The electric free-floating carsharing (FFCS) system is an emerging type of shared mobility and is widely adopted in urban areas due to its eco-friendliness, effectiveness, and flexibility. However, as most trips in FFCS are uni-directional, the distributions of vehicles in FFCS are usually spatially uneven. The operators of FFCS must relocate cars during the operation period to maintain the availability of cars to the users and improve the profitability of the system for dealing with imbalanced vehicle distribution caused by uneven demand. To optimize the relocation operations for FFCS operators, this study formulates the problem as a mixed-integer linear programming (MILP) model, which simultaneously addresses dynamic relocation, battery charging of electric vehicles, and scheduling of relocation staff in an FFCS with advanced reservation. A novel, efficient algorithm using a new structure of relocation tuples (RTs) is proposed to solve the problem that facilitates the search for feasible solutions using an RT exchange-based local search algorithm. Acceleration techniques are introduced to strengthen the solution search in large-scale scenarios. Numerical examples are used to evaluate the performance of the solution algorithm and validate the benefit of the proposed methodology. This shows that the methodology could be used by operators for decision-making at different levels.
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