Abstract
A two-dimensional (2D) model of infiltration-mediated combustion in a porous sample with all boundaries closed to gas penetration except for one open to exchange with a large bath of gas is considered. Numerical analysis with account of heat losses through the side surface has shown that the profile of gas pressure is substantially two-dimensional. Due to heat losses, the transversal gas flow begins to occur from a cold wall (where there is no reaction and gas consumption) to the sample center (where gas is deficient). As a result, the distribution of conversion degree over sample cross sections exhibits a maximum near the side surface, which reasonably agrees with the experimental data obtained for combustion of tantalum powder in nitrogen gas in quartz tubes.
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More From: International Journal of Self-Propagating High-Temperature Synthesis
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