Abstract
A free energy minimization procedure is presented for the evaluation of the association equilibrium of nonideal electrolytes in the mean spherical approximation (MSA). This model is applied to electrostatic Bjerrum association of 2-2 electrolytes in water, to chemical association of 1-1 electrolytes in low dielectric constant media, and to weak electrolytes in water. The present model is also applicable to mixtures of associating electrolytes
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