Abstract
The Bronsted acid-catalyzed transformations of cyclic olefins in zeolites HZSM5 and H-mordenite were elucidated by the radiolysis/EPR method. Products of catalytic reactions were spin- labeled by radiolytic means and identified by using EPR spectroscopy. Comparison of reactions on HZSM5 and H-mordenite reveals strong shape selectivity on reactions in these catalysts. The radiolysis/EPR method is a new in situ spectroscopy with excellent sensitivity and structural specificity for the study of reaction mechanisms in zeolite catalysts.
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