Abstract
We demonstrate electrical tunnel spin injection from a ferromagnet to graphene through a high-quality Al2O3 grown by atomic layer deposition (ALD). The graphene surface is functionalized with a self-assembled monolayer of 3,4,9,10-perylene tetracarboxylic acid (PTCA) to promote adhesion and growth of Al2O3 with a smooth surface. Using this composite tunnel barrier of ALD-Al2O3 and PTCA, a spin injection signal of ∼30Ω has been observed from non-local magnetoresistance measurements at 45K, revealing potentially high performance of ALD-Al2O3/PTCA tunnel barrier for spin injection into graphene.
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