Abstract

Time-resolved and ultrafast hard X-ray imaging, scattering and spectroscopy are powerful tools for elucidating the temporal and spatial evolution of complexity in materials. However, their temporal resolution has been limited by the storage-ring timing patterns and X-ray pulse width at synchrotron sources. Here we demonstrate that dynamic X-ray optics based on micro-electro-mechanical-system resonators can manipulate hard X-ray pulses on time scales down to 300 ps, comparable to the X-ray pulse width from typical synchrotron sources. This is achieved by timing the resonators with the storage ring to diffract X-ray pulses through the narrow Bragg peak of the single-crystalline material. Angular velocities exceeding 107 degrees s−1 are reached while maintaining the maximum linear velocity well below the sonic speed and material breakdown limit. As the time scale of the devices shortens, the devices promise to spatially disperse the temporal width of X-rays, thus generating a temporal resolution below the pulse-width limit.

Highlights

  • Time-resolved and ultrafast hard X-ray imaging, scattering and spectroscopy are powerful tools for elucidating the temporal and spatial evolution of complexity in materials

  • While X-ray free-electron lasers (XFELs) with a femtosecond pulse width are extremely effective in probing dynamics on ultrashort time scales, synchrotron-based X-ray sources are well suited for revealing the spatiotemporal evolution of mesoscopic details in materials

  • We demonstrate that a MEMS-based X-ray dynamic optics, oscillating with a frequency matched to a synchrotron storage ring with a 1.1-km circumference, can control and manipulate hard X-ray pulses significantly below one nanosecond at 300 ps

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Summary

Introduction

Time-resolved and ultrafast hard X-ray imaging, scattering and spectroscopy are powerful tools for elucidating the temporal and spatial evolution of complexity in materials Their temporal resolution has been limited by the storage-ring timing patterns and X-ray pulse width at synchrotron sources. We demonstrate that a MEMS-based X-ray dynamic optics, oscillating with a frequency matched to a synchrotron storage ring with a 1.1-km circumference, can control and manipulate hard X-ray pulses significantly below one nanosecond at 300 ps. With this exceptional time scale, we are one step closer to achieving pulse streaking and pulse slicing that would allow us to access information at a sub-pulse temporal scale

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