Abstract
For the purpose of alleviating the negative influence of rhodamine B (RhB) abuse on the environment, it is imperative to design a green and efficient photocatalyst for tackling organic dye-contaminated wastewater. Herein, a novel SiO2/g-C3N4/BiOBr/Bi (denoted as Si/CN/BiOB/Bi) photocatalyst with enhanced photodegradation activity has been successfully created. The influence of variable parameters including Bi doping amount, initial concentration of RhB, photocatalyst dosage, and reaction temperature on the photocatalytic performance of Si/CN/BiOB/Bi under visible light illumination are analyzed in detail. Results indicated that the degradation rate constant of RhB over Si/CN/BiOB/Bi-0.5 is 25.1, 18.1, and 2.2 times higher than that of CN, Si/CN, and Si/CN/BiOB, respectively. The Si/CN/BiOB/Bi-0.5 photocatalyst displayed high photocatalytic performance after 5 recycled runs. The improved photocatalytic performance can be attributed to the novel morphology as well as the excellent synergetic effects of Si/CN, BiOBr, and Bi, which enables the catalysts to accelerate the separation of photogenerated carriers. In brief, a new Si/CN/BiOB/Bi photocatalyst has a great application perspective for the purification of RhB wastewater.
Published Version
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