Time-dependent variational approach to solve multi-dimensional time-dependent Schrödinger equation

Abstract

We present an efficient approach to solve multi-dimensional time-dependent Schrödinger equation (TDSE) in an intense laser field. In this approach, each spatial degree of freedom is treated as a distinguishable quasi-particle. The non-separable Coulomb potential is regarded as a two-body operator between different quasi-particles. The time-dependent variational principle is used to derive the equations of motion. Then the high-order multi-dimensional problem is broken down into several lower-order coupled equations, which can be efficiently solved. As a demonstration, we apply this method to solve the two-dimensional TDSE. The accuracy is tested by comparing the direct solutions of TDSE using several examples such as the strong-field ionization and the high harmonic generation. The results show that the present method is much more computationally efficient than the conventional one without sacrificing accuracy. The present method can be straightforwardly extended to three-dimensional problems. Our study provides a flexible method to investigate the laser-atom interaction in the nonperturbative regime.