Abstract

Hund metals have attracted attention in recent years due to their unconventional superconductivity, which supposedly originates from non-Fermi-liquid (NFL) properties of the normal state. When studying Hund metals using dynamical mean-field theory, one arrives at a self-consistent "Hund impurity problem" involving a multiorbital quantum impurity with nonzero Hund coupling interacting with a metallic bath. If its spin and orbital degrees of freedom are screened at different energy scales, $T_\mathrm{sp} < T_\mathrm{orb}$, the intermediate energy window is governed by a novel NFL fixed point, whose nature had not yet been clarified. We resolve this problem by providing an analytical solution of a paradigmatic example of a Hund impurity problem, involving two spin and three orbital degrees of freedom. To this end, we combine a state-of-the-art implementation of the numerical renormalization group, capable of exploiting non-Abelian symmetries, with a generalization of Affleck and Ludwig's conformal field theory (CFT) approach for multichannel Kondo models. We characterize the NFL fixed point of Hund metals in detail for a Kondo model with an impurity forming an SU(2)$\times$SU(3) spin-orbital multiplet, tuned such that the NFL energy window is very wide. The impurity's spin and orbital susceptibilities then exhibit striking power-law behavior, which we explain using CFT arguments. We find excellent agreement between CFT predictions and numerical renormalization group results. Our main physical conclusion is that the regime of spin-orbital separation, where orbital degrees of freedom have been screened but spin degrees of freedom have not, features anomalously strong local spin fluctuations: the impurity susceptibility increases as $\chi_\mathrm{sp}^\mathrm{imp} \sim \omega^{-\gamma}$, with $\gamma > 1$.

Highlights

  • The chain is diagonalized iteratively while discarding high-energy states, thereby zooming in on low-energy properties: the level spacing of a chain ending at site k is of order ωk ∝ Λ−k=2, where Λ > 1 is a discretization parameter

  • Ðq; S; λÞ are shown at the top, and → indicates boundary operators obtained via double fusion. (NRG parameters: Λ 1⁄4 2.5; number of kept multiplets, Nkeep 1⁄4 3000; half-bandwidth of the bath, D 1⁄4 1.) (b) Illustrations of the ground states encountered during the flow. (c),(d) Imaginary part of the spin and orbital susceptibilities of (c) the impurity and (d) the bath site coupled to it (Wilson chain site k 1⁄4 0)

  • We provide technical details for our conformal field theory (CFT) analysis of the NFL and FL fixed points of the three-orbital Kondo model discussed in Secs

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Summary

Introduction

Hund metals are multiorbital materials with broad bands which are correlated via the ferromagnetic Hund coupling JH, rather than the Hubbard interaction U. The coupling JH implements Hund’s rule, favoring electronic states with maximal spin, which causes Hund metals to be fundamentally different from Mott insulators. This is a new exciting area of condensed matter physics; for a recent review with numerous references, see Ref. Hund metals are a very diverse class of materials, including transition metal oxides

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