Abstract
The molecular beam electric resonance method has been used to measure the vibrational energy distribution of CsF produced in the chemical reactions Cs + SF 6 and SF 4. The reaction Cs + SF 6 yields a perfect Boltzmann distribution for the products CsF. For the reaction Cs + SF 4 a more complicated distribution has been found which, according to the molecular structure of SF 4, can be explained as a superposition of two Boltzmann distributions of different vibrational temperatures.
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