Adiabatic Passage Research Articles

Spatial adiabatic passage of ultracold atoms in optical tweezers.

Coherent manipulation of matter waves, a distinctive hallmark of quantum mechanics, is fundamental to modern quantum technologies. Spatial adiabatic passage (SAP) is a prime example of this phenomenon, where a wave packet is transferred between two uncoupled localized modes by adjusting the tunneling coupling to an intermediate third mode in a counterintuitive sequence. Although this concept was introduced over two decades ago, its observation was previously limited to electromagnetic waves. In this study, we demonstrate this quantum interference effect using massive particles that tunnel between three micro-optical traps ("optical tweezers"). We begin by preparing ultracold fermionic atoms in low vibrational eigenstates of one trap, followed by manipulating the distance between the traps to execute the SAP protocol. We observe a smooth and high-efficiency transfer of atoms between the two outer traps, with a very low population remaining in the central trap. These findings open possibilities for advanced control schemes in optical tweezer array platforms.

Non-Abelian braiding in three-fold degenerate subspace and the acceleration

Non-Abelian braiding operations of quantum states have attracted substantial attention due to their great potentials for realizing topological quantum computations. The adiabatic version of quantum braiding is robust against systematic errors, yet will suffer from decoherence and dephasing effects due to a long evolution time. In this paper, we propose to realize the braiding process in a three-fold degenerate subspace of a seven-level system, where the non-Abelian effect can be detected by changing the orders of the braiding. We accelerate the adiabatic control through adding auxiliary coupling terms according to a shortcut to adiabatic theory for the non-Abelian case. Furthermore, by generalizing the parallel adiabatic passages, adiabatic control can be accelerated through only reshaping the original control waveforms and the effective pulses area will be significantly reduced. Therefore, the proposed schemes may provide an experimentally feasible way to investigate the non-Abelian braiding in atomic systems and the waveguide systems.

Restoring Adiabatic State Transfer in Time-Modulated Non-Hermitian Systems.

Non-Hermitian systems have attracted much interest in recent decades, driven partly by the existence of exotic spectral singularities, known as exceptional points (EPs), where the dimensionality of the system evolution operator is reduced. Among various intriguing applications, the discovery of EPs has suggested the potential for implementing a symmetric mode switch, when encircling them in a system parameter space. However, subsequent theoretical and experimental works have revealed that dynamical encirclement of EPs invariably results in asymmetric mode conversion; namely, the mode switching depends only on the winding direction but not on the initial state. This chirality arises from the failure of adiabaticity due to the complex spectrum of non-Hermitian systems. Although the chirality revealed has undoubtedly made a significant impact in the field, a realization of the originally sought symmetric adiabatic passage in non-Hermitian systems with EPs has since been elusive. In this work, we bridge this gap and theoretically demonstrate that adiabaticity, and therefore a symmetric state transfer, is achievable when dynamically winding around an EP. This becomes feasible by specifically choosing a trajectory in the system parameter space along which the corresponding evolution operator attains a real spectrum. Our findings, thus, offer a promise for advancing various wave manipulation protocols in both quantum and classical domains.

Quantum Interference and Coherent Population Trapping in a Double Quantum Dot.

Quantum interference is a natural consequence of wave-particle duality in quantum mechanics, and is widely observed at the atomic scale. One interesting manifestation of quantum interference is coherent population trapping (CPT), first proposed in three-level driven atomic systems and observed in quantum optical experiments. Here, we demonstrate CPT in a gate-defined semiconductor double quantum dot (DQD), with some unique twists as compared to the atomic systems. Specifically, we observe CPT in both driven and nondriven situations. We further show that CPT in a driven DQD could be used to generate adiabatic state transfer. Moreover, our experiment reveals a nontrivial modulation to the CPT caused by the longitudinal driving field, yielding an odd-even effect and a tunable CPT. Our results broaden the field of CPT, and open up the possibility of quantum simulation and quantum computation based on adiabatic passage in quantum dot systems.

Fast preparation of Dicke state by shortcuts to adiabatic passages

Dicke state is one of the most useful multipartite quantum states. In this paper, by utilizing the method of designing the evolution operators to construct shortcuts to adiabatic passages (STAP), we have implemented the fast preparation of Dicke states |D3(2)〉 and |D4(2)〉 with one step. Specifically, with the assistance of quantum Zeno dynamics, the original Hamiltonian of the system is simplified into an effective Hamiltonian. Under the dynamic evolution of this effective Hamiltonian, the pulse control is realized by selecting two appropriate auxiliary parameters. This not only greatly shortens the evolution time but also optimizes the operation of the quantum system. In addition, we have discussed the effects of decoherence, parameter fluctuations and noise on fidelity. The results indicate that the proposed protocol maintains high fidelity. Finally, the fast preparation of Dicke state |Dn(2)〉 can be achieved based on the same method.

Generalized cluster correlation expansion theory for stimulated Raman adiabatic passage processes in the presence of a spin bath

Generalized cluster correlation expansion theory for stimulated Raman adiabatic passage processes in the presence of a spin bath

A state-selected continuous wave laser excitation method for determining CO2's rotational state distribution in a supersonic molecular beam.

State-resolved experiments can provide fundamental insight into the mechanisms behind chemical reactions. Here, we describe our methods for characterizing state-resolved experiments probing the outcome of the collision between CO2 molecules and surfaces. We create a molecular beam from a supersonic expansion that passes through an ultra-high vacuum system. The CO2 is vibrationally excited by a continuous wave infrared (IR) laser using rapid adiabatic passage. We attenuate the fractional excitation using a CO2 absorption cell in the IR beam path. We combine Monte Carlo simulations and molecular beam energy measurements to find the initial rotational state distribution of the molecular beam. We find that our pure CO2 beam from a 300K source has a rotational temperature of ∼26K.

Robust cascaded frequency conversion through shortcuts to adiabaticity

We propose a cascaded frequency conversion technique based on Stark-chirped rapid shortcuts to adiabatic passage (SCRSAP). The implementation of this technique corrects the coupling function in Stark-chirped rapid adiabatic passage (SCRAP) technique by means of shortcuts to adiabaticity (STA) counter-diabatic (CD) driving. The results of numerical simulations show that SCRSAP technique allows efficient frequency conversion at lower pump laser intensity and a wider range of delay parameters than SCRAP technique, and the STA technique improves the robustness of the process to temperature and signal frequency variations in adiabatic frequency conversion.

Dicke State Generation and Extreme Spin Squeezing via Rapid Adiabatic Passage.

Considering the unique energy level structure of the one-axis twisting Hamiltonian in combination with standard rotations, we propose the implementation of a rapid adiabatic passage scheme on the Dicke state basis. The method permits to drive Dicke states of the many-atom system into entangled states with maximum quantum Fisher information. The designed states allow us to overcome the classical limit of phase sensitivity in quantum metrology and sensing. We show how to generate superpositions of Dicke states, which maximize metrological gain for a Ramsey interferometric measurement. The proposed scheme is remarkably robust to variations of the driving field and has favorable time scaling, especially for a small to moderate (∼1000) number of atoms, where the total time does not depend on the number of atoms.

Adiabatically Manipulated Systems Interacting with Spin Baths beyond the Rotating Wave Approximation

The Stimulated Raman Adiabatic Passage (STIRAP) on a three-state system interacting with a spin bath is considered, focusing on the efficiency of the population transfer. Our analysis is based on the perturbation treatment of the interaction term evaluated beyond the Rotating Wave Approximation, thus focusing on the limit of weak system–bath coupling. The analytical expression of the correction to the efficiency and the consequent numerical analysis show that, in most of the cases, the effects of the environment are negligible, confirming the robustness of the population transfer.

Reciprocity relations in a biologically inspired nanomagnonic system with dipolar coupling

Magnetosome chains in magnetotactic bacteria present ideal nanomagnonic model systems for studying collective resonance modes of dipolar-coupled single domain particles in relation to their spatial arrangement. Using microresonator-based ferromagnetic resonance (FMR) spectroscopy, electron microscopy, and micromagnetic modeling, we here provide insights into the complex magnonic activity within a single magnetosome chain. While the angular dependence of its FMR spectrum is dominated by twofold symmetry features due to the uniaxial anisotropy of linear chain segments, we also observed an unexpected behavior such as interrupted lines and flat bands due to the intricate geometrical details of this particular chain, such as a cross-like structural anomaly where a pair of particles is oriented perpendicular to the main axis of the chain and thus breaks the prevailing axial dipolar coupling symmetry. Such a cross junction formed by four particles exhibits interesting magnonic network properties. Notably, we observe reciprocity in the sense that the spectral response of one particle to an excitation of another one is identical to the response of the latter given an excitation of the former. Furthermore, we have identified that magnonic coupling between A and B can be facilitated via a dark state, as in magnonic stimulated Raman adiabatic passage, and that this dark-state coupling can be made non-reciprocal between A and B by breaking the symmetry of the spatial arrangement of the four particles.

Robust parallel laser driving of quantum dots for multiplexing of quantum light sources

Deterministic sources of quantum light (i.e. single photons or pairs of entangled photons) are required for a whole host of applications in quantum technology, including quantum imaging, quantum cryptography and the long-distance transfer of quantum information in future quantum networks. Semiconductor quantum dots are ideal candidates for solid-state quantum emitters as these artificial atoms have large dipole moments and a quantum confined energy level structure, enabling the realization of single photon sources with high repetition rates and high single photon purity. Quantum dots may also be triggered using a laser pulse for on-demand operation. The naturally-occurring size variations in ensembles of quantum dots offers the potential to increase the bandwidth of quantum communication systems through wavelength-division multiplexing, but conventional laser triggering schemes based on Rabi rotations are ineffective when applied to inequivalent emitters. Here we report the demonstration of the simultaneous triggering of >10 quantum dots using adiabatic rapid passage. We show that high-fidelity quantum state inversion is possible in a system of quantum dots with a 15 meV range of optical transition energies using a single broadband, chirped laser pulse, laying the foundation for high-bandwidth, multiplexed quantum networks.

Microcanonical treatment of HCl dissociative chemisorption on Au(111): Reactive dampening through inefficient translational energy coupling and an active surface.

Microcanonical unimolecular rate theory is applied to Shirhatti and Wodtke's recent supersonic molecular beam experiments examining the activated dissociative chemisorption of HCl on Au(111). A precursor mediated microcanonical trapping (PMMT) model (where the surface vibrates and HCl rotations, vibration, and translation directed along the surface normal are treated as active degrees of freedom) gave dissociative sticking coefficient predictions that are several orders of magnitude higher than experimental values but in good accord with prior quantum and molecular dynamics simulations. Density functional theory (DFT) electronic structure calculations using the Perdew-Burke-Ernzerhof (PBE) functional served to fix the vibrational frequencies of the reactive transition state and the threshold energy for dissociation, E0 = 72.9 kJ/mol. To explore the possibilities of varying threshold energy, coupling to phonons, and dynamics, a three-parameter [E0, s, ɛn] dynamically biased (d-) PMMT model was fit to the experiments. A dynamical bias was introduced using an efficiency, ɛn, of normal translational energy to contribute to the active exchangeable energy capable of promoting reactivity. To achieve the low sticking probabilities observed in experiment, severe normal translational energy dampening (ɛn → 0.26) was imposed, leading to a large vibrational efficacy of ηv = εv/εn = 3.85. The optimal threshold energy for dissociation was E0 = 30.88 kJ/mol, some 40 kJ/mol below the PBE-DFT prediction, and the optimal number of Au surface oscillators was s = 1. The d-PMMT modeling indicates that HCl/Au(111) reactivity can be consistent with electronically adiabatic passage across a relatively low and late transition state that dynamically disfavors normal translational energy.

Robust temporal adiabatic passage with perfect frequency conversion between detuned acoustic cavities

For classical waves, phase matching is vital for enabling efficient energy transfer in many scenarios, such as waveguide coupling and nonlinear optical frequency conversion. Here, we propose a temporal quasi-phase matching method and realize robust and complete acoustical energy transfer between arbitrarily detuned cavities. In a set of three cavities, A, B, and C, the time-varying coupling is established between adjacent elements. Analogy to the concept of stimulated Raman adiabatic passage, amplitudes of the two couplings are modulated as time-delayed Gaussian functions, and the couplings’ signs are periodically flipped to eliminate temporal phase mismatching. As a result, robust and complete acoustic energy transfer from A to C is achieved. The non-reciprocal frequency conversion properties of our design are demonstrated. Our research takes a pivotal step towards expanding wave steering through time-dependent modulations and is promising to extend the frequency conversion based on state evolution in various linear Hermitian systems to nonlinear and non-Hermitian regimes.

Accelerated Adiabatic Passage of a Single Electron Spin Qubit in Quantum Dots.

Adiabatic processes can keep the quantum system in its instantaneous eigenstate, which is robust to noises and dissipation. However, it is limited by sufficiently slow evolution. Here, we experimentally demonstrate the transitionless quantum driving (TLQD) of the shortcuts to adiabaticity in gate-defined semiconductor quantum dots (QDs) to greatly accelerate the conventional adiabatic passage for the first time. For a given efficiency of quantum state transfer, the acceleration can be more than twofold. The dynamic properties also prove that the TLQD can guarantee fast and high-fidelity quantum state transfer. In order to compensate for the diabatic errors caused by dephasing noises, the modified TLQD is proposed and demonstrated in experiment by enlarging the width of the counterdiabatic drivings. The benchmarking shows that the state transfer fidelity of 97.8% can be achieved. This work will greatly promote researches and applications about quantum simulations and adiabatic quantum computation based on the gate-defined QDs.

Chirped Pulses Meet Quantum Dots: Innovations, Challenges, and Future Perspectives

AbstractShaped laser pulses have been remarkably effective in investigating various aspects of light–matter interactions spanning a broad range of research. Chirped laser pulses exhibiting a time‐varying frequency, or quadratic spectral phase, form a crucial category in the group of shaped laser pulses. This type of pulses have made a ubiquitous presence from spectroscopic applications to developments in high‐power laser technology, and from nanophotonics to quantum optical communication, ever since their introduction. In the case of quantum technologies recently, substantial efforts are being invested toward achieving a truly scalable architecture. Concurrently, it is important to develop methods to produce robust photon sources. In this context, semiconductor quantum dots hold great potential, due to their exceptional photophysical properties and on‐demand operating nature. Concerning the scalability aspect of semiconductor quantum dots, it is advantageous to develop a simple, yet robust method to generate photon states from it. Chirped pulse excitation has been widely demonstrated as a robust and efficient state preparation scheme in quantum dots, thereby boosting its applicability as a stable photon source in a real‐world scenario. Despite the rapid growth and advancements in laser technologies, the generation and control of chirped laser pulses can be demanding. Here, an overview of a selected few approaches is presented to tailor and characterize chirped pulses for the efficient excitation of a quantum dot source. By taking the chirped‐pulse‐induced adiabatic rapid passage process in quantum dot as an example, numerical design examples are presented along with experimental advantages and challenges in each method and conclude with an outlook on future perspectives.

Highly efficient creation and detection of deeply bound molecules via invariant-based inverse engineering with feasible modified drivings.

Stimulated Raman Adiabatic Passage (STIRAP) and its variants, such as M-type chainwise-STIRAP, allow for efficiently transferring the populations in a multilevel system and have widely been used to prepare molecules in their rovibrational ground state. However, their transfer efficiencies are generally imperfect. The main obstacle is the presence of losses and the requirement to make the dynamics adiabatic. To this end, in the present paper, a new theoretical method is proposed for the efficient and robust creation and detection of deeply bound molecules in three-level Λ-type and five-level M-type systems via "Invariant-based shortcut-to-adiabaticity." In the regime of large detunings, we first reduce the dynamics of three- and five-level molecular systems to those of effective two- and three-level counterparts. By doing so, the major molecular losses from the excited states can be well suppressed. Consequently, the effective two-level counterpart can be directly compatible with two different "Invariant-based Inverse Engineering" protocols; the results show that both protocols give a comparable performance and have a good experimental feasibility. For the effective three-level counterpart, by considering a relation among the four incident pulses, we show that this model can be further generalized to an effective Λ-type one with the simplest resonant coupling. This generalized model permits us to borrow the "Invariant-based Inverse Engineering" protocol from a standard three-level Λ-type system to a five-level M-type system. Numerical calculations show that the weakly bound molecules can be efficiently transferred to their deeply bound states without strong laser pulses, and the stability against parameter variations is well preserved. Finally, the detection of ultracold deeply bound molecules is discussed.

Laser-free trapped ion entangling gates with AESE: adiabatic elimination of spin-motion entanglement

We discuss a laser-free, two-qubit geometric phase gate technique for generating high-fidelity entanglement between two trapped ions. The scheme works by ramping the spin-dependent force on and off slowly relative to the gate detunings, which adiabatically eliminates the spin-motion entanglement (AESE). We show how gates performed with AESE can eliminate spin-motion entanglement with multiple modes simultaneously, without having to specifically tune the control field detunings. This is because the spin-motion entanglement is suppressed by operating the control fields in a certain parametric limit, rather than by engineering an optimized control sequence. We also discuss physical implementations that use either electronic or ferromagnetic magnetic field gradients. In the latter, we show how to ‘AESE’ the system by smoothly turning on the effective spin-dependent force by shelving from a magnetic field insensitive state to a magnetic field sensitive state slowly relative to the gate mode frequencies. We show how to do this with a Rabi or adiabatic rapid passage transition. Finally, we show how gating with AESE significantly decreases the gate’s sensitivity to common sources of motional decoherence, making it easier to perform high-fidelity gates at Doppler temperatures.

Stereodynamical control of cold HD + D2 collisions.

We report full-dimensional quantum calculations of stereodynamic control of HD(v = 1, j = 2) + D2 collisions that has been probed experimentally by Perreault et al. using the Stark-induced adiabatic Raman passage (SARP) technique. Computations were performed on two highly accurate full-dimensional H4 potential energy surfaces. It is found that for both potential surfaces, rotational quenching of HD from with concurrent rotational excitation of D2 from is the dominant transition with cross sections four times larger than that of elastically scattered D2 for the same quenching transition in HD. This process was not considered in the original analysis of the SARP experiments that probed ΔjHD = -2 transitions in HD(vHD = 1, jHD = 2) + D2 collisions. Cross sections are characterized by an l = 3 resonance for ortho-D2(jD2 = 0) collisions, while both l = 1 and l = 3 resonances are observed for the para-D2(jD2 = 1) partner. While our results are in excellent agreement with prior measurements of elastic and inelastic differential cross sections, the agreement is less satisfactory with the SARP experiments, in particular for the transition for which the theoretical calculations indicate that D2 rotational excitation channel is the dominant inelastic process.

Temporal Quasi-Phase Matching Assists Robust Acoustic Adiabatic Passage

Recent work demonstrated stimulated Raman adiabatic passage-type transfer of energy along 3 acoustic cavities. After brief comments on the stimulated Raman adiabatic passage method, remarks on the scientific and technological relevance of this work are presented, followed by noting other recent important applications of the process.