137Cs Fluxes Research Articles

Impacts of farmland decontamination on 137Cs transfers in rivers after Fukushima nuclear accident: Evidence from a retrospective sediment core study

Following the Fukushima Daiichi Nuclear Power Plant disaster in March 2011, the Japanese government initiated an unprecedented decontamination programme to remediate 137Cs-contaminated soils and allow population return. This programme involved the removal of topsoil under farmland and residential land, and its replacement with “fresh soil” composed of granitic saprolite. However, decontamination was limited to these two land uses, without remediating forests, which cover 70 % of the surface area in the affected region. In this unprecedented context, the specific impact of this unique decontamination programme on 137Cs transfers in river systems remains to be quantified at the catchment scale. In this study, based on the analysis of a sediment core collected in June 2021 in the Mano Dam reservoir draining a decontaminated catchment, the effects of soil decontamination on particle-bound 137Cs dynamics and sediment source contributions in response to a succession of extreme precipitation events were retrospectively assessed. The sequence of sediment layer deposition and its chronology were reconstructed through the analysis of several diagnostic properties (organic matter, elemental geochemistry, visible colourimetry, granulometry) and contextual information. During abandonment (2011–2016), cropland contribution decreased (31 %). Concurrently, 137Cs activity and deposition flux decreased (19 and 29%year−1, respectively). Following decontamination (2017), sediment transfer increased (270 %) in response to increased contributions from decontaminated cropland and “fresh soil” (625 % and 180 % respectively). Meanwhile, forest contributions remained stable. In contrast, 137Cs activity dropped (65 %), although 137Cs deposition flux remained constant. Forests acted as a stable source of 137Cs. Accordingly, 137Cs deposition flux after decontamination (2016–2021) was similar to that observed during the 5-years period of land abandonment (2011–2016), as a result of the regrowth of spontaneous vegetation over farmland, protecting soil against erosion. Future research should further investigate the impact of longer land abandonment that prevailed in some regions decontaminated lately on the 137Cs fluxes in the rivers.

Reactivity and bioconcentration of stable cesium in a hyperturbid fluvial-estuarine continuum: A combination of field observations and geochemical modeling

Effective, post-accidental management needs an accurate understanding of the biogeochemical behavior of radionuclides in surface environments at a regional scale. Studies on stable isotopes (element homologs) can improve this knowledge. This work focuses on the biogeochemical behavior of stable cesium (Cs) along a major European fluvial-estuarine system, the Gironde Estuary (SW France). We present results obtained from (i) a long-term monitoring (2014–2017) of dissolved (Csd) and particulate (Csp) Cs concentrations at five sites along the freshwater continuum of the Garonne watershed, (ii) Csd and Csp concentrations during four oceanographic campaigns at contrasting hydrological conditions along longitudinal profiles of the estuarine system, (iii) a 24 h cycle of Csp at the estuary mouth, and (iv) a historical trend of Cs bioconcentration in wild oysters at the estuary mouth (RNO/ROCCH, 1984–2017). In addition, we model the partitioning of Cs within the estuarine environment for clay mineral interactions via PhreeqC. At fluvial sites, we observe a geogenic dependence of the Csp and a seasonal variability of Csd, with a downstream increase of the solid-liquid partitioning (log10 Kd values from 3.64 to 6.75 L kg−1) for suspended particulate matter (SPM) < 200 mg L−1. Along the estuarine salinity gradients, Cs shows a non-conservative behavior where fresh SPM (defined as Cs-depleted particles recently put in contact with Csd) act as a Cs sink during both flood and low discharge (drought) conditions. This sorption behavior was explained by the geochemical model, highlighting the relevance of ionic strength, water and SPM residence times. However, at high salinities, the overall log10 Kd value decreases from 6.02 to 5.20 for SPM ∼300–350 mg L−1 due to the Csd oceanic endmember. Despite wild oysters showing low bioconcentration factors (∼1220 L kg−1) at the estuary mouth, they are sensitive organisms to Cs fluxes.

Transport of radioactive materials from terrestrial to marine environments in Fukushima over the past decade

Abstract While 20 % of radionuclides released from the Fukushima Daiichi Nuclear Power Plant accident had been deposited in the terrestrial environment, rivers remain the long-term source for 137Cs, primarily through particulate transfer, from terrestrial to marine ecosystems. In this study, we estimated the suspended 137Cs flux to the ocean at 11 sites in the coastal area between October 2012 and December 2020 to be 17 TBq, based on our long-term monitoring data of concentrations of suspended 137Cs and suspended solids. The cumulative loss of suspended 137Cs from each site to the ocean ranged from 0.1 % to 1.7 % of initial deposition throughout the observation period, depending on the effect of dam lakes and normalized river discharge. The higher loss is also thought to be the large outflow of runoff during the typhoon. The current level of the suspended 137Cs concentrations was lowered to 1/10–1/100 of those immediately after the accident. The average value of the decreasing trend for each site was approximated using the equation: y = a1 e −k 1 t + a2 e −k 2t. The rate constant k 1 is higher in areas with intensive land use, such as pastures, bare land, and water surfaces, and k 2 is lower in urban areas.

Assessment of the input of particulate 239,240Pu and 137Cs from the Neman River into the Curonian Lagoon

The Curonian Lagoon is a unique system that is a temporary reservoir of water, accumulating about 62% of the suspended solids in the river runoff. The average activity of plutonium in the suspended particulate matter in the water of the Neris River was 0.26±0.02 Bq/kg, and the activity of 137Cs ranged from 23±8 to 49±12 Bq/kg. The average 137Cs flux to the Curonian Lagoon in the particulate and dissolved species was estimated to be (78±61) × 109 Bq/year. Preliminary estimates indicate that the annual input of 239,240Pu from the Neman River into the Curonian Lagoon is about 0.9 GBq, of which 0.56 GBq accumulates in the sediment of the lagoon.

Persistent impact of Fukushima decontamination on soil erosion and suspended sediment

In Fukushima, government-led decontamination reduced radiation risk and recovered 137Cs-contaminated soil, yet its long-term downstream impacts remain unclear. Here we provide the comprehensive decontamination impact assessment from 2013 to 2018 using governmental decontamination data, high-resolution satellite images and concurrent river monitoring results. We find that regional erosion potential intensified during decontamination (2013–2016) but decreased in the subsequent revegetation stage. Compared with 2013, suspended sediment at the 1-year-flood discharge increased by 237.1% in 2016. A mixing model suggests that the gradually increasing sediment from decontaminated regions caused a rapid particulate 137Cs decline, whereas no significant changes in downstream discharge-normalized 137Cs flux were observed after decontamination. Our findings demonstrate that upstream decontamination caused persistently excessive suspended sediment loads downstream, though with reduced 137Cs concentration, and that rapid vegetation recovery can shorten the duration of such unsustainable impacts. Future upstream remediation should thus consider pre-assessing local natural restoration and preparing appropriate revegetation measures in remediated regions for downstream sustainability.

Temporal variability of 137Cs concentrations in coastal sediments off Fukushima

Large amounts of radiocesium were released into marine environments following the Fukushima Daiichi Nuclear Power Plant accident in March 2011. Released radiocesium influenced not only marine environment but also marine biota in Fukushima. Since marine biota as fisheries products is important for Japanese market, it is important to assess the distribution of radiocesium in coastal environment off Fukushima for safety concerns of radioactive contamination. Radiocesium concentrations in sediments are important for understanding fishing ground conditions and for proving the safety of fisheries products in Fukushima. In this study, monthly monitoring data collected from May 2011 to March 2020 were analyzed to describe the temporal variability of 137Cs concentrations in coastal sediments off Fukushima (total of 3647 samples from eight lines at depths of 7–125 m off Fukushima, and three sites in Matsukawa-ura Lagoon). The 137Cs concentration in sediment showed a decreasing trend, but our nonlinear model fitting suggested that this rate of decrease had slowed down. Additionally, 137Cs concentrations were up to 4.08 times greater in shallow sampling sites (7, 10, 20 m depth) following heavy rainfall events (before five months vs. after five months), such as typhoons. These observations were consistent with increasing input from particulate 137Cs fluxes from rivers and increasing dissolved 137Cs concentrations in seawater. Finally, our numerical modeling suggested that riverine 137Cs input could maintain 137Cs concentrations in coastal sediment. These results indicate that riverine 137Cs input following heavy rainfall events is the main factor for maintaining 137Cs concentrations in coastal sediments near the Fukushima Daiichi Nuclear Power Plant.

A comparative study of riverine 137Cs dynamics during high-flow events at three contaminated river catchments in Fukushima

This study presents the temporal variations in riverine 137Cs concentrations and fluxes to the ocean during high-flow events in three coastal river catchments contaminated by the Fukushima Daiichi Nuclear Power Plant accident. River water samples were collected at points downstream in the Niida, Ukedo, and Takase Rivers during three high-flow events that occurred in 2019–2020. Variations in both the dissolved and particulate 137Cs concentrations appeared to reflect the spatial pattern of the 137Cs inventory in the catchments, rather than variations in physico-chemical properties of water and suspended solid. Negative relationships between the 137Cs concentration and δ15N in suspended solid were found in all rivers during the intense rainfall events, suggesting an increased contribution of sediment from forested areas to the elevation of particulate 137Cs concentration. The 137Cs flux ranged from 0.33 to 19 GBq, depending on the rainfall erosivity. The particulate 137Cs fluxes from the Ukedo River were relatively low compared with the other two rivers and were attributed to the effect of the Ogaki Dam reservoir upstream. The percentage of 137Cs desorbed in seawater relative to 137Cs in suspended solids ranged from 2.8% to 6.6% and tended to be higher with a higher fraction of exchangeable 137Cs. The estimated potential release of 137Cs desorbed from suspended solids to the ocean was 0.022–0.57 GBq, and its ratio to the direct flux of dissolved 137Cs was 0.12–6.2. Episodic sampling during high-flow events demonstrated that the particulate 137Cs flux depends on catchment characteristics and controls 137Cs transfer to the ocean.

Remobilisation of radiocaesium from bottom sediments to water column in reservoirs in Fukushima, Japan

Reservoir sediments generally act as a sink for radionuclides derived from nuclear accidents, but under anaerobic conditions, several radionuclides remobilise in bioavailable form from sediments to water columns, which may contribute to the long-term contamination of aquatic products. This study systematically investigated the 137Cs activities of sediment–pore water, providing a direct evidence of the remobilisation of bioavailable 137Cs from sediments in two highly contaminated reservoirs affected by the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident. We observed that the dissolved 137Cs activity concentration of pore water (3.0–65.8 Bq L−1) was one to two orders of magnitude higher than that of reservoir water. Moreover, the distribution coefficient (Kd) values for the 137Cs of sediment–pore water (2.6–14 × 103 L kg−1) decreased with depth. The Kd values were significantly and negatively correlated with the concentration of the major 137Cs competing cation NH4+. Our results strongly indicate a competitive ion exchange process between 137Cs and NH4+ via a highly selective interaction with the frayed edge sites of phyllosilicate minerals, which is the major reason for the variability of Kd values of sediment–pore water, even in the Fukushima case. Additionally, the sediment accumulation rates were relatively high, and the annual depositional rate of exchangeable 137Cs prevailed over the annual diffusive flux of 137Cs from the sediment to the overlying water. This finding indicates that even after 10 years since the FDNPP accident, the bioavailable 137Cs is still continuously supplied from the catchment covered by mountainous forests, and reservoir sediments are a long-term important source of bioavailable 137Cs in the riverine system. Our findings provide important parameter values for mid- and long-term assessments of the radiation impact of radionuclide discharges to freshwater environments.

Evaluation of contribution rate of the infiltrated water collected using zero-tension lysimeter to the downward migration of 137Cs derived from the FDNPP accident in a cedar forest soil

The vertical distribution of 137Cs in forest soil is important for predicting air dose rates and future cycling in forest ecosystems. However, there are many unexplained questions about the mechanisms of its downward migration. In this study, the 137Cs flux by rainfall infiltration was observed for three years from August 2017 using zero-tension lysimeters in a mature cedar forest where monitoring of the vertical distribution of 137Cs has been conducted since 2011. As a result, the 137Cs concentration in infiltrated water through the litter layer, 5 cm and 10 cm showed a tendency to be high in summer, but no such seasonal variation was found at 20 cm. Although the 137Cs inventory in the litter layer has been exponentially decreasing, the annual 137Cs fluxes in infiltrated water through the litter layer were almost the same in three years, and about 0.14–0.17% of the deposition density of 137Cs. Comparing these 137Cs fluxes with the apparent amounts of downward migration of 137Cs estimated from the change in the vertical distribution of 137Cs, the contribution rate of the infiltrated water to downward migration of 137Cs from litter to soil was calculated to be 8.5–17.7%. Similarly, the contribution rate in mineral soil layers was calculated to be 0.6–0.8% on a measured basis and estimated to be 3.0 ± 0.2% after correcting the amount of collected water, which is a problem with zero-tension lysimeter. It indicates that rainfall infiltration can explain a small part of the downward migration of 137Cs, thus further studies are required to clarify the contribution rate of remaining mechanisms such as advection-diffusion, colloidal transport, physical mixing, bioturbation, and growth and death of plant roots.

Vertical distribution and transport of radiocesium via branchflow and stemflow through the canopy of cedar and oak stands in the aftermath of the Fukushima Dai-ichi Nuclear Power Plant accident

Aiming to fill a need for data regarding radiocesium transport via both branchflow and stemflow through forests impacted by radioactive fallout, this study examined the vertical variation of radiocesium flux from branchflow and stemflow through the canopies of young Japanese cedar (Cryptomeria japonica (L. f.) D. Don) and Japanese oak (Quercus serrata Murray) trees in the aftermath of the Fukushima Dai-ichi Nuclear Power Plant accident. In forested areas approximately 40 km northwest of the location of the Fukushima Dai-ichi accident, the 137Cs concentration varied significantly among sampling periods and between the two forests, with the oak stand exhibiting higher 137Cs concentrations and depositional fluxes than the cedar stand. Expressed per unit trunk basal area, the depositional flux of 137Cs generated from the cedar and oak stands was 375 and 2810 Bq m−2 year−1, respectively. Of this total, 71% and 48% originated from the cedar and oak canopy, respectively, while the remainder originated from the trunk. Accordingly, the origin of radiocesium was more balanced for the oak stand with almost half of the flux coming from the canopy (48%) and the other half from the trunk (52%). Only about a quarter (29%) of the radiocesium flux originated from the trunk in Japanese cedar. Results from this work provide needed data that can enable a more thorough conceptualization of radiocesium cycling in forests. Coupling these empirical results with a physically-based model would likely lead to better forest management and proactive strategies for rehabilitating radioactively-contaminated forests and reducing the exposure risk of radiation dose rate for those that utilize forest products.

Validity of the source term for the Fukushima Dai-ichi Nuclear Power Station accident estimated using local-scale atmospheric dispersion simulations to reproduce the large-scale atmospheric dispersion of 137Cs

The source term of 137Cs from the Fukushima Dai-ichi Nuclear Power Station (FDNPS) accident was estimated from the results of local-scale atmospheric dispersion simulations and measurements. To confirm the source term's validity for reproducing the large-scale atmospheric dispersion of 137Cs, this study conducted hemispheric-scale atmospheric and oceanic dispersion simulations. In the dispersion simulations, the atmospheric-dispersion database system Worldwide version of System for Prediction of Environmental Emergency Dose Information (WSPEEDI)-DB and oceanic dispersion model SEA-GEARN-FDM that were developed by the Japan Atomic Energy Agency were used. Compared with the air concentrations of 137Cs measured by the Comprehensive Nuclear-Test-Ban Treaty Organization, overall, the WSPEEDI-DB simulations well reproduced the measurements, whereas the simulation results partly overestimated some measurements. Furthermore, the validity of the deposition of 137Cs by WSPEEDI-DB was investigated using SEA-GEARN-FDM and concentrations of 137Cs in seawater sampled from the North Pacific. Seawater concentrations of 137Cs by the oceanic dispersion simulation, in which the deposition flux of 137Cs by WSPEEDI-DB was used as input from the atmosphere to oceans, were statistically consistent to the measurement. However, the simulated seawater concentrations of 137Cs were underestimated regionally in the North Pacific. Both the overestimation of air concentrations and underestimation of seawater concentrations could be attributed to the less amounts of 137Cs deposition by less precipitation over the North Pacific. The overestimation and underestimation could be improved without contradiction between the air and seawater concentrations of 137Cs using more realistic precipitation in atmospheric dispersion simulations. This shows that the source term validated in this study could reproduce the spatiotemporal distribution of 137Cs from the FDNPS accident in both local and large-scale atmospheric dispersion simulations.

Significance of Fukushima-derived radiocaesium flux via river-estuary-ocean system

The environmental dynamics of Fukushima-derived radiocaesium from land to ocean and the impact of its flux on the marine environment are matters of concern because radiocaesium will be continually transported to the open ocean for the next several decades, or possibly more than one hundred years. In order to assess the distribution and flux of radiocaesium in a river-estuary-ocean system, we investigated the activity concentration of radiocaesium in Matsukawa-ura Lagoon, the largest lagoon in Fukushima, where it is very easy to carry out observations with a wide salinity gradient. Activity concentrations of dissolved 137Cs are elevated in seawater of low to intermediate salinity. It can thus be inferred that radiocaesium desorbs from suspended particles in an estuarine area. The porewater activity concentration of 137Cs in lagoon sediment was about 10 times higher than that in the overlying lagoon water. This direct measurement indicates that a significant amount of radiocaesium in sediment desorbs into porewater. From the results of a mass balance model, dissolved 137Cs flux from the lagoon's bottom is 15.3 ± 3.7 times greater than the riverine input, including desorption from particles. In the case of the whole Pacific coast of northeastern Japan (Miyagi, Fukushima, and Ibaraki Prefectures), dissolved 137Cs flux into the open ocean, including diffusion of porewater, is estimated to be up to 1.5 times greater than the sum of riverine input and the ongoing release from the Fukushima Dai-ichi Nuclear Power Station's harbor. Consequently, our results suggest that radiocaesium is transported to the open ocean under the control of various processes, not only by desorption from particles but also, for example, by the diffusion of porewater.

Importance of desorption process from Abukuma River's suspended particles in increasing dissolved 137Cs in coastal water during river-flood caused by typhoons

Desorption of radiocesium (137Cs) from riverine particles into seawater strongly influences 137Cs concentrations in coastal seawater. This process is important for quantifying the input of radionuclides to marine environments. Here we quantify the particulate 137Cs flux from the Abukuma River, Japan, during typhoon Hagibis and following typhoons in 2019 and estimate the resulting increased dissolved 137Cs levels in coastal seawater. Particulate 137Cs export flux, 1.1 × 1012 Bq, from the Abukuma River during the 4-day period of typhoon Hagibis (12–15 October 2019) equaled two-thirds of the annual flux during 2012–2015, the period of high 137Cs levels following the Fukushima Daiichi Nuclear Power Plant accident. The flux of the desorbed fraction from the Abukuma River during typhoon Hagibis was 0.061–0.12 × 1012Bq, and its daily flux to the surrounding coastal seawater (1.5–3.0 × 1010 Bq/d) was one to two orders of magnitude greater than the estimated input to the coastal seawater during the pre-typhoon period (1.3× 108–1.0 × 109 Bq/d). Simulated results suggest that the massive influx of riverine particles and subsequent desorption of 137Cs increased dissolved 137Cs levels in the coastal seawater by an order of magnitude, from 3.3 mBq/L (pre-typhoon level) to 45–126 mBq/L. This found pathway opens up new scenarios involving radionuclide dynamics in the boundary area of river-sea system.

Fine-tuning of 210Pb-based methods for dating vegetated saltmarsh sediments

Abstract Saltmarshes, wetlands, inter-tidal mudflats are highly productive natural ecosystems with significant ecological value. 210Pb and 137Cs have been used for establishing chronologies at a centennial scale in these sediments. They are relevant for assessing how saltmarshes are vulnerable to climate change, natural hazards and contamination from human inputs. This paper aims to review and adapt existing methods for the 210Pb-based radiometric dating of these sediments where the subterranean production and decay of OM are sources of achronicity. This limits the use of the basic assumption of considering the sediment as a continuous medium. From the available evidence, 210Pb fluxes onto sediments may be mediated by the activities bound to the mass flows, suggesting that models assuming a constant flux should be handled with care. The activity concentrations of excess 210Pb required by CF-CS, CIC and TERESA radiometric models must be those of the sediment mineral fraction, while CRS and PLUM can work with the composite sediment matrix. A review of these issues and application of the models is illustrated with new data from two recent saltmarsh sediment cores. The effects of non-ideal boundary conditions in radiometric dating and the system time-average of 137Cs fluxes are discussed. Although specific to vegetated saltmarshes, this topic and the present results have generic applications for other vegetated coastal sediments.

Impacts of freeze-thaw processes and subsequent runoff on 137Cs washoff from bare land in Fukushima

The deposited 137Cs is one of the long-lived radionuclides, that was released following the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident, has been hydrologically transported as particulates in the terrestrial environment of the Fukushima region. The impact of freeze-thaw processes and subsequent runoff affecting the 137Cs flux and concentration in sediment discharge were revealed in bare land erosion plot following the FDNPP accident by detailed monitoring and laser scanner measurement on the soil surface. We found that surface topographic changes due to the frost-heaving during the winter-spring period, and rill formation during the summer. We also found the evident seasonal changes in 137Cs concentration; high during the early spring and gradually decreased thereafter, then surface runoff from the plot frequently occurred during spring and autumn when rainfall was high and reached a maximum in summer. From these results, the higher 137Cs concentration in spring was caused by a mixture of unstable surface sediment following freeze-thaw processes and then transported in the early spring, but erosion amount is not significant because of the less rainfall event. The sediment with a lower 137Cs concentration, which was supplied from the rill erosion and its expansion, was wash-offed during the summer, contributing most of the flux from erosion in bare land in Fukushima region. In case, heavy rainfall occurs in the early spring, caution is required because high concentrations of cesium may flow down into the river.

Environmental change and human land‐use over the past 200 years in the Great Hinggan Mountains, Northeastern China

AbstractMountain ecosystems are sensitive to environmental changes and are affected by direct and indirect anthropogenic activities. This study sought to understand the impacts of human occupation, environmental and climate change on the Great Hinggan Mountains (GHM) in Northeastern China. The last 200 years of environmental changes are reconstructed by analyzing sediment cores from five small mountain lakes. Cores were dated using 210Pb and 137Cs radioisotopes, microscopic charcoal identified regional fire activity and fossil pollen analysis reconstructed temporal and spatial changes in vegetation. Peaks in 137Cs, 226Ra and microscopic charcoal flux were found to follow similar trends between sites. The radioisotope records reflect redistribution processes, such as erosion and fire events, which overwhelm the atmospheric fallout signal in the GHM. Microscopic charcoal increased from 1950 CE and peaked at all sites after 2000 CE suggesting that current fire management, coupled with a warmer climate due to global warming, may be leading to more wildfire events in the region. Pinus, Quercus and Betula declined at all sites as human occupation occurred in the early 1900s. Initially, open forest and grassland expanded in response to overexploitation of forests, followed by arboreal pollen reaching maximum values after 2000 CE. This study concludes that the present‐day mixed coniferous broad‐leaved forest dominating the southern region of the GHM is a product of changing fire activity, excessive logging and, more recently, forestry management and vegetation regeneration. Results suggest further management strategies are needed to address land degradation and wildfire events in mountain regions of Northeastern China.

Вміст 90Sr та 137Cs в депо і біогенних потоках типових насаджень Чорнобильської зони відчуження

The paper reports results of the study of depots and biogenic fluxes of 90Sr and 137Cs in the typical coniferous (Scots pine) and deciduous (Silver birch) forest ecosystems of the Chernobyl Exclusion Zone during 2016 - 2018. Data on activity concentrations and shares of the total activity of the studied radionuclides in the components of aboveground and underground biomass and their vertical distributions by 10 cm layers of the soil profile up to a depth of 1 m are presented. The downward and upward fluxes of 90Sr and 137Cs activity (including the processes of their deposition as a result of growth and formation biomass) are calculated in annual terms. Significantly higher 90Sr mobility in elements of forest ecosystems than 137Cs is confirmed. The estimated flux values for the investigated forest areas indicate a gradual further increase in the share of these radionuclides in the aboveground biomass components (up to 0.9 %·year-1 from the total activity in forest ecosystems) owing to the increase of organic matter stocks.

7Be, 210Pbatm and 137Cs in Snow Deposits in the Arctic Part of Western Siberia (Yamal-Nenets Autonomous District)

Radioactive isotopes (7Be, 210Pbatm and 137Cs) are used as indicators of processes associated with the transfer of matter from the atmosphere. Studying snow cover can provide information about the seasonal deposition flux of the isotopes to the Earth’s surface over the entire period of snow accumulation. The purpose of this study is to identify the features of 7Be, 210Pbatm and 137Cs deposition with the atmospheric precipitation in winter in the Arctic part of Western Siberia and to study the contribution of the particulate fractions of suspended matter in snow water to the total content of the radionuclides in samples of integrated seasonal snowfall. Snow samples were taken over a wide area along the highways around Novy Urengoy in April 2019. The suspended matter in snow samples was divided into three fractions. The isotopic composition was determined by high-resolution semiconductor gamma-spectrometry. The seasonal deposition flux of 7Be and 210Pbatm in the winter at the time of sampling averaged 58.7 and 25.2 Bq m−2 season−1, respectively. The average specific activity of 7Be and 210Pbatm in the snow water was 248.0 and 104.5 mBq L−1. The deposition flux of 137Cs from the atmosphere was low compared to 7Be and 210Pbatm and did not exceed 0.39 Bq m−2 season−1 at all sampling points. This indicates an insignificant modern flux of the radionuclide from the atmosphere. The separation of suspended matter in snow water by particulate fractions shows that the studied isotopes are present in all the extracted fractions: &gt;3, 0.45–3 and &lt;0.45 μm. The main part of 210Pbatm in all studied samples is in the coarse-grained fraction &gt;3 μm. Most 7Be is contained in finely dispersed aerosols, colloids, or a dissolved component (where the fraction &lt;0.45 μm). A significant increase in the contribution of coarse-grained fractions of suspended matter in snow water to the total activity of 7Be in snow precipitation was observed in territories with a higher anthropogenic impact.

Deposition processes over complex topographies: Experimental data meets atmospheric modeling

The present paper describes the assessment of the atmospheric deposition processes in a basin valley through a multidisciplinary approach based on the data collected within an extensive physico-chemical characterization of the soils, combined with the local meteorology. Surface soil cores were collected on a NNW-SSE transect across the Terni basin (Central Italy), between the Monti Martani and the Monti Sabini chains (956 m a.s.l.), featuring the heavily polluted urban and industrial enclave of Terni on its bottom. Airborne radiotracers, namely 210Pb and 137Cs, have been used to highlight atmospheric deposition.We observed an increased deposition flux of 210Pb and 137Cs at sites located at the highest altitudes, and the associated concentration profiles in soil allowed to evaluate the role of atmospheric deposition. We also obtained a comprehensive dataset of stable anthropogenic pollutants of atmospheric origin that showed heterogeneity along the transect. The behavior has been explained by the local characteristic of the soil, by seeder-feeder processes promoted by the atmospheric circulation, and was reconciled with the concentration profile of radiotracers by factor analysis. Finally, the substantial impact of the local industrial activities on soil profiles and the role of the planetary boundary layer has been discussed and supported by simulations employing a Lagrangian dispersion model.

Reservoir sediments as a long-term source of dissolved radiocaesium in water system; a mass balance case study of an artificial reservoir in Fukushima, Japan

Because of their large mobility and high bioavailability, it is necessary to elucidate the origins and dynamics of dissolved radionuclides in river and reservoir systems to assess the transfer of those radionuclides from water to crops and aquatic organisms. Elution from contaminated reservoir sediments, a potential source of dissolved radionuclides, presents a long-term concern, particularly for long-lived radionuclides. In this study, we systematically investigated caesium-137 (137Cs) concentrations using a time-series suite of input and output water samples collected from 2014 to 2019 from the Ogaki Dam Reservoir, which has a catchment with a high 137Cs inventory due to the Fukushima Dai-ichi Nuclear Power Plant accident. The results of our study showed that dissolved 137Cs concentration was significantly higher in the output water than that in the main input water, and that the effective ecological half-life of dissolved 137Cs in the output water was longer than in the main input water. We quantitatively evaluated the mass balance of dissolved 137Cs in the reservoir to elucidate how much dissolved 137Cs from the rivers and production from reservoir sediments contribute to 137Cs in the reservoir output. The annual output of dissolved 137Cs was significantly higher than the total input of dissolved 137Cs, with approximately 32%–40% of the dissolved 137Cs in the output water presumably being produced from reservoir sediments. Consequently, the estimated dissolved 137Cs fluxes from reservoir sediments to overlying water were 0.57–1.3 × 104 Bq m−2 y−1. This implies that approximately 0.04%–0.09% of 137Cs accumulated in the sediments was released through elution to the overlying water each year. Reservoir sediments containing high 137Cs levels may thus become even more important as sources of bioavailable dissolved 137Cs in the future.