Thrust generation through pulse-laser ablation has been proposed for use in propulsion systems in space. However, to achieve a high thrust performance, the energy efficiency must be improved and it is important to determine the behavior of the ablation plume to identify where energy losses occur. In this study, the ion-current distribution of a plume with aluminum ablation was measured. A neodymium-doped yttrium aluminum garnet (Nd:YAG) laser with a wavelength and pulse width of 1064 nm and 9±2 ns, respectively, was used for the ablation. Experiments were conducted at three different fluences: 10, 15, and 20 J/cm2. The fluence was varied in two ways: changing the beam-spot diameter while maintaining the single-pulse energy and changing the single-pulse energy while maintaining the beam-spot diameter. The ion current was measured at various angles using Faraday probes. The generated impulse and reduction mass were also measured. By combining and analyzing the results, the divergence angle of momentum, mean valence of ablated aluminum, and energy efficiencies of several processes were estimated.