The accurate assessment of aerodynamic damping is essential when estimating the impact of aero-elastic effects on crosswind-excited line-like structures. This study aims to determine the crosswind aerodynamic damping of a circular cylinder by curve-fitting to the response probability density function. The generalized Van der Pol oscillator model is employed to depict the nonlinearity associated with amplitude-dependent aerodynamic damping. The initial section of this study presents the theoretical foundation of the identified approach used in this research. Subsequently, the efficacy of the identification methodology is validated by means of a stochastic simulation of the crosswind response of a circular cylinder. Moreover, identification of nonlinear aerodynamic damping is further accomplished by the utilization of an aero-elastic model wind tunnel test. The identified nonlinear aerodynamic damping is then utilized to determine the response statistical quantities for a total of 16 chimneys. The determined aerodynamic damping provides a satisfactory assessment of the peak response, which is crucial for design considerations.