Abstract
Progress in experimental techniques at nanoscale makes measurements of noise in molecular junctions possible. These data are important source of information not accessible through average flux measurements. The emergence of optoelectronics, the recently shown possibility of strong light-matter couplings, and developments in the field of quantum thermodynamics are making measurements of transport statistics even more important. Theoretical methods for noise evaluation in first principles simulations can be roughly divided into approaches for weak intra-system interactions, and those treating strong interactions for systems weakly coupled to baths. We argue that due to structure of its diagrammatic expansion, and the use of many-body states as a basis of its formulation, the recently introduced nonequilibrium diagrammatic technique for Hubbard Green functions is a relatively inexpensive method suitable for evaluation of noise characteristics in first principles simulations over a wide range of parameters. We illustrate viability of the approach by simulations of noise and noise spectrum within generic models for non-, weakly and strongly interacting systems. Results of the simulations are compared to exact data (where available) and to simulations performed within approaches best suited for each of the three parameter regimes.
Highlights
The theoretical concept of full counting statistics was originally proposed by Levitov and Lesovik[19, 20], and further developed in numerous studies[1]
We note in passing that earlier studies of Hubbard NEGF53, 54 were restricted to the evaluation of two-time correlation functions only, while simulation of noise spectrum requires evaluation of multi-time correlation functions
Results of simulations show that the Hubbard nonequilibrium Green function (NEGF) is an inexpensive method capable to reproduce satisfactory noise characteristics of junctions over a wide range of parameters
Summary
The theoretical concept of full counting statistics was originally proposed by Levitov and Lesovik[19, 20], and further developed in numerous studies[1]. We present noise simulation in model systems within the Hubbard NEGF, comparing results to those of other approaches. Note that Lindblad/Redfield QME does not yield noise spectrum; current and zero-frequency noise were simulated within the FCS
Published Version (
Free)
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have