Unusual dynamics of spin-[formula omitted] antiferromagnets on the triangular lattice in magnetic field

Abstract

We theoretically discuss dynamical properties of spin-12 Heisenberg antiferromagnet on the triangular lattice in magnetic field H. We use the recently proposed bond-operator theory which operates with quantum states of the whole magnetic unit cell containing three spins. This technique describes accurately short-range spin correlations and provides a quantitative description of elementary excitations which appear in other approaches as bound states of conventional low-energy quasiparticles (e.g., magnons). In quantitative agreement with previous numerical and analytical findings, we observe four phases with coplanar spin arrangements upon the field increasing: the three-sublattice Y-phase, the collinear “up-up-down” (UUD) state, the non-collinear V-phase, and the collinear fully polarized (FP) state. We demonstrate that apart from magnons (spin-1 quasiparticles) there are spin-0 elementary excitations in the UUD state one of which is long lived and its spectrum lies below magnon branches. This mode originates from a high-energy quasiparticle at H=0 and it produces anomalies only in the longitudinal spin correlator because longitudinal and transverse channels are separated in collinear states. All other spin-0 excitations have finite lifetime and produce visibly anomalies in the dynamical structure factor. In the V-phase, we obtain multiple short-wavelength spin excitations which have no counterparts in the semiclassical spin-wave theory. Besides, we demonstrate a highly nontrivial field evolution of quasiparticles spectra on the way from one collinear state (UUD) to another one (FP) via the non-collinear V-phase (in which the longitudinal and the transverse channels are mixed). In particular, some parts of the spin-0 branch in the UUD state become parts of the spin-1 (magnon) branch in the FP phase whereas some parts of one magnon branch turn into parts of spin-2 branch. Such evolution would be very difficult to find by any conventional analytical approach. Our results are in good agreement with neutron experimental data obtained recently in Ba3CoSb2O9, KYbSe2, and CsYbSe2.