Abstract
AbstractRaman spectra of the ν1 bands of AsH3 have been obtained for the liquid state and for phase I of the solid state. It is shown that phase I is a plastic crystalline phase. A modeling procedure applied to the vibrational autocorrelation function shows that the modulation of the vibrational frequency is fast and that the vibrational dephasing is probably caused by the rotations. Evidence for a ν1‐ν3 Coriolis‐coupling effect is also presented.
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