Abstract
We explore the possibility of tomographic imaging the difference between the helium 1s2s triplet and singlet states using high-order harmonic generation. The harmonic spectrum from helium is studied using the rescattering model with multielectron-formulated dipole moments incorporated. By performing a numerical simulation of one-dimensional model helium atoms in a laser pulse, we show that the modified rescattering model correctly predicted the minimum positions of harmonic spectra. The harmonic spectrum is shown related to the multielectron recombination dipole moment by a shape factor. We further demonstrate that the topological difference between the singlet and triplet wavefunctions can be recognized from functions constructed using the harmonic signals.
Published Version
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