 and screened for the presence of enteric viruses using PCR and sequencing. The potential relationship of viral data with African dust storms and other climatic variables (viz., the seasonality, origin of the air mass and PM levels) was analyzed. Enteroviruses and Rotaviruses were detected in 15.4% (20/130) and 36.9% (48/130) of the samples, respectively. No significant statistical relationships were observed with African dust storms or the origin of the air masses, although higher percentages of positives were obtained for dust storm days. Enterovirus detection was significantly linked to warmer seasons, and PM2.5 levels showed an inverse correlation with a rotaviral presence. This is the first multi-year report to describe the presence of Enterovirus and Rotavirus genetic sequences in air samples collected in an outdoor urban environment. The data illustrates the need for source region sampling to determine links and the influence of the weather and climatic and regional wind patterns on long-range atmospheric dispersion of viruses in future research efforts.

Millennial-scale variations in dustiness recorded in Mid-Atlantic sediments from 0 to 70 ka

Sedimentary records of dust deposition in the subtropical Atlantic provide important constraints on millennial- and orbital-scale variability in atmospheric circulation and North African aridity. Constant flux proxies, such as extraterrestrial helium-3, yield dust flux records that are independent of the biases caused by lateral sediment transport and limited resolution that may be associated with age-model-derived mass accumulation rates. However, Atlantic dust records constrained using constant flux proxies are sparsely distributed and generally limited to the past 20 ka. Here we extend the Atlantic record of North African dust deposition to 70 ka using extraterrestrial helium-3 and measurements of titanium, thorium, and terrigenous helium-4 in two sediment cores collected at 26°N and 29°N on the Mid-Atlantic Ridge and compare results to model estimates for dust deposition in the subtropical North Atlantic. Dust proxy fluxes between 26°N and 29°N are well correlated, despite variability in lateral sediment transport, and underscore the utility of extraterrestrial helium-3 for constraining millennial-scale variability in dust deposition. Similarities between Mid-Atlantic dust flux trends and those observed along the Northwest African margin corroborate previous interpretations of dust flux variability over the past 20 ka and suggest that long distance transport and depositional processes do not overly obscure the signal of North African dust emissions. The 70 ka Mid-Atlantic record reveals a slight increase in North African dustiness from Marine Isotope Stage 4 through the Last Glacial Maximum and a dramatic decrease in dustiness associated with the African Humid Period. On the millennial-scale, the new records exhibit brief dust maxima coincident with North Atlantic cold periods such as the Younger Dryas, and multiple Heinrich Stadials. The correlation between Mid-Atlantic dust fluxes and previous constraints on North African aridity is high. However, precipitation exerts less control on dust flux variability prior to the African Humid Period, when wind variability governs dust emissions from consistently dry dust source regions. Thus, the Mid-Atlantic dust record supports the hypothesis that both aridity and wind strength drive dust flux variability across changing climatic conditions.

Measurements of windblown dust characteristics and ocean fertilization potential: The ephemeral river valleys of Namibia

Abstract Delivery of nutrients to the ocean by mineral aerosol deposition involves complex biogeochemical interactions that include atmospheric processing, dissolution and biotic uptake of available nutrients in the surface waters. Research into the fertilization potential of aeolian dust is currently constrained by a lack of understanding of the nutrient composition and bioavailability in dust source areas. Further, research into hot-spots of dust emission has largely focused on paleo-lacustrine sources and pans, to the detriment of other potential sources such as ephemeral river valleys in desert regions. Here, we investigate the sediment characteristics and nutrient content of windblown and surface sediments of a largely overlooked southern African dust source, Namibia’s ephemeral river valleys. We deployed monitoring equipment in three river valleys to capture deflated sediments and monitor airborne dust concentration and meteorological conditions throughout an annual dust season. Our results show that windblown dust within the river valleys is easily transportable offshore from Namibia over the Benguela Upwelling System, an intensely productive region of the South Atlantic Ocean. We demonstrate that the windblown dust contains iron, phosphorus and nitrogen nutrients, each of which may positively impact primary production rates when deposited in the complex upwelling system. The river valley dust has a significantly higher content of nutrients than either of southern Africa’s major dry lake bed dust sources, Etosha and Makgadikgadi Pans. This aeolian work builds on previous source sediment findings proposing the ephemeral river valleys of Namibia as regionally important sources of dust with enhanced ocean fertilisation potential.

The Role of African Dust in Atlantic Climate During Heinrich Events

AbstractIncreased ice discharge in the North Atlantic is thought to cause a weakening, or collapse, of the Atlantic meridional overturning circulation (AMOC) during Heinrich events. Paleoclimate records indicate that these periods were marked by severe tropical aridity and dustiness. Although the driver of these events is still under debate, large freshwater input is necessary for climate models to simulate the magnitude, geographical extent, and abruptness of these events, indicating that they may be missing feedbacks. We hypothesize that the dust‐climate feedback is one such feedback that has not been previously considered. Here we analyze the role of dust‐climate feedbacks on the AMOC by parameterizing the dust radiative effects in an intermediate complexity model and consider uncertainties due to wind stress forcing and the magnitude of both atmospheric dust loading and freshwater hosing. We simulate both stable and unstable AMOC regimes by changing the prescribed wind stress forcing. In the unstable regime, additional dust loading during Heinrich events cools and freshens the North Atlantic and abruptly reduces the AMOC by 20% relative to a control simulation. In the stable regime, however, additional dust forcing alone does not alter the AMOC strength. Including both freshwater and dust forcing results in a cooling of the subtropical North Atlantic more comparable to proxy records than with freshwater forcing alone. We conclude that dust‐climate feedbacks may provide amplification to Heinrich cooling by further weakening AMOC and increasing North Atlantic sea ice coverage.