Aerosol Direct Effect Research Articles

Elevation-dependence of warming due to aerosol-induced snow darkening over the Himalayan-Tibetan region

Temperature trends over the high-altitude mountains depict an increase with elevation during recent years. These stratified warming trends observed over the Himalayan-Tibetan (HT) regions are higher than the mean warming trends observed over low-elevation regions of South and East Asia, which is attributed to several factors including snow albedo feedback, clouds and water vapor feedback. In this study, we demonstrate the effects of deposition of absorbing aerosols like black carbon and dust on snow albedo and its implications for elevation-dependent warming (EDW). Though the aerosol concentration decreases with elevation, warming due to aerosol-induced snow darkening increases with elevation. Further, surface cooling due to the direct radiative effects (DRE) of aerosols is found to decrease with elevation, which also favors higher warming at high altitudes. The effects of both the deposition of absorbing aerosols on snow albedo and the surface cooling due to the DRE of atmospheric aerosols could strengthen EDW. This study clearly shows the potential of albedo feedback due to aerosol-cryosphere interaction as one of the physical mechanisms contributing to the observed EDW over the HT region.

Impacts of vertical distribution of Southeast Asian biomass burning emissions on aerosol distributions and direct radiative effects over East Asia

The impacts of vertical distribution of biomass burning (BB) emissions on aerosol distributions and direct radiative effects over the BB source regions of Mainland Southeast Asia (MSEA) and downwind East Asian regions during spring (March to May) 2019 were investigated by applying an online coupled regional chemistry-aerosol-climate model (RIEMS-Chem). Model validation against a variety of observations demonstrated a generally good skill of the model in simulating aerosol chemical components, aerosol optical depth (AOD), and vertical distribution of aerosol extinction coefficient (EXT) when BB emissions were included. Four methods were adopted to represent injection height of BB emissions, including (1) a physical process-based parameterization (BB_param), (2) satellite-based prescribed profiles (BB_prof), (3) temporal-spatial varied injection profiles from the GFAS (Global Fire Assimilation System) dataset (BB_GFAS), and (4) BB emissions released at a fixed altitude (BB_high). The BB_param experiment generally produced better statistics compared to observations. Different BB injection height treatments considerably affected concentrations and distributions of BB aerosols, aerosol optical properties, direct radiative effects of BB aerosols (DREBB), atmospheric heating rate, and cloud fractions. The simulated sub-regional (100–120°E and 19–26°N, including major BB source and downwind areas) and seasonal mean DREBB at the top of the atmosphere (TOA) were +1.7 W m−2, +1.3 W m−2, +1.2 W m−2, and +1.7 W m−2 in the BB_param, BB_prof, BB_GFAS, and BB_high experiments, respectively, while the corresponding mean DREBB at the surface were −30.3 W m−2, -19.1 W m−2, -19.0 W m−2, and -22.1 W m−2. It is noticed that the DREBB at TOA and at the surface in BB_GFAS were just 68% and 63% of the values in BB_param, and the different injection height treatment had larger influences on DREBB at the surface than at TOA. The BB aerosol-induced atmospheric heating rate was up to 0.8–1.2 K/day in BB_param, which was larger than those in other experiments. Low cloud was enhanced while middle and high clouds were reduced by BB aerosols over northern MSEA. The BB aerosol-induced changes in cloud fractions in the BB_param experiment (up to 0.15 for low cloud and −0.05 for middle and high cloud) were approximately twice those in the other experiments. This study demonstrates the importance and necessity of properly representing the injection height of BB emissions in model estimation of radiative and climatic effects of BB aerosols.

Effects of Spring Dust Aerosols on Direct Radiative Forcing in China from 2000 to 2020

In order to understand the mechanism of dust aerosol influence on regional climate change, it is crucial to quantify the radiative forcing effect of dust aerosols. However, studies on the direct radiative forcing of dust aerosols over long time series in China are still lacking. The direct radiative forcing effect of dust aerosols in China over the past 20 years was simulated and evaluated based on the WRF-Chem (Weather Research and Forecasting model coupled to Chemistry) model in conjunction with remote sensing satellites and ground-based observations. The results showed that dust aerosols exhibited an obvious inter-annual positive radiative forcing effect (about 0.38 W m−2) on net radiation at the top of the atmosphere, mainly in northwest China and the North China Plain, while at the atmosphere dust aerosols presented negative radiative forcing effects on shortwave radiation and positive effects on longwave radiation, with a value of 1.54 W m−2 of net radiative forcing, showing a warming effect. Dust aerosols have a net radiative forcing value of −1.16 W m−2 at the surface, indicating a cooling effect, with a positive forcing effect on longwave radiation and a negative forcing effect on shortwave radiation, both of which coincide with the geographical distribution of dust aerosol concentrations. In terms of inter-monthly variations, at both the atmosphere and top of the atmosphere, the dust aerosols net radiative forcing values showed an increasing trend, with March (−0.20 W m−2 and 0.68 W m−2) < April (0.48 W m−2 and 1.44 W m−2) < May (0.94 W m−2 and 2.42 W m−2). Meanwhile, at the surface, the dust aerosols net radiative forcing values displayed a decreasing trend, with March (−0.88 W m−2) > April (−0.96 W m−2) > May (−1.48 W m−2).

Aerosol Optical Properties of Extreme Global Wildfires and Estimated Radiative Forcing With GCOM‐C SGLI

AbstractTo understand the climate impact of the wildfires, it is essential to monitor the aerosol emissions from biomass burning and to estimate their optical properties and radiative forcing. This study analyzed wildfires in Brazil, Angola, Australia, California, Siberia, and South‐east Asia that occurred after 2018 using data obtained with the Second‐generation GLobal Imager (SGLI) onboard Global Change Observation Mission—Climate which is a polar‐orbit satellite launched by JAXA on 23 December 2017. We showed the SGLI‐based 4‐year variation of the aerosol optical properties, Aerosol Optical Thickness, Ångström Exponent (AE), and Single Scattering Albedo (SSA) for each region complemented with other satellite‐ and ground‐based data. From the SSA and AE relationship analyses, we confirmed that their optical properties depend on the relative humidity and type of burned vegetation, which is consistent with the previous studies. Moreover, we estimated the net incoming radiation at the top of the atmosphere during the intense fire periods to understand the impact of the direct effect of biomass burning aerosols on radiative forcing. The estimates show a significant negative radiative forcing (i.e., a cooling effect) over the ocean (−78 and −96 Wm−2in Australia and California, respectively). In contrast, small values are observed over land (∼−10 Wm−2for all six regions). Therefore, taking the regional characteristics of the optical properties and surface reflectance into account is necessary to estimate the effect on radiative forcing and future impacts of a short‐lived climate forcer from wildfires.

The Dichotomy of Wet and Dry Trends Over India by Aerosol Indirect Effects in CMIP5 Models

AbstractAerosol‐cloud interactions, also known as aerosol indirect effect (AIE), substantially impact rainfall frequency and intensity. Here, we analyze NEX‐GDDP, a multimodel ensemble of high‐resolution (0.25°) historical simulations and future projections statistically downscaled from 21 CMIP5 models, to quantify the importance of AIE on extreme climate indices, specifically consecutive dry days (CDD), consecutive wet days (CWD), and simple daily intensity index (SDII). The 21 NEX‐GDDP CMIP5 models are classified into models with reliable (REM) and unreliable (UREM) monsoon climate simulated over India based on their simulations of the climate indices. The REM group is further decomposed based on whether the models represent only the direct (REMADE) or the direct and indirect (REMALL) aerosol effects. Compared to REMADE, including all aerosol effects significantly improves the model skills in simulating the observed historical trends of all three climate indices over India. Specifically, AIE enhances dry days and reduces wet days in India in the historical period, consistent with the observed changes. However, by the middle and end of the 21st century, there is a relative decrease in dry days and an increase in wet days and precipitation intensity. Moreover, the REMALL simulated future CWD and CDD changes are mostly opposite to those in REMADE, indicating the substantial role of AIE in the future projection of dry and wet climates. These findings underscore the crucial role of AIE in future projections of the Indian hydroclimate and motivate efforts to accurately represent AIE in climate models.

Impacts of aerosol direct effects on PM2.5 and O3 respond to the reductions of different primary emissions in Beijing-Tianjin-Hebei and surrounding area

In recent years, the rapid pollution emission reductions significantly decreased the PM2.5, which weakened the aerosol radiation feedback effect and in turn influenced the changes of PM2.5 and O3. To promote our understanding of this effect, we used an online-coupled meteorology-chemistry model (WRF-Chem) to investigate the influence of aerosol direct effects (ADE) on PM2.5 and O3 responding to different pollutant emissions reduction for a summer PM2.5-O3 compound pollution month in Beijing-Tian-Hebei region (BTH) and surrounding area. We performed scenario simulations with turning on/off both aerosol influences on the meteorology (ADE_MET) and photolysis (ADE_PHO), and turning on only ADE_PHO with different reduction ratios for primary PM2.5 (100%), SO2 (80%) and NOx (40%) emissions. Our results showed that total reduction of primary PM2.5, SO2 and NOx emissions led to overall declines of surface PM2.5 in BTH and surrounding area. The SO2 and NOx emission reductions both furtherly decreased PM2.5 via the changed ADE, while the primary PM2.5 emission reduction increased the PM2.5 by its induced ADE. Different from PM2.5, O3 significantly increased in BTH after cutting the three types of emissions. The primary PM2.5 emission reduction led to O3 increase over the whole region mostly by the induced ADE, while the NOx emission reduction directly enhanced O3 in the plain areas mainly due to incompatible reduction of NOx and VOCs emissions. The O3 enhanced by emission-reduction-induced ADE accounted for 56.1% of the total increase. The ADE_PHO caused by PM2.5 primary emissions reduction was the dominant contribution to the total ADE induced increases of PM2.5 and O3, which enhanced the photolysis of gases and led to overall increase of oxidants that strengthened secondary aerosol formation, and also promoted the production of O3 via photochemical processes. The results implicate that with the continuously strengthened abatement of PM2.5 primary emissions, it may offset part of the reduction effect on PM2.5 decrease by the changed ADE, and also increase O3 over the whole region. The results also suggested that while controlling both PM2.5 and O3 in BTH in summer, not only the cooperative emission reduction of NOx and VOCs is essential, the induced ADE effect by PM2.5 primary emissions reduction should also be considered.

Effects of anthropogenic aerosols on the evolution of Indian summer monsoon

The NCAR Community Earth System Model is used to study the influences of anthropogenic aerosols on the Indian summer monsoon (ISM). We perform two sets of 30-year simulations subject to the prescribed perpetual SST annual cycle. One is triggered by the year 2000 climatology anthropogenic aerosol emissions data over the Indian Peninsula (referred to as AERO), and the other one is by the year 1850 (referred to as CTL). Only aerosol direct effects are included in the experiments. In our results, the transition of ISM in AERO relative to the CTL exhibits a similar ensemble-mean onset date with a larger spread, and more abrupt onset in late spring, and an earlier but more gradual withdrawal in early fall. The aerosols-induced circulation changes feature an upward motion over the northeastern Indian Peninsula and strengthened anticyclonic circulation over the Arabia Sea in the pre-monsoon season, and a northward shift of monsoon flow in the developed monsoon period along with strengthened local meridional circulation over northern India. The strengthened anticyclonic circulation over Arabia Sea caused a 16% increase in natural dust transport from the Middle East in the pre-monsoon season. The elevated aerosol heating over Tibet causes stronger ascending motion in the pre-monsoon period that leads to earlier and more abrupt ISM onset. The earlier monsoon withdrawal is attributed to the aerosol-induced anticyclonic flow within 10°–25°N and cyclonic flow within 0°–10°N over eastern India and Bay of Bengal that resemble the ISM seasonal transition in September.

Direct Radiative Effects of Aerosols on Numerical Weather Forecasts—A Comparison of Two Aerosol Datasets in the NCEP GFS

Abstract This study compares aerosol direct radiative effects on numerical weather forecasts made by the NCEP Global Forecast System (GFS) with two different aerosol datasets, the Optical Properties of Aerosols and Clouds (OPAC) and MERRA-2 aerosol climatologies. The underestimation of aerosol optical depth (AOD) by OPAC over northwest Africa, central to East Africa, the Arabian Peninsula, Southeast Asia, and the Indo-Gangetic Plain, and overestimation in the storm-track regions in both hemispheres are reduced by MERRA-2. Surface downward shortwave (SW) and longwave (LW) fluxes and the top-of-the-atmosphere SW and outgoing LW fluxes from model forecasts are compared with CERES satellite observations. Forecasts made with OPAC aerosols have large radiative flux biases, especially in northwest Africa and the storm-track regions. These biases are also reduced in the forecasts made with MERRA-2 aerosols. The improvements from MERRA-2 are most noticeable in the surface downward SW fluxes. GFS medium-range weather forecasts made with the MERRA-2 aerosols demonstrated slightly improved forecast accuracy of sea level pressure and precipitation over the Indian and East Asian summer monsoon region. A stronger Africa easterly jet is produced, associated with a low pressure over the east Atlantic Ocean and west of northwest Africa. Impacts on large-scale skill scores such as 500-hPa geopotential height anomaly correlation are generally positive in the Northern Hemisphere and the Pacific and North American regions in both the winter and summer seasons.

Emissions Background, Climate, and Season Determine the Impacts of Past and Future Pandemic Lockdowns on Atmospheric Composition and Climate

AbstractCOVID‐19 pandemic responses affected atmospheric composition and climate. These effects depend on the background emissions, climate, and season in which they occur. Although using multiple scenarios is common in explorations of long‐term climate change, they are rarely used to explore atmospheric composition or climate changes in response to transient emission perturbations on the scale of COVID‐19 lockdowns. We used the ModelE Earth system model to evaluate how atmospheric and climate impacts depend on the decade and season in which lockdowns occurred. Global COVID‐19‐related anomalies in aerosols and trace gases differed by up to an order of magnitude or more when comparing lockdowns in 1980, 2008, 2020, and 2051. Regional atmospheric composition anomalies tended to be largest when emissions were near a historical peak: 1980 in Europe and temperate North America, 2008 or 2020 in eastern Asia, and 2051 in south Asia. Regional aerosol direct effect anomalies were almost always less than 0.1 W m−2 during the first pandemic year, but over 0.1 W m−2 in Europe and exceeded 0.2 W m−2 in Europe and temperate North America in 1980, generally changing in tandem with regional emissions. In contrast, direct effect anomalies in Asia were positive in 1980 and negative in 2008, suggesting they may be primarily determined by exogenous emission anomalies. Shifting COVID‐19 onset in 2020 by 3, 6, or 9 months also altered atmospheric composition on the order of 2%–25% globally. In all scenarios, changes in surface temperature or precipitation appeared unrelated to local atmospheric compositional changes.

Mechanisms of hydrological responses to volcanic eruptions in the Asian monsoon and westerlies-dominated subregions

Abstract. Explosive volcanic eruptions affect surface climate, especially in monsoon regions, but responses vary in different regions and to volcanic aerosol injection (VAI) in different hemispheres. Here, we use six ensemble members from the last-millennium experiment of the Coupled Model Intercomparison Project Phase 5 to investigate the mechanisms of regional hydrological responses to different hemispheric VAIs in the Asian monsoon region (AMR). Northern hemispheric VAI (NHVAI) leads to an intensified aridity over the AMR after northern hemispheric VAI (NHVAI); spatially, a distinct inverse response pattern to the climatological conditions emerges, with an intensified aridity in the relatively wettest area (RWA) but a weakened aridity in the relatively driest area (RDA) of the AMR. Southern hemispheric VAI (SHVAI) shows a weakened aridity over the AMR, but the spatial response pattern is not that clear due to small aerosol magnitude. The mechanism of the hydrological impact relates to the indirect change of atmospheric circulation due to the direct radiative effect of volcanic aerosols. The decreased thermal contrast between the land and the ocean after NHVAI results in a weakened East Asian summer monsoon and South Asian summer monsoon. This changes the moisture transport and cloud formation in the monsoon and westerlies-dominated subregions. The subsequent radiative effect and physical feedbacks of local clouds lead to different hydrological effects in different areas. Results here indicate that future volcanic eruptions may temporarily alleviate the uneven distribution of precipitation in the AMR, which should be considered in the near-term climate predictions and future strategies of local adaptation to global warming. The local hydrological responses and mechanisms found here can also provide a reference for stratospheric aerosol engineering.

Observations on the decadal variability of aerosol in eastern Himalayan foothills: Evidence of an anthropologically induced positive shift

The decadal variability of direct radiative effects of aerosols is investigated at Dibrugarh, a site in northeast India (NEI) at the eastern Himalayan foothills, primarily using multi-wavelength solar radiometer measurements spanning from October 2001 to February 2020. The ground-based aerosol observations are combined with satellite remote sensing, reanalysis data, and model simulations to study the change in atmospheric particle loading over the region. Observations indicate a statistically significant increase (∼0.015 yr−1) in Aerosol Optical Depth (AOD) during the last two decades in line with an increase in human activity. As compared to 2001–2007 (we call it as Stage I), the aerosol burden has grown rapidly during 2008 until 2020 (Stage II). AOD at 500 nm is found to increase by ∼40% from Stage I to Stage II, resulting in an increase in the aerosol direct radiative forcing (DRF) at the top of the atmosphere (TOA) by ∼43% during stage II (∼−16.0 W m-2), from the base value of −11.2 W m−2 in Stage I. Decreasing biomass burning activities, black carbon aerosol mass concentration, and high sulfate and organic aerosols are the primary factors responsible for the trend in TOA cooling by −0.46 W m−2 yr−1. This is further aided by the decrease in rainfall over NEI. MERRA-2 data analysis shows a similar enhancements in aerosol load over the entire NEI and the adjacent highly polluted Indo-Gangetic Plains (IGP). A similar feature is seen over the IGP, primarily driven by anthropogenic emissions, but precedes that in NEI by about a year. A simulation of the regional climate model (RegCM) over the south Asian domain quantifies the contribution of aerosol loading over NEI due to the aerosols carried from the IGP. In the highest aerosol loading period, about 12–30% of the aerosols, equivalent to 15–30% of atmospheric warming, are transported from the IGP to the NEI.

Aerosol radiative feedback enhances particulate pollution over India: A process understanding

In this study, we investigate the role of aerosol direct radiative feedback on regional meteorological changes and subsequent distribution of air pollutant with the focus on particulate matter PM2.5 and ozone (O3) over India. WRF-Chem simulations have been applied for Baseline case with both aerosol direct and indirect effects and another simulation including only aerosol indirect effects. The aerosol direct radiative feedback on the meteorology and air quality were investigated by taking the differences between these two simulations. A comprehensive model evaluation showed the model had the capacity to reproduce the observations and well captured the temporal and spatial variation in meteorological and aerosol fields. We found that the reduction in incoming shortwave solar radiation, temperature at 2 m and planetary boundary layer height annually and across all the season due to aerosol radiation interaction (ARI). The concentration of PM2.5 and gaseous precursors like SO2 and NO2 showed enhancements, while O3 concentration mostly showed a reduction. Spatial and annual average PM2.5 concentration was increased by +6%, SO2 concentration was increased by +1.4%, NO2 concentration was increased by +3.4%, and O3 concentration was reduced by −1.4%. Largest regional increases of 40% in particulate pollution induced by ARI occurred over north-western Indian region. The increase in PM2.5 concentration was highly related to stabilisation induced through meteorological variables and increases in primary aerosol concentration. The decrease in O3 concentration was highly related increases in NO2 and SO2 concentration. In the most polluted regions of India, ARI significantly enhance surface-level particulate pollution and related premature mortality, of particular concern considering likely future increasing trends. This study highlights the importance of inclusion and better representations of ARI and for implementing effective mitigation plans.

Investigation of aerosol direct radiative forcing during a dust storm using a regional climate model over Turkiye

Dust particles originating from arid zones can be transported long distances and change the radiation budget. Understanding atmospheric aerosols and their radiative forcing is important to determine their global and regional climate effects. The aim of this study is to simulate the dust transport event that occurred on March 22, 2018, using RegCM-4.5 and investigate the radiative forcing effect of Saharan dust particles. The model was run with the 4 dust bin chemistry option and the direct effect of aerosols on the regional radiation balance was investigated. Validation of the model was made by a comparison between simulated aerosol optical depth (AOD) and MODIS satellite data. The radiative forcing at the top and surface was calculated at all sky conditions. During the dust episode, the shortwave radiative forcing was ranging between -3 and -50 W/m2 at surface and -2 and -22 W/m2 at top of atmosphere while the longwave radiative forcing was between 0.5 and 8 W/m2 at surface and 0.2 and 2 W/m2 at top of atmosphere over Turkiye. In Istanbul it produced a cooling up to -18 W/m2 at surface and -9 W/m2 at top of atmosphere, a warming up to 3.5 W/m2 at surface and 0.6 W/m2 at top of atmosphere.

Enviro-HIRLAM model estimates of elevated black carbon pollution over Ukraine resulted from forest fires

Abstract. Biomass burning is one of the biggest sources of atmospheric black carbon (BC), which negatively impacts human health and contributes to climate forcing. In this work, we explore the horizontal and vertical variability of BC concentrations over Ukraine during wildfires in August 2010. Using the Enviro-HIRLAM modelling framework, the BC atmospheric transport was modelled for coarse, accumulation, and Aitken mode aerosol particles emitted by the wildfire. Elevated pollution levels were observed within the boundary layer. The influence of the BC emissions from the wildfire was identified up to 550 hPa level for the coarse and accumulation modes and at distances of about 2000 km from the fire areas. BC was mainly transported in the lowest 3 km layer and mainly deposited at night and in the morning hours due to the formation of strong surface temperature inversions. As modelling is the only available source of BC data in Ukraine, our results were compared with ground-level measurements of dust, which showed an increase in concentration of up to 73 % during wildfires in comparison to average values. The BC contribution was found to be 10 %–20 % of the total aerosol mass near the wildfires in the lowest 2 km layer. At a distance, BC contribution exceeded 10 % only in urban areas. In the areas with a high BC content represented by both accumulation and coarse modes, downwelling surface long-wave radiation increased up to 20 W m−2, and 2 m air temperature increased by 1–4 ∘C during the midday hours. The findings of this case study can help to understand the behaviour of BC distribution and possible direct aerosol effects during anticyclonic conditions, which are often observed in mid-latitudes in the summer and lead to wildfire occurrences.

Interaction between different mixing aerosol direct effects and East Asian summer monsoon

Aerosol mixtures, which are still unclear in current knowledge, may cause large uncertainties in aerosol climate effect assessments. To better understand this research gap, a well-developed online coupled regional climate-chemistry model is employed here to investigate the influences of different aerosol mixing states on the direct interactions between aerosols and the East Asian summer monsoon (EASM). The results show that anthropogenic aerosols have high-level loadings with heterogeneous spatial distributions in East Asia. Black carbon aerosol loading accounts for more than 13% of the totals in this region in summer. Thus, different aerosol mixing states cause very different aerosol single scattering albedos, with a variation of 0.27 in East Asia in summer. Consequently, the sign of the aerosol instantaneous direct radiative forcing at the top of the atmosphere is changed, varying from − 0.95 to + 1.50 W/m2 with increasing internal mixing aerosols. The influence of aerosol mixtures on regional climate responses seems to be weaker. The EASM circulation can be enhanced due to the warming effect of anthropogenic aerosols in the lower atmosphere, which further induces considerable aerosol accumulation associated with dynamic field anomaly, decrease in rainfall and so on, despite aerosol mixtures. However, this interaction between aerosols and the EASM will become more obvious if the aerosols are more mixed internally. Additionally, the differences in aerosol-induced EASM anomalies during the strongest and weakest monsoon index years are highly determined by the aerosol mixing states. The results here may further help us better address the environmental and climate change issues in East Asia.

Radiative effects and feedbacks of anthropogenic aerosols on boundary layer meteorology and fine particulate matter during the COVID-19 lockdown over China

The COVID-19 epidemic has exerted significant impacts on human health, social and economic activities, air quality and atmospheric chemistry, and potentially on climate change. In this study, an online coupled regional climate–chemistry–aerosol model (RIEMS-Chem) was applied to explore the direct, indirect, and feedback effects of anthropogenic aerosols on radiation, boundary layer meteorology, and fine particulate matter during the COVID-19 lockdown period from 23 January to 8 April 2020 over China. Model performance was validated against a variety of observations for meteorological variables, PM2.5 and its chemical components, aerosol optical properties, as well as shortwave radiation flux, which demonstrated that RIEMS-Chem was able to reproduce the spatial distribution and temporal variation of the above variables reasonably well. During the study period, direct radiative effect (DRE) of anthropogenic aerosols was stronger than indirect radiative effect (IRE) in most regions north of the Yangtze River, whereas IRE dominated over DRE in the Yangtze River regions and South China. In North China, DRE induced larger changes in meteorology and PM2.5 than those induced by IRE, whereas in South China, the changes by IRE were remarkably larger than those by DRE. Emission reduction alone during the COVID-19 lockdown reduced PM2.5 concentration by approximately 32 % on average over East China. As a result, DRE at the surface was weakened by 15 %, whereas IRE changed little over East China, leading to a decrease in total radiative effect (TRE) by approximately 7 % in terms of domain average. The DRE-induced changes in meteorology and PM2.5 were weakened due to emission reduction, whereas the IRE-induced changes were almost the same between the cases with and without emission reductions. By aerosol radiative and feedback effects, the COVID-19 emission reductions resulted in 0.06 °C and 0.04 °C surface warming, 1.6 and 4.0 μg m−3 PM2.5 decrease, 0.4 and 1.3 mm precipitation increase during the lockdown period in 2020 in terms of domain average over North China and South China, respectively, whereas the lockdown caused negligible changes on average over East Asia.

Water Solubility Distribution of Organic Matter Accounts for the Discrepancy in Hygroscopicity among Sub- and Supersaturated Humidity Regimes.

Water uptake properties of organic matter (OM) are critical for aerosol direct and indirect effects. OM contains various chemical species that have a wide range of water solubility. However, the role of water solubility on water uptake by OM has poorly been investigated. We experimentally retrieved water solubility distributions of water-soluble OM (WSOM) from combustion of mosquito coil and tropical peat using the 1-octanol-water partitioning method. In addition, hygroscopic growth and cloud condensation nuclei (CCN) activity of solubility-segregated WSOM were measured. The dominant fraction of WSOM from mosquito coil smoldering was highly soluble (water solubility (S) > 10-2 g cm-3), while that from peat combustion contained ∼40% of less-soluble species (S < 10-3 g cm-3). The difference in water solubility distributions induced changes in the roles of less water-soluble fractions (S < 10-3 g cm-3) on CCN activity. Namely, the less water-soluble fraction from mosquito coil combustion fully dissolved at the point of critical supersaturation, while that for tropical peat smoldering was limited by water solubility. The present result suggests that water solubility distributions of OM, rather than its bulk chemical property, need to be quantified for understanding the water uptake process.

The dominant role of aerosol-cloud interactions in aerosol-boundary layer feedback: Case studies in three megacities in China

Interactions between aerosols and meteorology have received increasing attention in recent decades. Through interactions with radiation, aerosols involve in thermodynamic processes and cause cloud adjustment, referred to as the direct and semi-direct effects respectively. They also involve in cloud microphysical processes by severing as cloud condensation nuclei or ice nuclei, referred to as indirect effect. Aerosol direct effect is found to potentially exacerbate air quality by stabilizing the planetary boundary layer (PBL). However, their impacts through the interaction with clouds, including semi-direct and indirect effect remain unclear. In this study, we conducted model simulations to evaluate the direct, semi-direct and indirect effects of aerosols in PBL structure and surface PM2.5 concentration during three heavy haze events under overcast conditions. Overall, the aerosol-PBL feedback results in a 22%–36% decrease of PBL height and 5%–28% increase of PM2.5 concentration. The indirect effect always has the largest impact on PBL and PM2.5 pollution, accounting for 59%–84% of the changes. The semi-direct effect is the weakest on average, although it can exceed the direct effect at certain times and locations. Black carbon aerosols play the vital role in both the direct and semi-direct effects. Our findings promote the understanding of heavy haze formation, and highlight the dominant role of aerosol-cloud interaction in the feedback process of aerosols to PBL structure and air quality.

Direct Radiative Effects of Dust Aerosols over Northwest China Revealed by Satellite-Derived Aerosol Three-Dimensional Distribution

Direct Radiative Effects of Dust Aerosols over Northwest China Revealed by Satellite-Derived Aerosol Three-Dimensional Distribution

Fire–climate interactions through the aerosol radiative effect in a global chemistry–climate–vegetation model

Abstract. Fire emissions influence radiation, climate, and ecosystems through aerosol radiative effects. These can drive rapid atmospheric and land surface adjustments which feed back to affect fire emissions. However, the magnitude of such feedback remains unclear on the global scale. Here, we quantify the impacts of fire aerosols on radiative forcing and the fast atmospheric response through direct, indirect, and albedo effects based on the two-way simulations using a well-established chemistry–climate–vegetation model. Globally, fire emissions cause a reduction of 0.565 ± 0.166 W m−2 in net radiation at the top of the atmosphere with dominant contributions by the aerosol indirect effect (AIE). Consequently, terrestrial surface air temperature decreases by 0.061 ± 0.165 ∘C with coolings of &gt;0.25 ∘C over the eastern Amazon, the western US, and boreal Asia. Both the aerosol direct effect (ADE) and AIE contribute to such cooling, while the aerosol albedo effect (AAE) exerts an offset warming, especially at high latitudes. Land precipitation decreases by 0.180 ± 0.966 mm per month (1.78 % ± 9.56 %) mainly due to the inhibition in central Africa by AIE. Such a rainfall deficit further reduces regional leaf area index (LAI) and lightning ignitions, leading to changes in fire emissions. Globally, fire emissions reduce by 2 %–3 % because of the fire-induced fast responses in humidity, lightning, and LAI. The fire aerosol radiative effects may cause larger perturbations to climate systems with likely more fires under global warming.