Aerosol Optical Characteristics Research Articles

Annual and Seasonal Variations in Aerosol Optical Characteristics in the Huai River Basin, China from 2007 to 2021

Over the past three decades, China has seen aerosol levels substantially surpass the global average, significantly impacting regional climate. This study investigates the long-term and seasonal variations of aerosols in the Huai River Basin (HRB) using MODIS, CALIOP observations from 2007 to 2021, and ground-based measurements. A notable finding is a significant decline in the annual mean Aerosol Optical Depth (AOD) across the HRB, with MODIS showing a decrease of approximately 0.023 to 0.027 per year, while CALIOP, which misses thin aerosol layers, recorded a decrease of about 0.016 per year. This downward trend is corroborated by improvements in air quality, as evidenced by PM2.5 measurements and visibility-based aerosol extinction coefficients. Aerosol decreases occurred at all heights, but for aerosols below 800 m, with an annual AOD decrease of 0.011. The study also quantifies the long-term trends of five major aerosol types, identifying Polluted Dust (PD) as the predominant frequency type (46%), which has significantly decreased, contributing to about 68% of the total AOD reduction observed by CALIOP (0.011 per year). Despite this, Dust and Polluted Continental (PC) aerosols persist, with PC showing no clear trend of decrease. Seasonal analysis reveals aerosol peaks in summer, contrary to surface measurements, attributed to variations in the Boundary Layer (BL) depth, affecting aerosol distribution and extinction. Furthermore, the study explores the influence of seasonal wind patterns on aerosol type variation, noting that shifts in wind direction contribute to the observed changes in aerosol types, particularly affecting Dust and PD occurrences. The integration of satellite and ground measurements provides a comprehensive view of regional aerosol properties, highlighting the effectiveness of China’s environmental policies in aerosol reduction. Nonetheless, the persistence of high PD and PC levels underscores the need for continued efforts to reduce both primary and secondary aerosol production to further enhance regional air quality.

Aerosol Vertical Structure and Optical Properties during Two Dust and Haze Episodes in a Typical Valley Basin City, Lanzhou of Northwest China

The vertical profiles of aerosol optical properties are vital to clarify their transboundary transport, climate forcing and environmental health influences. Based on synergistic measurements of multiple advanced detection techniques, this study investigated aerosol vertical structure and optical characteristics during two dust and haze events in Lanzhou of northwest China. Dust particles originated from remote deserts traveled eastward at different altitudes and reached Lanzhou on 10 April 2020. The trans-regional aloft (~4.0 km) dust particles were entrained into the ground, and significantly modified aerosol optical properties over Lanzhou. The maximum aerosol extinction coefficient (σ), volumetric depolarization ratio (VDR), optical depth at 500 nm (AOD500), and surface PM10 and PM2.5 concentrations were 0.4~1.5 km−1, 0.15~0.30, 0.5~3.0, 200~590 μg/m3 and 134 μg/m3, respectively, under the heavy dust event, which were 3 to 11 times greater than those at the background level. The corresponding Ångström exponent (AE440–870), fine-mode fraction (FMF) and PM2.5/PM10 values consistently persisted within the ranges of 0.10 to 0.50, 0.20 to 0.50, and 0.20 to 0.50, respectively. These findings implied a prevailing dominance of coarse-mode and irregular non-spherical particles. A severe haze episode stemming from local emissions appeared at Lanzhou from 30 December 2020 to 2 January 2021. The low-altitude transboundary transport aerosols seriously deteriorated the air quality level in Lanzhou, and aerosol loading, surface air pollutants and fine-mode particles strikingly increased during the gradual strengthening of haze process. The maximum AOD500, AE440–870nm, FMF, PM2.5 and PM10 concentrations, and PM2.5/PM10 were 0.65, 1.50, 0.85, 110 μg/m3, 180 μg/m3 and 0.68 on 2 January 2021, respectively, while the corresponding σ and VDR at 0.20–0.80 km height were maintained at 0.68 km−1 and 0.03~0.12, implying that fine-mode and spherical small particles were predominant. The profile of ozone concentration exhibited a prominent two-layer structure (0.60–1.40 km and 0.10–0.30 km), and both concentrations at two heights always remained at high levels (60~72 μg/m3) during the entire haze event. Conversely, surface ozone concentration showed a significant decrease during severe haze period, with the peak value of 20~30 μg/m3, which was much smaller than that before haze pollution (~80 μg/m3 on 30 December). Our results also highlighted that the vertical profile of aerosol extinction coefficient was a good proxy for evaluating mass concentrations of surface particulate matters under uniform mixing layers, which was of great scientific significance for retrieving surface air pollutants in remote desert or ocean regions. These statistics of the aerosol vertical profiles and optical properties under heavy dust and haze events in Lanzhou would contribute to investigate and validate the transboundary transport and radiative forcing of aloft aerosols in the application of climate models or satellite remote sensing.

Aerosol optical and radiative characteristics under contrasting pollution conditions in a typical urban valley in Northwestern China

Aerosol optical and radiative properties play a key role in climate change. Precisely pinpointing the optical and radiative properties of various types of aerosols during diverse pollution events in urban settings remains a challenge. In this study, aerosol optical and radiative properties under contrasting pollution conditions were investigated, including dusty, haze, fireworks, and clean days, in a typical urban valley in Northwestern China, based on observations from the Sun-Sky photometers and simulations from libRadtran. The results show that on dusty days aerosols have high absorption and low backscattering, while on haze days they are characterized by fine, absorptive organic aerosol particles with pronounced forward scattering in the ultraviolet and visible spectra. On fireworks days during Chinese New Year (CNY), fine-mode aerosols from fireworks dominate, with the highest scattering and the lowest absorption under the four pollution conditions, and the particle peak radius growth responds rapidly to changes in relative humidity. Aerosols generally cause Earth's surface cooling and atmospheric warming across various pollution conditions. Notably, dusty days, clean days, and haze days all exhibit a lower positive aerosol radiative forcing (ARF) in the ultraviolet (UV) spectrum at the top of the atmosphere (TOA) due to lower single-scattering albedo (SSA). In contrast, CNY uniquely displays negative UV_ARF at TOA, attributed to high-SSA non-absorptive particles. Aerosols on dusty days have higher positive radiative forcing than on haze days, emphasizing the absorptive impact of mixed dust aerosols. These findings provide valuable insights into the behavior of aerosols under various pollution conditions in a typical urban valley, contributing to a better understanding of the environmental effects of various aerosols in arid urban regions.

Optical Characteristics of Aerosol and Carbon Monoxide Content in the Atmosphere over Irkutsk Oblast and Buryatia in 2010–2021

Optical Characteristics of Aerosol and Carbon Monoxide Content in the Atmosphere over Irkutsk Oblast and Buryatia in 2010–2021

Investigation of the characteristics of atmospheric and meteorological parameters of a severe dust storm in the Mumbai during January 2022

In recent years, India has experienced frequent dust storms, which have a significant impact on local climatic conditions. This research focuses on a significant dust storm event that took place in January 2022 across the Arabian Sea and its effects on the Mumbai region. The study utilizes a combination of ground-based measurements and satellite observations of optical parameters to investigate different atmospheric and meteorological parameters. The analysis of aerosol optical characteristics observed through Moderate Resolution Imaging Spectroradiometer (MODIS) and Ozone Monitoring Instrument (OMI) data indicates significant variations during the dust storm day in comparison to pre- and post-dust storm days. There is a huge surge in the Aerosol Optical Depth (AOD) values Ångström Exponent (AE) values decrease. This confirms the presence of coarser particles in the affected region. The elevated values of the Aerosol Index (AI) on dusty days shows the presence of UV-absorbing aerosols. The ground-based measurements obtained by Central Pollution Control Board (CPCB) in the Mumbai region shows a rapid surge in the PM concentrations during the dust storm day. This study also highlights the change in the meteorological conditions associated with the occurrence of dust storm. The back trajectory analysis shows that most of the air-mass parcels transported from the Arabian Sea. The findings of this study collectively emphasize the substantial impact of dust storms on local atmospheric chemistry and the climatic system.

The Aerosol Optical Characteristics in Different Dust Events Based on a 532 nm and 355 nm Polarization Lidar in Beijing

Extreme weather events are happening more frequently as a result of global climate change. Dust storms broke out in the spring of 2017 in China and drastically impacted the local air quality. In this study, a variety of data, including aerosol vertical profiles, surface particle concentration, meteorological parameters, and MODIS–derived aerosol optical depth, as well as backward trajectory analysis, were employed to analyze two dust events from April to May in Beijing. The dust plumes were mainly concentrated below 0.8 km, with peak PM10 values of 1000 μg·m−3 and 300 μg·m−3 in the two cases. The aerosols showed different vertical distribution characteristics. The pure dust in case 1 from 4 to 5 May 2017 had a longer duration (2 days) and presented a larger aerosol extinction coefficient (2.27 km−1 at 355 nm and 1.25 km−1 at 532 nm) than that of the mixed dust in case 2 on 17 April 2017 (2.01 km−1 at 355 nm and 1.33 km−1 at 532 nm). The particle depolarization ratio (PDR) remained constant (0.24 ± 0.03 in case 1) from the surface to 0.8 km in height. In contrast, the PDR profile in the mixed dust (case 2) layer was split into two regions—large values exceeding 0.15 above 0.6 km and small values of 0.11 ± 0.03 below 0.6 km. The influence of meteorological information on aerosol distribution was also investigated, and wind was predominant through the observing period. The pure dust in case 1 was mainly from Mongolia, with strong northwest winds, while the near-surface mixed pollution was caused by the combination of long-transported sand and local emission. Furthermore, lidar-derived profiles of dust mass concentrations in the two cases were presented. This study reveals the vertical characteristics of dust aerosols in the production and dissipation of localized dust events and confirms the efficacy of thorough observations with multiple approaches from the ground to space to monitor dust events in real time.

Profiling of Aerosols and Clouds over High Altitude Urban Atmosphere in Eastern Himalaya: A Ground-Based Observation Using Raman LIDAR

Profiles of aerosols and cloud layers have been investigated over a high-altitude urban atmosphere in the eastern Himalayas in India, for the first time, using a Raman LIDAR. The study was conducted post-monsoon season over Darjeeling (latitude 27°01′ N longitude 88°36′ E, 2200 masl), a tourist destination in north-eastern India. In addition to the aerosols and cloud characterization and atmospheric boundary layer detection, the profile of the water vapor mixing ratio has also been analyzed. Effects of atmospheric dynamics have been studied using the vertical profiles of the normalized standard deviation of RCS along with the water vapor mixing ratio. The aerosol optical characteristics below and above the Atmospheric Boundary Layer (ABL) region were studied separately, along with the interrelation of their optical and microphysical properties with synoptic meteorological parameters. The backscatter coefficient and the extinction coefficient were found in the range from 7.15×10−10 m−1 sr−1 to 3.01×10−5 m−1 sr−1 and from 1.02×10−5 m−1 to 2.28×10−3 m−1, respectively. The LIDAR ratio varies between 3.9 to 78.39 sr over all altitudes. The variation of the linear depolarization ratio from 0.19 to 0.32 indicates the dominance, of non-spherical particles. The periodicity observed in different parameters may be indicative of atmospheric wave phenomena. Cloud parameters, such as scattering coefficients, top and bottom height, and optical depth for different cloud phases, have been evaluated. A co-located Micro Rain Radar has been used with LIDAR for cloud life cycle study.

The Vertical Distributions of Aerosol Optical Characteristics Based on Lidar in Nanyang City from 2021 to 2022

To investigate the vertical distribution of aerosol optical characteristics in Nanyang City, a ground-based dual-wavelength (532 nm and 355 nm) lidar system was developed for aerosol observation at the Nanyang Normal University Station (NYNU) from November 2021 to December 2022. Spatio-temporal dynamics information on vertical distributions of aerosol optical properties during polluted and non-polluted days was obtained. Aerosols were characterized by low altitudes (up to 2 km), thinner layers, and high-altitude (up to 4 km) thick layers during non-polluted and polluted days, with extinction coefficient values of ~0.03 km−1 and ~0.2 km−1, respectively. The mean values of the extinction coefficient at different altitudes (0~5 km) were all about ten-times higher on polluted days (0.04~0.19 km−1) than on non-polluted days (0.004~0.02 km−1). These results indicate that aerosol loadings and variations at different altitudes (0~5 km) were much higher and more prominent on polluted days than non-polluted days. The results show ten-times larger aerosol optical depth (AOD) values (0.4~0.6) on polluted days than on non-polluted days (0.05~0.08). At the same time, AOD values on both polluted and non-polluted days slightly decreased from 19:00 to 05:00, possibly due to dry depositions at nighttime. For the first time, this study established a ground-based lidar remote sensing system to investigate the vertical distribution of atmospheric aerosol optical characteristics in Henan Province. The experimental results can provide scientific dataset support for the local government to prevent and control air pollution.

Variations in aerosol optical characteristics from SKYNET measurements in Beijing

Atmospheric aerosols have significant impacts on climate and environment, so the study on aerosol optical properties is of great scientific significance for climate change and atmospheric environment. The variations in column-integrated aerosol optical properties over Beijing were investigated from March 2016 to December 2019 based on the SKYNET data products. Higher values of AOD and AE found in summer indicate that it is important to pay more attention to fine particle pollution in summer. By fitting the AOD data of SKYNET with AERONET at same waveband, we found that monthly variations in aerosol optical depth estimated from SKYNET observation were mostly consistent with the AERONET data. Aerosols were divided into several modes according to optical characteristics, which deepen some insight into aerosol optical and radiative properties and revealed that the weak absorption aerosol dominated and contributed much to the radiation transport in Beijing. Data derived from the polarization lidar CALIPSO were combined with aerosol optical depth (AOD) from SKYNET and these results were consistent, which further identified the scientific of data. The random forest algorithm was used to interpolate the missing AOD500nm observations. The original results and the interpolation results were fitted with MODIS respectively, which proved that the random forest algorithm can supplement the missing results well. This work will be of great significance in addressing the impacts of aerosols on climate and environment, and will help reduce the uncertainty of the impacts of aerosols on the Earth's radiation budget. All work will provide scientific support for the prevention and control of specific pollution.

Aerosol Optical Properties and Types over Southern Africa and Reunion Island Determined from Ground-Based and Satellite Observations over a 13-Year Period (2008–2021)

Fires occur seasonally in Southern Africa, from June to November, increasing tropospheric aerosol loading and triggering harmful consequences for the environment and human health. This study aims to examine 13 years of aerosol optical characteristics and types over Southern Africa and Reunion Island. Using AERONET sun photometers and MODIS observations, we found that a high aerosol optical depth and Angström exponent are associated with two predominant types of aerosols (biomass burning/urban industrial and mixed type) throughout the spring season. According to CALIOP observations, the major aerosol types with occurrence frequencies above 10% are polluted continental/smoke, polluted dust, and elevated smoke, whereas dust, clean continental, and dusty marine have occurrence frequencies below 1%. In comparison to other seasons, the vertical profiles of elevated smoke have different shapes in spring, with a seasonal shift in the peak altitude (from 3–4 km), when fire activity is at its maximum. At these altitudes, the northern regions presented occurrence frequencies of 32% on average, while lower values were found for the southern or farthest regions (<10–20% on average). The Lagrangian HYSPLIT model back-trajectories demonstrated eastward transport, with air masses from South America and the Atlantic Ocean that recirculate around the study sites. The aerosols are mainly derived from active biomass burning areas near the study sites and, to a lesser extent, from remote sources such as South America.

Simulated depolarization ratios for dust and smoke at laser wavelengths: implications for lidar application.

Polarization measurements have been widely used to detect aerosol properties by remote sensing in recent decades. To better understand the polarization characteristics of aerosols by lidar, the numerically exact T-matrix method was used to simulate the depolarization ratio (DR) of dust and smoke aerosols at typical laser wavelengths in this study. The results show that the DRs of dust and smoke aerosols have obviously different spectral dependences. Moreover, the ratio of DRs at two wavelengths has an obvious linear relationship with the microphysical properties of aerosols, including aspect ratio, effective radius and complex refractive index. At short wavelengths, we can use it to invert the absorption characteristics of particles, further improving the detection ability of lidar. Comparing the simulation results of different channels, DR, (color ratio) CR and (lidar ratio) LR have a good logarithmic fitting relationship at 532 nm and 1064 nm, which helps to classify the aerosol types. On this basis, a new inversion algorithm, "1β+1α+2δ", was presented. By this algorithm, the backscattering coefficient (β), extinction coefficient (α), DR (δ) at 532 nm and 1064 nm can be used to expand the range of inversion and compare lidar data with different configurations to obtain more extensive optical characteristics of aerosols. Our study enhances the application of laser remote sensing in aerosol observations more accurately.

Optical Characteristics of Aerosol and Carbon Monoxide Content in the Atmosphere over the Irkutsk Region and Buryatia in 2010–2021

Optical Characteristics of Aerosol and Carbon Monoxide Content in the Atmosphere over the Irkutsk Region and Buryatia in 2010–2021

LOVE IS BLIND. Season 3. 12 episodes. Netflix, 2022.

Religious Studies ReviewVolume 49, Issue 1 p. 69-69 Short Reviews of Recent Publications: Religion, Arts and Culture LOVE IS BLIND. Season 3. 12 episodes. Netflix, 2022. First published: 24 April 2023 https://doi.org/10.1111/rsr.16343Read the full textAboutRelatedInformationPDFPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessClose modalShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL No abstract is available for this article. Volume49, Issue1Special Issue: Unique Approaches to Christianity in Africa and BeyondMarch 2023Pages 69-69 RelatedInformation RecommendedBroadcasting in the Age of NetflixSylvia Harvey, A Companion to Television, [1]Vertical aerosol profiles from Raman polarization lidar observations during the dry season AMMA field campaignBirgit Heese, Matthias Wiegner, Journal of Geophysical Research: AtmospheresNetflix, Inc. and Online TelevisionJane Shattuc, A Companion to Television, [1]Investigating the aerosol optical and radiative characteristics of heavy haze episodes in Beijing during January of 2013Jianrong Bi, Jianping Huang, Zhiyuan Hu, B. N. Holben, Zhiqiang Guo, Journal of Geophysical Research: AtmospheresCognitive styles in hypomanic episodes of bipolar I disorderClaudia Lex, Martin Hautzinger, Thomas D Meyer, Bipolar Disorders

Difference between global and regional aerosol model classifications and associated implications for spaceborne aerosol optical depth retrieval

AbstractAerosol model are generally adopted to describe the physical and optical characteristics of aerosols in different regions, and this is important for climate and environmental studies as well as satellite aerosol retrieval. However, current mainstream aerosol retrieval algorithms still lack differentiated and dynamic descriptions of aerosol models, and the aerosol optical depth (AOD) retrieval accuracy is hence largely compromised. Therefore, in this study, we aimed to investigate the difference between global and regional aerosol model classifications and the impact of these differences on satellite AOD retrieval. We developed global and regional (for China) aerosol models through the K-means cluster analysis method, and used the 6SV radiative transfer model based on these global and regional aerosol models to simulate air pollution events. The cluster analysis revealed that both global and regional aerosols can be clustered into five main aerosol types with different optical and physical parameters. The aerosol types include strongly absorbing, moderately absorbing, weakly absorbing, dust and coarse-fine mixed aerosols. These two aerosol models exhibited distinct seasonal variations. Comparing the clustering results obtained with the two models at five Aerosol Robotic Network (AERONET) sites, we found that the proportion of strongly absorbing aerosols in the global results is low. According to the China clustering results, a higher proportion of strongly absorbing aerosols occurred in autumn, winter, and early spring, and dust aerosols attained an increasing proportion in spring. Comparing the aerosol parameters with observational data, the regional aerosol model performed better than the global aerosol model. Simulations of AOD during a pollution episode and in different seasons at the Beijing-CAMS site with the 6SV radiative transfer model further confirmed that the regional aerosol model achieved a better simulation accuracy than the global model. The findings suggest that regional aerosol models can provide a useful reference for satellite remote sensing algorithm, climate change and air pollution assessment, and that the dynamic description of the aerosol model is a key parameter in satellite AOD retrieval algorithms.

Optical characteristics of aerosol and its potential sources over Nam Co in the Tibetan Plateau during Asian summer monsoon period

Aerosols over the Tibetan Plateau (TP) play an important role in the regional and global climate change and ecological environment. The Second Tibetan Plateau Scientific Expedition and Research Program (STEP) carried out observation experiment at the Nam Co Station for Multisphere Observation and Research, Chinese Academy of Sciences (Nam Co Station, 30°46′N, 90°59′E, 4730 m) in the central TP from August 5 to September 11, 2020. This paper investigated the aerosol optical properties and its potential sources over Nam Co region. The main results are as follow: the average aerosol optical depth was 0.025 during the observation period; the average black carbon (BC) concentration and aerosol number concentration was 37 ng/m3 and 129 N/cm3, respectively; the diurnal variation and vertical distribution of aerosol were affected by the local meteorological elements. Frequent southerly winds during the summer monsoon led to a certain contribution of South Asia to the BC concentration in Nam Co region. And particles from the Taklimakan Desert led to dramatic increasing of aerosol number concentration over Nam Co region. The aerosol optical characteristics and influencing factors over the central TP were analyzed, which is beneficial to further study the influence of aerosols over the TP on regional and global weather and climate.

Wintertime aerosol properties of urban desert region of western India: Implications in regional climate assessment

This study assessed the inter-relation between physiochemical and optical characteristics of aerosols measured at a desert-urban region affected by anthropogenic sources and desert dust during October 2020 to January 2021. Based on horizontal visibility and measured PM2.5 concentration, clear (37 %), light (33 %) and high (31 %) pollution periods were identified. Elemental and organic carbon (50 ± 15 μgm−3; 31 %) and secondary inorganics (53 ± 21 μgm−3; 33 %) dominated the PM2.5 mass (160 ± 4 μgm−3) during high pollution period with low dust (14 ± 7 μgm−3; 8 %) content. Interestingly, the clear pollution period was also influenced by carbonaceous fraction (19 ± 8 μgm−3; 32 %) and secondary inorganics (19 ± 5 μgm−3; 32 %), but the PM2.5 concentrations (59 ± 9 μgm−3) were ∼ one-third as compared to high pollution period. High scattering coefficients were observed which were comparable to highly polluted Indian city like Delhi. An exponential increase in non-absorbing material was observed and showed clear influence on light absorption capacity of EC and dust due to coating/mixing. High absorption Ångström exponent (AAE) >0.6 was observed for the ratio of non-absorbing to light absorbing components (LAC) in the range of 1–2.5 and EC/PM2.5 fraction of 7–14 %. While further increase in non-absorbing to absorbing components ratio > 4 and low amount of EC (<4 %) tend to decrease AAE below 0.4. Higher mass absorption cross-section (>30 m2g−1 of EC) was observed when 4–10 % EC fraction of PM2.5 associated with 1.5–3.5 times non-absorbing components to total absorbing components. Likewise, absorption enhanced by three to five folds compared to uncoated EC for low EC fraction (3–6 %) in PM2.5, but high non-absorbing to absorbing component ratio (>2.5). Interestingly, absorption was minimally amplified for nominal coating fraction associated with significant core materials or vice-versa. These findings have implications not only in regional climate assessment but also for other regions with comparable geography and source-mixes.

Improved Aerosol Lidar Ratio Profile by Introducing Pseudo-Constant

Aerosol lidar ratio (LR) is important for inversion of aerosol optical characteristics. Single aerosol LR value adopted in the inversion not only causes difficulties in improving aerosol inversion accuracy but also hinders the analysis of aerosol types. In this paper, a pseudo-constant method with certain universality is proposed for inverting aerosol LR profiles. Simulation results show a decrease in the mean absolute error (MAE) of the aerosol LR from 3.57% (iteration method) and 9.96% (Fernald method) to 1.82% (pseudo-constant method). In the near-surface region (<1.5 km), the MAE of aerosol LR decreases from 4.97% (iteration) and 21.66% (Fernald) to 1.54% (pseudo-constant). Moreover, the inversion accuracy of aerosol LR obtained from pseudo-constant method is less influenced by the precision of the pre-estimated aerosol LR value than that from iteration method. Experimentally, the aerosol LR and aerosol extinction coefficient profiles obtained from the pseudo-constant method are more accurate than those from the iteration and Fernald methods. In addition, both the simulations and experiments indicate that the pseudo-constant method has higher efficiency; the processing time is shortened from approximately 5 s per signal (iteration) to approximately 0.1 s per signal. Finally, aerosol types can be distinguished to a certain degree by combining the improved aerosol LR profile.

Experimental demonstration of spectral suppression effect improvement for multi-longitudinal mode high-spectral-resolution lidar.

The multi-longitudinal mode high-spectral-resolution lidar (MLM-HSRL) is an effective technique for detecting atmospheric optical characteristics of aerosols. Due to the excessive longitudinal mode numbers, the current MLM-HSRL cannot obtain a well spectral suppression effect, which seriously affects the retrieval accuracy of the optical characteristic parameters. In this paper, a new index called Longitudinal Mode Rejection Ratio (LMRR) has been proposed to evaluate the spectral suppression effect of the MLM-HSRL; a novel mismatch error and mode control (MEMC) technique is proposed to improve the spectral suppression effect of the MLM-HSRL, which contributes to developing the scientific potential of the MLM-HSRL for aerosol remote sensing. Based on our self-developed MLM laser, through controlling the longitudinal mode frequency-pulled shift of the MLM laser, adjusting the total mismatch error, and reducing the longitudinal mode numbers, we realize the LMRR index improved from about 5 to over 30, and the working stability of the system is also promoted by decreasing the longitudinal mode numbers. The experiment well improves the spectral suppression effect and verifies the effectiveness of the proposed MEMC technique. To the best of our knowledge, for the first time, the study addresses the conundrum of the lower spectral suppression effect for the MLM-HSRL. This work would help to provide a powerful support for the high-precision, long-term, and stable operation of the MLM-HSRL in the future.

Aerosol optical properties over an urban industrial area, Raipur, Chhattisgarh, India

Optical properties of aerosols including Aerosol optical depth (AOD), Angstrom exponent (AE) and Single scattering albedo (SSA)) were derived and analyzed for classifying the aerosols and identification of possible sources with percentage contribution over an urban-industrial city Raipur, India, during the year 2019 to 2021. The mean annual values of AOD and AE during 2019–2021 were 0.53 ± 0.2 and 1.20 ± 0.33 respectively, with the highest AOD (AE) values in summer:(0.67 ± 0.21 (0.98 ± 0.13)), spring: (0.52 ± 0.17 (0.93 ± 0.23)), autumn: (0.59 ± 0.21 (1.36 ± 0.26)) and winter: (0.44 ± 0.15 (1.49 ± 0.15)) respectively. The results revealed the dominance of finer aerosols with higher (lower) AE value during the winter (summer) season. Whereas, lower (higher) SSA values during the winter (summer) indicated the presence of absorbing types of aerosols. Based on the aerosol optical characteristics (AOD versus AE), three distinct aerosol types were discovered throughout the study period, namely mixed aerosols (60%), biomass-urban (37%), and dust aerosols (3%). To discriminate between urban and biomass burning aerosols, optical characteristics (AE versus SSA) were examined and found three main sources: mixed aerosols (71%) urban-industrial (21%) and biomass burning aerosols (8%). These findings will be useful for identifying potential sources as well as serve as an input for estimating the radiative forcing caused by regional aerosols.

Novel Inversion Algorithm for the Atmospheric Aerosol Extinction Coefficient Based on an Improved Genetic Algorithm

As an important atmospheric component, aerosols play a very important role in the radiation budget balance of the earth–atmosphere system. To study the optical characteristics of aerosols, it is necessary to use an inversion algorithm to process the lidar return signal to obtain both the aerosol extinction coefficient and the backscattering coefficient. However, the lidar return power equation is ill-conditioned and contains two unknown parameters, meaning that traditional inversion algorithms must be solved by adopting certain assumptions (e.g., a uniform atmosphere and the lidar ratio), which to a certain extent can seriously affect the inversion accuracy. Here, to improve the accuracy of the aerosol extinction coefficient inversion, an inversion method based on an improved genetic algorithm is proposed. Using the U.S. Standard Atmosphere model and the return power equation, the aerosol extinction coefficient and the backscattering coefficient are independent variables that randomly provide initial values to simulate the theoretical lidar power. Then, the genetic algorithm is used to approximate the theoretical lidar power to the measured lidar return power with height; when the two are infinitely close, the values of the corresponding two independent variables (i.e., the extinction and backscattering coefficients) are inverted. Experiments performed to compare the different effects between a simple genetic algorithm and the improved genetic algorithm showed the proposed method capable of inverting the aerosol extinction coefficient without reliance on traditional inversion methods, representing a novel approach to the inversion of the aerosol extinction coefficient and the backscattering coefficient.