Abstract
We present a theoretical study of doubly resonant three-photon ionization with radiation of sufficiently broad bandwidth to overlap all hyperfine levels of the resonant intermediate states. We demonstrate that isotopic selectivity in ionization is apt to occur under a variety of circumstances, although the degree may vary from negligible to quite significant, depending on the relative values of atomic and radiation parameters. Our theory provides a satisfactory quantitative interpretation of recent experimental data in Sn.
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More From: Physical review. A, Atomic, molecular, and optical physics
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