Abstract

Using a two-carriers model and the Hikami-Larkin-Nagaoka (HLN) theory, we investigate the influence of large area patterning on magnetotransport properties in bismuth thin films with a thickness of 50 nm. The patterned systems have been produced by means of nanospheres lithography complemented by RF-plasma etching leading to highly ordered antidot arrays with the hexagonal symmetry and a variable antidot size. Simultaneous measurements of transverse and longitudinal magnetoresistance in a broad temperature range provided comprehensive data on transport properties and enabled us to extract the values of charge carrier densities and mobilities. Weak antilocalization signatures observed at low temperatures provided information on spin-orbit scattering length ranging from 20 to 30 nm, elastic scattering length of approx. 60 nm, and strong dependence on temperature phase coherence length. We show that in the absence of antidots the charge carrier transport follow 2-dimensional behavior and the dimensionality for phase-coherent processes changes from two to three dimensions at temperature higher than 10 K. For the antidot arrays, however, a decrease of the power law dephasing exponent is observed which is a sign of the 1D-2D crossover caused by the geometry of the system. This results in changes of scattering events probability and phase coherence lengths depending on the antidot diameters, which opens up opportunity to tailor the magnetotransport characteristics.

Highlights

  • Bismuth is a semimetal which has attracted substantial attention due to its distinctive electronic properties

  • We focused on the Bi antidot arrays fabricated by nanosphere lithography (NSL)

  • We investigated the influence of large area patterning, developed topography, and mesoscopic defects on the magnetotransport properties of Bi antidot arrays fabricated by nanosphere lithography and compared them to the flat reference layers

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Summary

Introduction

Bismuth is a semimetal which has attracted substantial attention due to its distinctive electronic properties These include low carrier density (few orders of magnitude smaller than those of most metals), small carrier effective mass of ~0.001 me , high carrier mobility reaching ~103 m2 /Vs in pure crystals, and long carrier mean free path exceeding 1 μm in single crystals [1,2,3,4]. It is an exceptional material for studying quantum mechanics in the solid state; many important physics phenomena, such as de Haas-van Alphen effect and quantum linear magnetoresistance, were first observed in Bi [5,6,7]. Another interesting system in this context are the arrays of Bi antidots, in which the correlation between the dimensionality and electronic

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